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We present the results of experiments demonstrating the spectroscopic detection of F\"{o}rster resonance energy transfer from NH$_3$ in the $X\,^1A_1$ ground electronic state to helium atoms in 1s$n$s\,$^3$S$_1$ Rydberg levels, where $n=37$…

Chemical Physics · Physics 2018-01-08 V. Zhelyazkova , S. D. Hogan

In excited molecules, the interaction between the covalent Rydberg and ion-pair channels forms a unique class of excited Rydberg states, in which the infinite manifold of vibrational levels are the equivalent of atomic Rydberg states with a…

Atomic Physics · Physics 2016-06-22 Samuel Markson , Hossein Sadeghpour

A highly excited Rydberg atom via electromagnetically induced transparency with two color cascading lasers has extreme sensitivity to electric fields of microwave ranging from 100 MHz to over 1 THz. It can be used as susceptible atom-based…

Atomic Physics · Physics 2021-11-15 M. H. Cai , Z. S. Xu , S. H. You , H. P. Liu

We propose a promising hybrid quantum system, where a highly-excited atom strongly interacts with a superconducting LC oscillator via the electric field of capacitor. An external electrostatic field is applied to tune the energy spectrum of…

Rydberg Matter (RM) theory is previously shown to give good agreement with the unidentified infrared bands (UIR, UIB) that are observed in emission from many objects in space. From stimulated emission studies in RM, a slightly simpler…

Astrophysics · Physics 2007-10-18 Leif Holmlid

Rydberg atoms are ideal tools for quantum technologies. Due to their large size, their dipole-dipole interaction at micrometer-scale distances and their coupling to external fields are huge. Recent experiments vividly exhibit their interest…

Resonant mm-wave fields drive $n_0f(2) \rightarrow (n_0 \pm 1)g(2)$ transitions in a state-selected $n_0f(2)$ Rydberg gas of NO. This transformation produces a clear signature in the selected field ionization spectrum and dramatically…

Plasma Physics · Physics 2019-08-22 Fernanda Banic Viana Martins , James S. Keller , Edward R. Grant

High-sensitive measurement of radio-frequency (RF) electric field is available via the electromagnetically induced transparency (EIT) effect of Rydberg atom at room-temperature, which has been developed to be a promising atomic RF receiver.…

Atomic Physics · Physics 2019-03-27 Zhenfei Song , Wanfeng Zhang , Hongping Liu , Xiaochi Liu , Haiyang Zou , Jie Zhang , Jifeng Qu

Rydberg-atom electric field sensing has shown great potential from near-DC to THz with state-of-the-art measurement metrics realized in sensitivity, phase extraction, multi-band receptivity, etc. While Rydberg-atom sensors have shown…

Quantum Physics · Physics 2026-03-17 Aveek Chandra , Narongrit Paensin , Rainer Dumke

We propose a new kind of qubits composed of electric dipolar molecules. The electric dipolar molecules in an external uniform electric field will take simple harmonic oscillations, whose quantum states belonging to the two lowest energy…

Quantum Physics · Physics 2024-02-13 Yong-Yi Huang

Using a shared microwave resonator, we propose a transduction scheme between superconducting qubits and qubit states encoded in the low-lying internal levels of trapped atomic systems. The approach employs atomic Rydberg levels together…

Quantum Physics · Physics 2025-09-18 Fernando L. Semião , Matthias Keller

Recognition of multifrequency microwave (MW) electric fields is challenging because of the complex interference of multifrequency fields in practical applications. Rydberg atom-based measurements for multifrequency MW electric fields is…

Quantum Physics · Physics 2022-04-18 Zong-Kai Liu , Li-Hua Zhang , Bang Liu , Zheng-Yuan Zhang , Guang-Can Guo , Dong-Sheng Ding , Bao-Sen Shi

It has been argued that precise measurements of optical transition frequencies between Rydberg states of hydrogen-like ions could be used to obtain an improved value of the Rydberg constant and even to test Quantum Electrodynamics (QED)…

General Relativity and Quantum Cosmology · Physics 2018-08-01 F. Dahia , E. Maciel , A. S. Lemos

Rydberg atoms with principal quantum number n >> 1 have exaggerated atomic properties including dipole-dipole interactions that scale as n^4 and radiative lifetimes that scale as n^3. It was proposed a decade ago to take advantage of these…

Quantum Physics · Physics 2015-03-13 M. Saffman , T. G. Walker , K. Molmer

Rydberg atom-based electrometry enables traceable electric field measurements with high sensitivity over a large frequency range, from gigahertz to terahertz. Such measurements are particularly useful for the calibration of radio frequency…

Quantum Physics · Physics 2017-04-26 Santosh Kumar , Haoquan Fan , Harald Kübler , Akbar J. Jahangiri , James P. Shaffer

We present the direct measurements of electric-dipole moments for $5P_{3/2}\to nD_{5/2}$ transitions with $20<n<48$ for Rubidium atoms. The measurements were performed in an ultracold sample via observation of the Autler-Townes splitting in…

Quantum Physics · Physics 2015-05-27 M. J. Piotrowicz , C. MacCormick , A. Kowalczyk , S. Bergamini , I. I. Beterov , E. A. Yakshina

Nonequilibrium dynamics are closely related to various fields of research, in which vastly different phases emerge when parameters are changed. However, it is difficult to construct nonequilibrium systems that have sufficiently tunable…

We present measurements of hyperfine structure (HFS) of the $nP_J$ Rydberg states for large principal quantum number $n$ range ($n=41-55$) employing the microwave spectroscopy in an ultra-cold cesium Rydberg ensemble. A microwave field with…

Atomic Physics · Physics 2024-10-15 Rong Song , Jingxu Bai , Zhenhua Li , Yuechun Jiao , Suotang Jia , Jianming Zhao

Assemblies of interacting Rydberg atoms show promise for the quantum simulation of transport phenomena, quantum chemistry and condensed matter systems. Such schemes are typically limited by the finite lifetime of Rydberg states. Circular…

Atomic Physics · Physics 2018-10-30 M. M. Aliyu , A. Ulugöl , G. Abumwis , S. Wüster

We present a method to precisly measure the frequencies of transitions to high-$n$ Rydberg states of the hydrogen atom which are not subject to uncontrolled systematic shifts caused by stray electric fields. The method consists in recording…

Atomic Physics · Physics 2024-01-09 Simon Scheidegger , Josef A. Agner , Hansjürg Schmutz , Frédéric Merkt