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Abrupt time variations of the properties of optical materials have been at the center of intense research efforts in recent years, with the prospect of enabling extreme wave transformations and of leveraging time as a degree of freedom for…

Pump-probe spectroscopy is central for exploring ultrafast dynamics of fundamental excitations, collective modes and energy transfer processes. Typically carried out using conventional diffraction-limited optics, pump-probe experiments…

We study noise propagation dynamics in a femtosecond oscillator by injecting external noise on the pump intensity. We utilize a spectrally-resolved homodyne detection technique that enables simultaneous measurement of amplitude and phase…

Femtosecond pump-probe spectroscopy is applied to identify transient optical signatures of phase transitions in optimally doped YBa2Cu3O7-{\delta} films. To elucidate the dynamics of superconducting and pseudogap phases, the slow thermal…

Superconductivity · Physics 2015-06-12 Chunfeng Zhang , Wei Li , B. Gray , Bin He , Ye Wang , Fan Yang , Xiaoyong Wang , J. Chakhalian , Min Xiao

The classical pump-probe scheme for experiments with femtosecond laser is proposed to use for study the inequality of forward and reversed transitions in optics.

Optics · Physics 2007-05-23 V. A. Kuz'menko

We demonstrate a femtosecond pump-probe spectrometer which utilizes a white light supercontinuum as input, and relies on mutual synchronization of acousto-optical chopper, pump-probe delay stage and the CCD camera to record shot-to-shot…

Chemical Physics · Physics 2022-12-27 Vivek N. Bhat , Asha S. Thomas , Vivek Tiwari

We measure the photoionization cross-section of vibrationally excited levels in the S2 state of azulene by femtosecond pump-probe spectroscopy. At the wavelengths studied (349-265 nm in the pump) the transient signals exhibit two distinct…

Carrier and phonon dynamics in Bi2Se3 crystals are studied by a spatially resolved ultrafast pump-probe technique. Pronounced oscillations in differential reflection are observed with two distinct frequencies, and are attributed to coherent…

Mesoscale and Nanoscale Physics · Physics 2011-06-08 Nardeep Kumar , Brian A. Ruzicka , N. P. Butch , P. Syers , K. Kirshenbaum , J. Paglione , Hui Zhao

We present a novel optical transient absorption and reflection microscope based on a diffraction-limited pump pulse in combination with a wide-field probe pulse, for the spatio-temporal investigation of ultrafast population transport in…

Two-color side-view probing of light-matter interaction from minute focal volume of a tightly focused fs-laser pump pulse reveals charge dynamics with high 0.9 micrometers optical resolution and approximately ~20 fs temporal resolution in…

Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…

Optics · Physics 2021-04-07 Jun Jiang , David Grass , Yue Zhou , Warren S. Warren , Martin C. Fischer

We report ultrafast response of femtosecond photoexcited carriers in single layer reduced graphene oxide flakes suspended in water as well as few layer thick film deposited on indium tin oxide coated glass plate using pump-probe…

Materials Science · Physics 2011-06-30 Sunil Kumar , N. Kamaraju , K. S. Vasu , A. K. Sood

We demonstrate pump-probe techniques, namely the Doppler spectrometry and the reflectometry in detail, which directly capture the time-resolved ultrafast evolution of high intensity femtosecond laser-driven hot, dense plasma. These…

Atomically-thin molybdenum disulfide is emerging as a new nanomaterial with potential applications in the fields of electronic and photonics. Charge carrier dynamics plays an essential role in determining its electronic and optical…

Mesoscale and Nanoscale Physics · Physics 2012-07-09 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

Femtosecond time-resolved spectroscopy using 400 nm-pump and 800 nm-probe in CVD-grown multilayer graphene provides strong evidence for isotropic distribution of photoexcited carrier after initial relaxation. Indicative of such isotropic…

Mesoscale and Nanoscale Physics · Physics 2013-12-24 Xiao-Qing Yan , Zhi-Bo Liu , Jun Yao , Xin Zhao , Xu-Dong Chen , Yongsheng Chen , Jian-Guo Tian

A numerical method to calculate optical conductivity based on a pump-probe setup is presented. Its validity and limits are tested and demonstrated via the concrete numerical simulations on the half-filled one-dimensional extended Hubbard…

Strongly Correlated Electrons · Physics 2016-05-26 Can Shao , Takami Tohyama , Hong-Gang Luo , Hantao Lu

We discuss nonlinear spectra of selective reflection from high-density rubidium atomic vapor, where the self-broadening of the resonant transition $5S_{1/2}-5P_{3/2}$ dominates over the Doppler width. In the experiments, the hole-burning…

Atomic Physics · Physics 2026-01-16 V. A. Sautenkov , S. A. Saakyan , A. A. Bobrov , B. B. Zelener

The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond…

Quantum Physics · Physics 2015-06-22 Allan S. Johnson , Joel Yuen-Zhou , Alán Aspuru-Guzik , Jacob J. Krich

Spatiotemporal dynamics of excitons in isolated semiconducting single-walled carbon nanotubes are studied using transient absorption microscopy. Differential reflection and transmission of an 810-nm probe pulse after excitation by a 750-nm…

Mesoscale and Nanoscale Physics · Physics 2013-01-08 Brian A. Ruzicka , Rui Wang , Jessica Lohrman , Shenqiang Ren , Hui Zhao

Most of the vibrating mechanisms of optofluidicsystems are based on local heating of membranes that in-duces liquid flow. We report here a new type of diaphragmpump in a liquid film based on the optical radiation pres-sure force. We…

Optics · Physics 2017-01-09 Olivier Emile , Janine Emile