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The sensitivity of molecular fingerprinting is dramatically improved when placing the absorbing sample in a high-finesse optical cavity, thanks to the large increase of the effective path-length. As demonstrated recently, when the…

We have demonstrated a new technique that provides massively parallel comb spectroscopy sensitive specifically to ions through the combination of cavity-enhanced direct frequency comb spectroscopy with velocity modulation spectroscopy.…

Atomic Physics · Physics 2015-05-28 Laura C. Sinclair , Kevin C. Cossel , Tyler Coffey , Jun Ye , Eric A. Cornell

Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…

Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular…

We demonstrate broadband and sensitive cavity ring-down spectroscopy using a near infrared frequency comb and a time-resolved Fourier transform spectrometer. The cavity decays are measured simultaneously and spectrally sorted, leading to…

Optics · Physics 2022-01-28 Romain Dubreoucq , Lucile Rutkowski

High finesse frequency combs (HFC) with large ratio of the frequency spacing to the width of the spectral components have demonstrated remarkable results in many applications such as precision spectroscopy and metrology. We found that low…

Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…

Quantum Physics · Physics 2023-03-30 Alexandre Belsley

We present a new technique using a frequency comb laser and optical cavities for performing ultrafast transient absorption spectroscopy with improved sensitivity. Resonantly enhancing the probe pulses, we demonstrate a sensitivity of…

Optics · Physics 2016-04-05 Melanie A. R. Reber , Yuning Chen , Thomas K. Allison

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

We have recently introduced the Vernier-based Direct Frequency Comb Cavity-Enhanced Spectroscopy technique and we present the corresponding formalism for quantitative broadband spectroscopy. We achieve high sensitivity and broadband…

Optics · Physics 2016-11-23 Lucile Rutkowski , Jérôme Morville

Spectra comprised of hundreds of time-components for absorption path lengths up to 130 km have been recorded around 1050 nm by combining two recent techniques, intracavity laser spectroscopy with vertical external cavity surface emitting…

Optics · Physics 2009-11-13 Nathalie Picqué , Guy Guelachvili , Alexander A. Kachanov

Frequency comb absorption spectroscopy combined with low-noise, fast homodyne measurements provide a toolbox for ultra-sensitive absorption measurements. Integrating these schemes on photonic platforms to bring them closer to practical…

Optics · Physics 2023-03-20 Jake Biele , Sabine Wollmann , Euan Allen

Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…

Over the last two decades, frequency combs have brought breakthroughs in length metrology with traceability to length standards. In particular, frequency-comb-based spectral interferometry is regarded as a promising technology for…

Optics · Physics 2025-01-20 Yoon-Soo Jang , Heulbi Ahn , Sunghoon Eom , Jungjae Park , Jonghan Jin

Measuring the spectral properties of an optical frequency comb is among the most fundamental tasks of precision metrology. In contrast to general single-parameter measurement schemes, we demonstrate here single shot multiparameter…

Quantum Physics · Physics 2020-03-16 Y. Cai , J. Roslund , V. Thiel , C. Fabre , N. Treps

A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in…

We report what we believe to be the lowest phase noise optical-to-microwave frequency division using fiber-based femtosecond optical frequency combs: a residual phase noise of -120dBc/Hz at 1 Hz offset from a 11.55GHz carrier frequency. We…

Optics · Physics 2012-05-22 W. Zhang , Z. Xu , M. Lours , R. Boudot , Y. Kersale , A. N. Luiten , Y. Le Coq , G. Santarelli

Reducing the pulse repetition rate of an optical frequency comb increases the pulse energy for a given average power. This enhances the efficiency of nonlinear frequency conversion and it facilitates extending the accessible wavelength…

Optical frequency combs can potentially provide an efficient light source for multi-terabit-per-second optical superchannels. However, as the bandwidth of these multi-wavelength light sources is increased, it can result in low per-line…

Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…

Optics · Physics 2015-05-18 I. Coddington , W. C. Swann , N. R. Newbury
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