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The probability that photoionization of the caged atom in an endohedral system is accompanied by excitation of the fullerene shell is shown to be close to unity in broad intervals of the photoelectron energies. The result is obtained by…

Atomic Physics · Physics 2015-06-15 E. G. Drukarev , M. Ya. Amusia

Near-threshold resonances have been studied for Be-like ions with a focus on overlapping resonances among Rydberg series converging to different thresholds. The behavior of the overlapping as a function of Z and the approach to the limit of…

Atomic Physics · Physics 2012-05-25 W. -C. Chu , H. -L. Zhou , A. Hibbert , S. T. Manson

Ta2NiSe5 is considered a promising excitonic insulator (EI) candidate with slight phonon contributions, since it exhibits a tiny orthorhombic-to-monoclinic structural distortion at 328 K without any superlattice structure. Our synchrotron…

Strongly Correlated Electrons · Physics 2018-08-08 Akitoshi Nakano , Takumi Hasegawa , Shinya Tamura , Naoyuki Katayama , Satoshi Tsutsui , Hiroshi Sawa

Inter-Coulombic decay (ICD) resonances in the photoionization of Cl@C60 endofullerene molecule are calculated using a perturbative density functional theory (DFT) method. This is the first ICD study of an open shell atom in a fullerene…

Atomic and Molecular Clusters · Physics 2021-08-11 Ruma De , Esam Ali , Steven T. Manson , Himadri S. Chakraborty

The ionization of liquefied noble gases by radiation is known to be accompanied by fluctuations much larger than predicted by Poisson statistics. We have studied the fluctuations of both scintillation and ionization in liquid xenon and have…

We demonstrate strong interference patterns in the photoionization cross-section of the subvalent subshells of noble gas (NG) endohedral atoms NG@F. This interference is a result of common action of three factors: the effect of neighboring…

Atomic and Molecular Clusters · Physics 2007-10-25 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

We have investigated the electronic structures of newly discovered superconductor FeSe1-x by bulk-sensitive photoemission spectroscopy (PES). The large Fe 3d spectral weight is located in the vicinity of the Fermi level (EF) and it…

Superconductivity · Physics 2010-11-10 A. Yamasaki , S. Imada , K. Takase , T. Muro , Y. Kato , H. Kobori , A. Sugimura , N. Umeyama , H. Sato , Y. Hara , N. Miyakawa , S. I. Ikeda

We study the ground state structure and aspects of photoionization dynamics of the $Na_{20}@C_{240}$ endofullerene. The structure shows effects from the electronic coupling between the nested cluster and the fullerene cage. They include the…

Atomic and Molecular Clusters · Physics 2024-12-20 Rasheed Shaik , Hari R. Varma , Mohamed El-Amine Madjet , Fulu Zheng , Himadri S. Chakraborty

Photoionization cross sections, photoelectron angular-asymmetry parameters and photoionization time delays for $A$@C$_{60}$ endohedral atoms are studied with account for both the individual and combined effects of dipole static polarization…

Atomic Physics · Physics 2018-09-11 V. K. Dolmatov

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

We use femtosecond resonant soft x-ray diffraction to measure the optically stimulated ultrafast changes of charge density wave correlations in underdoped YBa2Cu3O6.6. We find that when coherent interlayer transport is enhanced by optical…

A photofragmentation study of gas-phase indole (C$_8$H$_7$N) upon single-photon ionization at a photon energy of 420 eV is presented. Indole was primarily inner-shell ionized at its nitrogen and carbon $1s$ orbitals. Electrons and ions were…

A hole in a 4d orbital of atomic xenon relaxes through Auger decay after a lifetime of 3 fs. Adding electronegative fluorine ligands to form xenon fluoride molecules, results in withdrawal of valence-electron density from Xe. Thus, within…

Chemical Physics · Physics 2008-02-23 Christian Buth , Robin Santra , Lorenz S. Cederbaum

We investigated CdTe nanocrystal tetrapods of different sizes by resonant inelastic light scattering at room temperature and under cryogenic conditions. We observe a strongly resonant behavior of the phonon scattering with the excitonic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 R. Krahne , G. Chilla , C. Schueller , L. Carbone , S. Kudera , G. Mannarini , L. Manna , D. Heitmannb , R. Cingolani

It is demonstrated that in fullerene C70 which can be considered as a deformed fullerene C60 in some sense there is a withdrawal of an electrodynamical forbiddance of a strong quadrupole light-molecule interaction which is realized in the…

Optics · Physics 2017-12-12 V. P. Chelibanov A. M. Polubotko

Effects of the interchannel coupling on the spin polarization of energetic photoelectrons emitted from atomic Ne valence subshells are examined. Like previously obtained results for cross sections and angular distributions, the…

Atomic Physics · Physics 2021-06-08 Himadri S. Chakraborty , Pranawa C. Deshmukh , Steven T. Manson

We report on experimental and theoretical results for the photoionization of Ag-like xenon ions, Xe$^{7+}$, in the photon energy range 95 to 145~eV. The measurements were carried out at the Advanced Light Source at an energy resolution of…

Coherent resonance is the effect of resonant excitation of nonlinear coherent modes in trapped Bose condensates. This novel effect is shown to be feasible for Bose-condensed trapped gases. Conditions for realizing this effect are derived. A…

Soft Condensed Matter · Physics 2007-05-23 V. I. Yukalov , E. P. Yukalova , V. S. Bagnato

In this Letter, we investigate the time delay of photoelectrons by fullerenes shell in endohedrals. We present general formulas in the frame of the random phase approximation with exchange (RPAE) applied to endohedrals A@CN that consist of…

Atomic and Molecular Clusters · Physics 2020-10-28 M. Ya. Amusia , L. V. Chernysheva

The Fe K X-ray absorption near edge structure (XANES) of BaFe2-xCoxAs2 superconductors was investigated. No appreciable alteration in shape or energy position of this edge was observed with Co substitution. This result provides experimental…

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