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We present a detailed study of the structural, electronic, magnetic and ferroelectric properties of prototypical \textit{proper} and \textit{improper} multiferroic (MF) systems such as BiFeO$_{3}$ and orthorhombic HoMnO$_{3}$, respectively,…

Materials Science · Physics 2017-03-15 A. Stroppa , S. Picozzi

In this work, we developed and showcased the occ-RI-K algorithm to compute the exact exchange contribution in density functional calculations of solids near the basis set limit. Within the gaussian planewave (GPW) density fitting, our…

Chemical Physics · Physics 2022-11-09 Joonho Lee , Adam Rettig , Xintian Feng , Evgeny Epifanovsky , Martin Head-Gordon

A computational study of the Electron Paramagnetic Resonance (EPR) $g$-tensors and hyperfine tensors of Li and Ga vacancies in LiGaO$_2$ is presented. Density Functinal Theory (DFT) calculations are carried out of the Ga and Li vacancies…

Materials Science · Physics 2020-04-22 Dmitry Skachkov , Walter Lambrecht , Klichchupong Dabsamut , Adisak Boonchun

Spin-polarized density functional calculations, magnetization, and neutron diffraction measurements are carried out to investigate the magnetic exchange interactions and strong correlation effects in Yb substituted inverse spinel nickel…

Materials Science · Physics 2017-07-26 Kodam Ugendar , S. Samanta , Sudhendra Rayaprol , V. Siruguri , G. Markandeyulu , B. R. K. Nanda

Positional polymorphism in solids refers to locally disordered unit cells that, on average, reproduce the high-symmetry structures observed in diffraction experiments. Standard theories of electron-phonon interactions fail to describe the…

The well-known spatial integration schemes in molecular electronic structure theory, immune to cusps and point singularities of some kind at atomic positions, use a set of weighting functions to split the integrand into a sum of…

Chemical Physics · Physics 2022-09-14 Dimitri N. Laikov

The effect of a magnetic (S=1/2) impurity coupled to a 2D system of correlated electrons (described by the t--J model) is studied by exact diagonalisations. It is found that, if the exchange coupling of the impurity with the neighboring…

Condensed Matter · Physics 2016-08-31 D. Poilblanc , D. J. Scalapino , W. Hanke

We employ magnetocapacitance and far-infrared spectroscopy techniques to study the spectrum of the double-layer electron system in a parabolic quantum well with a narrow tunnel barrier in the centre. For gate-bias-controlled asymmetric…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 V. T. Dolgopolov , A. A. Shashkin , E. V. Deviatov , F. Hastreiter , M. Hartung , A. Wixforth , K. L. Campman , A. C. Gossard

The study of the hyperfine anomaly of neutron rich nuclei, in particular, neutron halo nuclei, can give a very specific and unique way to measure their neutron distribution and confirm a halo structure. The hyperfine structure anomaly in…

Nuclear Theory · Physics 2009-08-18 Y. L. Parfenova , Ch. Leclercq-Willain

The study of zinc oxide, within the homogeneous electron gas approximation, results in overhybridization of zinc $3d$ shell with oxygen $2p$ shell, a problem shown for most transition metal chalcogenides. This problem can be partially…

Using a linear combination of atomic orbitals approach, we report a systematic comparison of various Density Functional Theory (DFT) and hybrid exchange-correlation functionals for the prediction of the electronic and structural properties…

Materials Science · Physics 2008-05-07 D. I. Bilc , R. Orlando , R. Shaltaf , G. -M. Rignanese , Jorge Íñiguez , Ph. Ghosez

The isolated substitutional gold impurity in bulk silicon is studied in detail using electronic structure calculations based on density-functional theory. The defect system is found to be a non-spin-polarized negative-U centre, thus…

Materials Science · Physics 2014-03-26 Fabiano Corsetti , Arash A. Mostofi

Motivated by the recently renewed interest in the superconducting bismuth perovskites, we investigate the electronic structure of the parent compounds ABiO$_{3}$ (A= Sr, Ba) using $ab$ $initio$ methods and tight-binding (TB) modeling. We…

Materials Science · Physics 2018-02-06 Arash Khazraie , Kateryna Foyevtsova , Ilya Elfimov , George A. Sawatzky

When described through a plane-wave basis set, the inclusion of exact nonlocal exchange in hybrid functionals gives rise to a singularity, which slows down the convergence with the density of sampled $k$ points in reciprocal space. In this…

Materials Science · Physics 2009-09-10 Peter Broqvist , Audrius Alkauskas , Alfredo Pasquarello

The energy positions of frontier orbitals in organic electronic materials are often studied experimentally by (inverse) photoemission spectroscopy and theoretically within density functional theory. However, standard exchange-correlation…

Most torsional barriers are predicted to high accuracy (about 1kJ/mol) by standard semilocal functionals, but a small subset has been found to have much larger errors. We create a database of almost 300 carbon-carbon torsional barriers,…

Chemical Physics · Physics 2021-02-16 Seungsoo Nam , Eunbyol Cho , Kieron Burke , Eunji Sim

Using a tight-binding Hamiltonian for phosphorene, we have calculated the real part of the polarizability and the corresponding dielectric function, Re$[\epsilon(\textbf{q},\omega)]$, at zero temperature (T = 0) with free carrier density…

Computational Physics · Physics 2018-09-11 Po Hsin Shih , Thi Nga Do , Godfrey Gumbs , Dipendra Dahal

We carried out Heyd-Scuseria-Ernzerhof hybrid density functional theory plane wave supercell calculations in wurtzite aluminum nitride in order to characterize the geometry, formation energies, transition levels and hyperfine tensors of the…

Materials Science · Physics 2014-11-27 A. Szállás , K. Szász , X. T. Trinh , N. T. Son , E. Janzén , A. Gali

A self-consistent scheme for determining the optimal fraction of exact exchange for full-range hybrid functionals is presented and applied to the calculation of band gaps and dielectric constants of solids. The exchange-correlation…

Materials Science · Physics 2015-01-15 Jonathan H Skone , Marco Govoni , Giulia Galli

We apply local orbital basis density functional theory (using SIESTA) coupled with a mapping to the Anderson impurity model to estimate the Coulomb assisted or correlated hybridization between transition metal d-orbitals and ligand…

Strongly Correlated Electrons · Physics 2009-11-11 A. Huebsch , J. C. Lin , J. Pan , D. L. Cox