Related papers: CO2 laser-driven reactions in pure acetylene flow
Electrons at the surface of a plasma that is irradiated by a laser with intensity in excess of $10^{23}~\mathrm{W}\mathrm{cm}^{-2}$ are accelerated so strongly that they emit bursts of synchrotron radiation. Although the combination of high…
We report, for the first time, quadrupole mass spectrometry of neutral and positive ionic hydrocarbon species measured at the rf biased substrate electrode of an inductively coupled plasma for acetylene rich C2H2:Ar mixtures under various…
In strong laser fields, sub-femtosecond control of chemical reactions with the carrier-envelope phase (CEP) becomes feasible. We have studied the control of reaction dynamics of acetylene and allene in intense few-cycle laser pulses at 750…
It is a long-standing dream of scientists to capture the ultra-fast dynamics of molecular or chemical reactions in real time and to make a molecular movie. With free-electron lasers delivering extreme ultraviolet (XUV) light at…
We report the generation of molecular hydrogen from water by laser irradiation, without any electrodes and photocatalysts. A near infrared pulsed nanosecond laser is used for exposure of colloidal solution of Au nanoparticles suspended in…
We experimentally and theoretically investigated the deprotonation process on nanosecond to microsecond timescale in ethylene and acetylene molecules, following their double ionization by a strong femtosecond laser field. In our experiments…
To exploit the high intensity of laser radiation, we propose to select frequencies at which single-photon absorption is of too low energy and two or more photons are needed to produce states of an atom that can undergo interatomic Coulombic…
We study the ring-opening decomposition of ethylene carbonate in the presence of a single lithium atom and on the surface of lithium metal. Combining accurate electronic structure theory, enhanced sampling, and machine learning, we…
Recently much attention has being attracted to the problem of limitations on the attainable intensity of high power lasers [A.M. Fedotov {\it et al.} Phys. Rev. Lett. \textbf{105}, 080402 (2010)]. The laser energy can be absorbed by…
Complex organic molecules (COMs) have been identified toward high- and low-mass protostars as well as molecular clouds, suggesting that these interstellar species originate from the early stage(s) of starformation. The reaction pathways…
We demonstrate and interpret a technique of laser-induced formation of thin metallic films using alkali atoms on the window of a dense-vapour cell. We show that this intriguing photo-stimulated process originates from the adsorption of Cs…
Nuclear reactions induced by a strong zeptosecond laser pulse are studied theoretically in the quasiadiabatic regime where the photon absorption rate is comparable to the nuclear equilibration rate. We find that multiple photon absorption…
Under pressure, carbon monoxide (CO) transforms into a polymer that can be recovered to ambient conditions. While this transformation can occur without additional stimuli, experimental observations have shown that laser irradiation can…
We suggest a technique based on the transfer of topological charge from applied laser radiation to directional and coherent optical fields generated in ladder-type excited atomic media to identify the major processes responsible for their…
The rapid development of high brilliance X-ray radiation sources is revolutionizing physics, chemistry, and biology research through their novel applications. Another breakthrough is anticipated with the construction of next-generation…
A model for laser light absorption in electron-positron plasmas self-consistently created via QED cascades is described. The laser energy is mainly absorbed due to hard photon emission via nonlinear Compton scattering. The degree of…
We investigate simultaneous multiphoton-multiatom processes in atomic gases exposed to laser fields under specific frequency conditions, where multiple atoms are simultaneously excited through the absorption of one laser photon each. These…
The photo-induced desorption and oxidation of CO on Ru(0001) is simulated using ab initio molecular dynamics with electronic friction that accounts for the non-equilibrated excited electrons and phonons. Different (O,CO) coverages are…
We report on an experimental and theoretical study of the ionization-fragmentation dynamics of argon dimers in intense few-cycle laser pulses with a tagged carrier-envelope phase. We find that a field-driven electron transfer process from…
In this paper we study photon emission in the interaction of the laser beam with an under-dense target and the attached reflecting plasma mirror. Photons are emitted due to the inverse Compton scattering when accelerated electrons interact…