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The combination of photoelectron spectroscopy and ultrafast light sources is on track to set new standards for detailed interrogation of dynamics and reactivity of molecules. A crucial prerequisite for further progress is the ability to not…

We theoretically investigate the effects of laser polarization on photoelectron angular distribution through laser-induced continuum structure. We focus on a polarization geometry where the probe and dressing lasers are both linearly…

Atomic Physics · Physics 2013-03-07 Gabriela Buica , Takashi Nakajima

The effect of an intense external linear polarized radiation field on the angular distributions and polarization states of the photons emitted during the radiative recombination is investigated. It is predicted, on symmetry grounds, and…

Other Condensed Matter · Physics 2009-11-13 Saverio Bivona , Giovanni Bonanno , Riccardo Burlon , Claudio Leone

We present angular distributions of photoelectrons of atomic model systems excited by intense linearly polarized laser pulses in the VUV- and XUV-regime. We solve the multi-dimensional time-dependent Schr\"odinger equation for one particle…

Atomic Physics · Physics 2010-03-16 S. Bauch , M. Bonitz

We describe the results of experiments and simulations performed with the aim of extending photoelectron spectroscopy with intense laser pulses to the case of molecular compounds. Dimer frame photoelectron angular distributions generated by…

Until recently, theoretical and experimental studies of photoelectron angular distributions (PADs) including non-dipole effects in atomic photo\-ionization have been performed mainly for the conventional plane-wave radiation. One can…

Atomic Physics · Physics 2023-08-21 Maksim D. Kiselev , Elena V. Gryzlova , Alexei N. Grum-Grzhimailo

We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show…

Recent experiments [D. Pengel, S. Kerbstadt, L. Englert, T. Bayer, and M. Wollenhaupt, \href{https://journals.aps.org/pra/abstract/10.1103/PhysRevA.96.043426}{{\PRA} {\bf 96} 043426 (2017)}] have measured the photoelectron momentum…

Atomic Physics · Physics 2019-12-18 G. S. J. Armstrong , D. D. A. Clarke , J. Benda , J. Wragg , A. C. Brown , H. W. van der Hart

We show theoretically and demonstrate experimentally that collapsing elliptically-polarized laser beams experience a nonlinear ellipse rotation that is highly sensitive to small fluctuations in the input power. For arbitrarily small…

We consider the process of atomic ionization driven by a laser pulse with varying ellipticity. We study distribution of the momenta of the photoelectrons, ionized by a strong laser field, emitted in the direction perpendicular to the…

Atomic Physics · Physics 2015-06-22 I. A. Ivanov

We present an experimental and theoretical study of core-level ionization of small hetero- and homo-nuclear molecules employing circularly polarized light and address molecular-frame photoelectron angular distributions in the light's…

We present theoretical calculations for polarization and ellipticity of high-order harmonics from aligned N$_2$, CO$_2$, and O$_2$ molecules generated by linearly polarized lasers. Within the rescattering model, the two polarization…

Atomic Physics · Physics 2010-12-13 Anh-Thu Le , R. R. Lucchese , C. D. Lin

We study ionization dynamics of aligned diatomic molecules N$_2$ in strong elliptical laser fields experimentally and theoretically. The alignment dependence of photoelectron momentum distributions (PMDs) of N$_2$ measured in experiments is…

We study tunneling ionization of HeH+ in strong elliptical laser fields numerically and analytically. The calculated photoelectron momentum distribution (PMD) show two different offset angles corresponding to ionization events occurring in…

Atomic Physics · Physics 2025-11-18 Jiayin Che , Sheng Ye , Shiqi Shen , Weiyan Li , Yanjun Chen

Nonlinear Thomson scattering of an electron motion in a combining field constituted by an elliptically polarized laser and a background magnetic field is investigated. The dependence of the electron trajectories, the fundamental frequency,…

Optics · Physics 2022-06-28 Hong Xiao , Cui-Wen Zhang , Hai-Bo Sang , Bai-Song Xie

Using a model methane-like chiral system, we theoretically demonstrate a possibility to access photoelectron circular dichroism (PECD) by a single experiment with two overlapping laser pulses of carrier frequencies $\omega$ and $2\omega$,…

Atomic and Molecular Clusters · Physics 2018-12-20 Philipp V. Demekhin , Anton N. Artemyev , Alexander Kastner , Thomas Baumert

We propose an alternative approach to the description and analysis of photoelectron angular distributions (PADs) resulting from isotropic samples in the case of few-photon absorption via electric fields of arbitrary polarization. As we…

Atomic Physics · Physics 2022-06-28 Andres F. Ordonez , Olga Smirnova

Strong-field ionization of polar molecules contains rich dynamical processes such as tunneling, excitation, and Stark shift. These processes occur on a sub-cycle time scale and are difficult to distinguish in ultrafast measurements. Here,…

Atomic Physics · Physics 2021-12-15 Jia-Yin Che , Chao Chen , Shang Wang , Guo-Guo Xin , Yan-Jun Chen

We provide a theory of the deflection of polar and non-polar rotating molecules by inhomogeneous static electric field. Rainbow-like features in the angular distribution of the scattered molecules are analyzed in detail. Furthermore, we…

Chemical Physics · Physics 2015-05-20 E. Gershnabel , I. Sh. Averbukh

Photoelectron Angular Distributions (PADs) resulting from 800 nm and 1300 nm strong field ionization of impulsively aligned CF$_3$I molecules were analyzed using time-dependent density functional theory (TDDFT). The normalized difference…

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