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Using first principles calculations, we study the microscopic origin of ferroelectricity (FE) induced by magnetic order in the orthorhombic HoMnO3. We obtain the largest ferroelectric polarization observed in the whole class of improper…

Materials Science · Physics 2009-11-13 Silvia Picozzi , Kunihiko Yamauchi , Biplab Sanyal , Ivan A. Sergienko , Elbio Dagotto

The ferroelectricity of multiferroics induced by spin order is commonly explained by considering either purely electronic or ion-displacement contribution. However, there is no general model which includes both effects simultaneously. Here,…

Strongly Correlated Electrons · Physics 2014-10-01 H. J. Xiang , P. S. Wang , M. -H. Whangbo , X. G. Gong

Ferroelectricity has been found to occur in several insulating systems, such as TbMnO$_3$ (TMO) and Ni$_3$V$_2$O$_8$ (NVO) which have more than one phase with incommensurately modulated long-range magnetic order. Here we give a…

Materials Science · Physics 2009-11-11 A. Brooks Harris

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

Simultaneous breaking of time reversal and inversion symmetries in multiferroics couples ferroelectricity to magnetism and is a source of unusual physical phenomena that can be used in next-generation electronic devices. A notable example…

Strongly Correlated Electrons · Physics 2025-12-02 S. E. Nikitin , N. D. Andriushin , Ø. S. Fjellvåg , E. Pomjakushina , A. A. Turrini , S. Artyukhin , C. W. Schneider , M. Mostovoy

Multiferroic TbMnO3 is investigated using x-ray diffraction in high magnetic fields. Measurements on first and second harmonic structural reflections due to modulations induced by the Mn and Tb magnetic order are presented as function of…

Strongly Correlated Electrons · Physics 2008-07-29 J. Strempfer , B. Bohnenbuck , I. Zegkinoglou , N. Aliouane , S. Landsgesell , M. v. Zimmermann , D. N. Argyriou

Orthorhombic HoMnO3 is a multiferroic in which Mn antiferromagnetic order induces ferroelectricity. A second transition occurs within the multiferroic phase, in which a strong enhancement of the ferroelectric polarization occurs…

Strongly Correlated Electrons · Physics 2021-01-04 Y. W. Windsor , M. Ramakrishnan , L. Rettig , A. Alberca , T. Lippert , C. W. Schneider , U. Staub

Multiferroic rare earth manganites attracted recent attention because of the coexistence of different types of magnetic and ferroelectric orders resulting in complex phase diagrams and a wealth of physical phenomena. The coupling and mutual…

Strongly Correlated Electrons · Physics 2007-05-23 B. Lorenz , C. R. dela Cruz , F. Yen , Y. Q. Wang , Y. Y. Sun , C. W. Chu

Multiferroics, showing simultaneous ordering of electrical and magnetic degrees of freedom, are remarkable materials as seen from both the academic and technological points of view. A prominent mechanism of multiferroicity is the…

Strongly Correlated Electrons · Physics 2012-08-31 P. Lunkenheimer , J. Müller , S. Krohns , F. Schrettle , A. Loidl , B. Hartmann , R. Rommel , M. de Souza , C. Hotta , J. A. Schlueter , M. Lang

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

Materials Science · Physics 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

Ferroelectric and ferromagnetic materials possess spontaneous electric and magnetic order, respectively, which can be switched by the corresponding applied electric and magnetic fields. Multiferroics combine these properties in a single…

Strongly Correlated Electrons · Physics 2012-11-27 J. Lee , S. A. Trugman , C. D. Batista , C. L. Zhang , D. Talbayev , X. S. Xu , S. --W. Cheong , D. A. Yarotski , A. J. Taylor , R. P. Prasankumar

Multiferroics, where two or more ferroic order parameters coexist, is one of the hottest fields in condensed matter physics and materials science[1-9]. However, the coexistence of magnetism and conventional ferroelectricity is physically…

Materials Science · Physics 2016-03-11 Xiangang Wan , Hang-Chen Ding , Sergey Y. Savrasov , Chun-Gang Duan

Within the broad class of multiferroics (compounds showing a coexistence of magnetism and ferroelectricity), we focus on the subclass of "improper electronic ferroelectrics", i.e. correlated materials where electronic degrees of freedom…

Materials Science · Physics 2012-07-26 Silvia Picozzi , Alessandro Stroppa

An effective model is developed to explain the phase diagram and the mechanism of magnetoelectric coupling in multiferroics, $RMn_2O_5$. We show that the nature of magnetoelectric coupling in $RMn_2O_5$ is a coupling between two Ising-type…

Strongly Correlated Electrons · Physics 2009-11-13 Chen Fang , Jiangping Hu

The ground state structural, electronic and magnetic properties of multiferroic TbMn$_2$O$_5$ are investigated via first-principles calculations. We show that the ferroelectricity in TbMn$_2$O$_5$ is driven by the non-centrosymmetric…

Materials Science · Physics 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

Neutron diffraction, magnetic susceptibility, specific heat, and dielectric constant measurements of single crystal Co3TeO6 have been measured to study the interplay between the ferroelectricity and magnetic order. Long range incommensurate…

It is still under intensive discussion, how magnetoelectric coupling actually occurs at the atomic scale in multiferroic BiFeO3. Nuclear solid-state techniques monitor local fields at the atomic scale. Using such an approach, we show that,…

Single-crystal synchrotron x-ray diffraction measurements in strong magnetic fields have been performed for magnetoelectric compounds GdMnO3 and TbMnO3. It has been found that the P || a ferroelectric phase induced by the application of a…

Strongly Correlated Electrons · Physics 2007-05-23 T. Arima , T. Goto , Y. Yamasaki , S. Miyasaka , K. Ishii , M. Tsubota , T. Inami , Y. Murakami , Y. Tokura

We investigate the crystal structure in multiferroic tetragonal perovskite Sr$_{1/2}$Ba$_{1/2}$MnO$_3$ with high accuracy of the order of 10$^{-3}$ Angstrom for an atomic displacement. The large atomic displacement for Mn ion from the…

Materials Science · Physics 2020-07-15 D. Okuyama , K. Yamauchi , H. Sakai , Y. Taguchi , Y. Tokura , K. Sugimoto , T. J. Sato , T. Oguchi

We present a unique example of giant magnetoelectric effect in a conventional multiferroic HoMnO3, where polarization is very large (~56 mC/m2) and the ferroelectric transition temperature is higher than the magnetic ordering temperature by…

Strongly Correlated Electrons · Physics 2015-05-13 N. Hur , I. K. Jeong , M. F. Hundley , S. B. Kim , S. -W. Cheong
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