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We propose a simple approach to measure the energy of the few-eV isomeric state in Th-229. To this end, U-229 nuclei are doped into VUV-transparent crystals, where they undergo alpha decay into Th-229, and, with a probability of 2%,…

Nuclear Experiment · Physics 2016-08-11 Simon Stellmer , Matthias Schreitl , Georgy Kazakov , Johannes Sterba , Thorsten Schumm

With direct polarizability measurements we demonstrated extremely low sensitivity of the inner-shell clock transition at $1.14\,\mu$m in Tm atoms to external dc electric fields and black-body radiation (BBR). We measured differential…

Atomic Physics · Physics 2021-07-13 A. Golovisin , E. Fedorova , D. Tregubov , D. Sukachev , K. Khabarova , V. Sorokin , N. Kolachevsky

An active optical clock based on highly charged Nd$^{9+}$ ion is proposed for the first time. The clock can offer ultra-narrow linewidth at the $\upmu$Hz-level which is more than two-order of magnitude below the currently recorded laser…

Atomic Physics · Physics 2021-07-23 Yan-mei Yu , Duo Pan , Shaolong Chen , Hua Guan , Kelin Gao , Jingbiao Chen

Recent developments in frequency metrology and optical clocks have been based on electronic transitions in atoms and singly charged ions as references. These systems have enabled relative frequency uncertainties at a level of a few parts in…

Atomic Physics · Physics 2018-12-06 M. G. Kozlov , M. S. Safronova , J. R. Crespo López-Urrutia , P. O. Schmidt

A new approach to observe the radiative decay of the $^{229}$Th nuclear isomer, and to determine its energy and radiative lifetime, is presented. Situated at a uniquely low excitation energy, this nuclear state might be a key ingredient for…

A method for highly accurate calculations of atomic electric quadrupole moments (EQM) is presented, using relativistic general-excitation-rank configuration interaction wavefunctions based on Dirac spinors. Application to the clock…

Atomic Physics · Physics 2023-02-06 Timo Fleig

We measure the spectrum of tellurium-130 in the vicinity of the 461~nm ${}^1\text{S}_0-{}^{1}\text{P}_1$ cycling transition in neutral strontium, a popular element for atomic clocks, quantum information, and quantum-degenerate gases. The…

Atomic Physics · Physics 2022-05-23 T. G. Akin , Bryan Hemingway , Steven Peil

Optical atomic clocks have already overcome the eighteenth decimal digit of instability and uncertainty demonstrating incredible control over external perturbations of the clock transition frequency. At the same time there is an increasing…

We demonstrate single-atom resolved imaging with a survival probability of $0.99932(8)$ and a fidelity of $0.99991(1)$, enabling us to perform repeated high-fidelity imaging of single atoms in tweezers for thousands of times. We further…

Quantum Gases · Physics 2019-05-02 Jacob P. Covey , Ivaylo S. Madjarov , Alexandre Cooper , Manuel Endres

The low-energy isomeric transition in Thorium-229 offers a unique interface between nuclear and atomic physics, presenting a resource for quantum technologies that is notably resilient to environmental decoherence. While early experiments…

Quantum Physics · Physics 2025-08-15 Jingbo Wang , Haixing Miao , Shiqian Ding , Dong E. Liu

We describe the current status of the Ca optical frequency standards with laser-cooled neutral atoms realized in two different laboratories for the purpose of developing a possible future optical atomic clock. Frequency measurements…

Atomic Physics · Physics 2009-11-10 U. Sterr , C. Degenhardt , H. Stoehr , Ch. Lisdat , H. Schnatz , J. Helmcke , F. Riehle , G. Wilpers , Ch. Oates , L. Hollberg

Recent advances in laser excitation of the low-energy nuclear isomer transition in $^{229}$Th have opened avenues for developing nuclear clocks, a novel quantum technology with exceptional performance and sensitivity to exotic physics. Here…

Atomic Physics · Physics 2025-08-19 U. C. Perera , H. W. T. Morgan , Eric R. Hudson , Andrei Derevianko

We study thorium-doped CaF$_2$ crystals as a possible platform for optical spectroscopy of the Th-229 nuclear isomer transition. We anticipate two major sources of background signal that might cover the nuclear spectroscopy signal:…

Instrumentation and Detectors · Physics 2016-01-05 Simon Stellmer , Matthias Schreitl , Thorsten Schumm

The internal conversion of nuclear transition in the ${}^{235}U$ atom is considered. The low-energy $\gamma-$quanta ($E_{\gamma} \approx$ 76.8 $eV$) are emitted during the $E3-$transition from the excited state ($I = (\frac12)^+$) of the…

Nuclear Theory · Physics 2010-01-20 Alexei M. Frolov

We report the first operation of a Ra$^{+}$ optical clock, a promising high-performance clock candidate. The clock uses a single trapped $^{226}$Ra$^{+}$ ion and operates on the $7s\ ^2S_{1/2}\rightarrow$ $6d\ ^2D_{5/2}$ electric quadrupole…

Atomic Physics · Physics 2022-01-27 C. A. Holliman , M. Fan , A. Contractor , S. M. Brewer , A. M. Jayich

Highly charged ions (HCIs) are insensitive to external perturbations and are attractive for the development of ultrastable clocks. However, only a few HCI candidates are known to provide optical clock transitions. In this Letter, we show…

Atomic Physics · Physics 2025-01-07 Chunhai Lyu , Christoph H. Keitel , Zoltán Harman

We calculate hyperfine structure of $^{229}$Th and its ions (Th~IV, Th~III, Th~II, Th~I) to reveal the dependence of the nuclear clock frequency on the hyperfine interaction (hfi). We calculate first and second-order hfi shifts and…

Atomic Physics · Physics 2023-12-18 V. A. Dzuba , V. V. Flambaum

Singly-ionized ytterbium, with ultra-narrow optical clock transitions at 467 nm and 436 nm, is a convenient system for the realization of optical atomic clocks and tests of present-day variation of fundamental constants. We present the…

We present an assessment of the (6s^{2})1S0 -> (6s7s)3P0 clock transition frequency in 199Hg with an uncertainty reduction of nearly three orders of magnitude and demonstrate an atomic quality factor, Q, of ~10^(14). The 199Hg atoms are…

Atomic Physics · Physics 2014-12-01 J. J. McFerran , L. Yi , S. Mejri , S. Di Manno , W. Zhang , J. Guéna , Y. Le Coq , S. Bize

Optical atomic clocks using highly-charged ions hold an intriguing promise of metrology at the 19th significant figure. Here we study transitions within the $4f^{12}$ ground-state electronic configuration of highly charged ions. We consider…

Atomic Physics · Physics 2015-06-11 V. A. Dzuba , A. Derevianko , V. V. Flambaum