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Related papers: Quantum coherent contributions in biological elect…

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Studies of nanoscale biological transport often use a mean-field approximation that is exact only when the system is at equilibrium and there are no interactions between particles on different sites in the network. We explore the…

Biological Physics · Physics 2022-11-01 Kiriko Terai , Jonathon L. Yuly , Peng Zhang , David N. Beratan

The century-long Michaelis-Menten rate law and its modifications in the modeling of biochemical rate processes stand on the assumption that the concentration of the complex of interacting molecules, at each moment, rapidly approaches an…

Molecular Networks · Quantitative Biology 2024-11-25 Junghun Chae , Roktaek Lim , Thomas L. P. Martin , Cheol-Min Ghim , Pan-Jun Kim

It is believed that the quantum coherence itself cannot explain the very high excitation energy transfer (EET) efficiency in the Fenna-Matthews-Olson (FMO) complex. In this paper, we show that this is not the case if the inter-site…

Biological Physics · Physics 2015-06-11 X. X. Yi , X. Y. Zhang , C. H. Oh

Objective: The bidomain model and the finite element method are an established standard to mathematically describe cardiac electrophysiology, but are both suboptimal choices for fast and large-scale simulations due to high computational…

Resonant energy transfers, i.e. the non-radiative redistribution of an electronic excitation between two particles coupled by the dipole-dipole interaction, lie at the heart of a variety of chemical and biological phenomena, most notably…

Understanding the mechanisms of efficient and robust energy transfer in organic systems provides us with new insights for the optimal design of artificial systems. In this paper, we explore the dynamics of excitation energy transfer (EET)…

Chemical Physics · Physics 2015-05-12 M. Qin , H. Z. Shen , X. L. Zhao , X. X. Yi

Photosystem II (PSII) reaction center is a unique protein-chromophore complex that is capable of efficiently separating electronic charges across the membrane after photoexcitation. In the PSII reaction center, the primary energy- and…

Hysteresis in organic electrochemical transistors (OECT) is a basic effect in which the measured current depends on the voltage sweep direction and velocity. This phenomenon has an important impact on different aspects of the application of…

Applied Physics · Physics 2024-04-29 Juan Bisquert , Baurzhan Ilyassov , Nir Tessler

A metal near the topological transition can be loosely viewed as consisting of two groups of electrons. First group are "bulk" electrons occupying most of the Brillouin zone. Second group are electrons with wave vectors close to the…

Disordered Systems and Neural Networks · Physics 2019-10-30 C. C. A. Houghton , E. G. Mishchenko , M. E. Raikh

In this paper, we study the role of collective vibrational motion in the phenomenon of electronic energy transfer (EET) along a chain of coupled electronic dipoles with varying excitation frequencies. Previous experimental work on EET in…

Quantum Physics · Physics 2015-03-13 F. L. Semião , K. Furuya , G. J. Milburn

Electron transfer is an important and fundamental process in chemistry, biology and physics, and has received significant attention in recent years. Perhaps one of the most intriguing questions concerns with the realization of the…

Mesoscale and Nanoscale Physics · Physics 2023-05-30 Bokang Hou , Michael Thoss , Uri Banin , Eran Rabani

Electronic Energy Transfer (EET) between chromophores is fundamental in many natural light-harvesting complexes, serving as a critical step for solar energy funneling in photosynthetic plants and bacteria. The complicated role of the…

Chemical Physics · Physics 2024-02-05 Colin Coane , Marco Romanelli , Giulia Dall'Osto , Rosa Di Felice , Stefano Corni

Iron-sulfur clusters conduct a wide variety of biochemical reactions that are conserved across all domains of life. The hyperfine structure of reactive ligands of these clusters can be studied experimentally and theoretically by means of…

Chemical Physics · Physics 2025-08-22 William C. Robinson , Victoria Pascutti , David A. Hall , Martín A. Mosquera

In this contribution we present calculations performed for interacting electron systems within a non-perturbative formulation of the cluster theory. Extrapolation of the model to describe the time dependence of the interacting systems is…

Atomic Physics · Physics 2009-11-13 M. Tomaselli , T. Kuehl , D. Ursescu , S. Fritzsche

We study an intermediate quantum coherent-incoherent charge transport mechanism in metal-molecule-metal junctions using B\"uttiker's probe technique. This tool allows us to include incoherent effects in a controlled manner, and thus to…

Mesoscale and Nanoscale Physics · Physics 2017-04-12 Hyehwang Kim , Michael Kilgour , Dvira Segal

We consider the dependence of the electron transfer in photosynthetic complexes on correlation properties of random fluctuations of the protein environment. The electron subsystem is modeled by a finite network of connected electron…

Biological Physics · Physics 2015-06-23 Alexander I. Nesterov , Gennady P. Berman

Electron-phonon relaxation in size-quantized systems may become inhibited when the spacing of discrete electron energy levels exceeds the magnitude of the phonon frequency. We show, however, that nanoclusters can support a fast nonradiative…

Atomic and Molecular Clusters · Physics 2007-05-23 Vitaly V. Kresin , Yu. N. Ovchinnikov

Chlorosomes are the largest and most efficient natural light-harvesting antenna systems. They contain thousands of pigment molecules - bacteriochlorophylls (BChls)- that are organized into supramolecular aggregates and form a very efficient…

Chemical Physics · Physics 2014-05-13 Takatoshi Fujita , Joonsuk Huh , Semion K. Saikin , Jennifer C. Brookes , Alan Aspuru-Guzik

Inclusive electron scattering off few-nucleon systems is investigated at $x>1$ and high momentum transfer, including the contributions from quasi-elastic and deep inelastic scattering processes. It is shown that at $x>1$ the inclusive cross…

Nuclear Theory · Physics 2011-04-15 S. Simula

Photosynthetic proteins have evolved over billions of years so as to undergo optimal energy transfer to the sites of charge separation. Based on spectroscopically detected quantum coherences, it has been suggested that this energy transfer…

Chemical Physics · Physics 2016-07-13 David Paleček , Petra Edlund , Sebastian Westenhoff , Donatas Zigmantas