Related papers: Ultrafast ring opening in CHD investigated by simp…
Slow motion movies are not only fascinating to watch, they also allow us to see intricate details of the mechanical dynamics of complex phenomena. If the images in each frame are replaced by terahertz (THz) waves, such movies can monitor…
We report on ultrafast optical experiments in which femtosecond mid-infrared radiation is used to excite the lattice of complex oxide heterostructures. By tuning the excitation energy to a vibrational mode of the substrate, a long-lived…
In this work we investigate the relaxation processes of 2-thiouracil after UV photoexcitation to the S2 state through the use of ultrafast, single-color, pump-probe UV/UV spectroscopy. We place focus on investigating the appearance and…
A time-resolved spectroscopic protocol exploiting terahertz-assisted photoionization is proposed to reconstruct transient density matrix. Population and coherence elements are effectively mapped onto spectrally separated peaks in…
Chirped-pulse Fourier transform microwave (CP-FTMW) spectroscopy is a versatile technique to record broadband gas-phase rotational spectra, enabling detailed investigations of molecular structure, dynamics, and hyperfine interactions. Here,…
A time-of-flight (ToF) imaging system is proposed and its working principle demonstrated. To realize this system, a new device, a free-space optical mixer, is designed and fabricated. A scene is illuminated (flashed) with a megahertz level…
We present the first results obtained at CFHT with the TRIDENT infrared camera, dedicated to the detection of faint companions close to bright nearby stars. Its main feature is the acquisition of three simultaneous images in three…
Modeling the timing performance of light-based radiation detectors accurately is essential for optimizing time-of-flight positron emission tomography (TOF-PET). We present an analytic framework that combines existing models to predict the…
We have used two-photon Fourier transform spectroscopy to investigate the first singlet excited state (S1) of a prototypical polyene molecule 1,5 -- Diphenyl-1,3,5-hexatriene. As the S1 state in the polyenes is a one-photon forbidden…
We report measurements of superradiant optical transition radiation in the 550-800 nm range produced by ultrashort relativistic electron bunches at a dielectric boundary. In the measured optical spectra, we observe photon production with…
Photonic crystals can integrate plasmonic materials such as indium tin oxide (ITO) in their structure. Exploiting ITO plasmonic properties it is possible to tune the photonic band gap of the photonic crystal upon the application of an…
A near-infrared camera in use at the Canada-France-Hawaii Telescope (CFHT) and at the 1.6-m telescope of the Observatoire du Mont-Megantic is described. The camera is based on a Hawaii-1 1024x1024 HgCdTe array detector. Its main feature is…
Nonradiative energy dissipation in electronically excited polyatomic molecules proceeds through conical intersections, loci of degeneracy between electronic states. We observe a marked enhancement of laser-induced double ionization in the…
Phase transitions driven by ultrashort laser pulses have attracted interest both for understanding the fundamental physics of phase transitions and for potential new data storage or device applications. In many cases these transitions…
A setup for extreme-ultraviolet time-resolved photoelectron spectroscopy (XUV-TRPES) of liquids is described based on a gas-dynamic flat jet formed by a microfluidic chip device. In comparison to a cylindrical jet that has a typical…
We demonstrate the implementation of a simple time-of-flight (ToF) mass spectrometer with medium-mass resolution ($m/\Delta m\sim50$) geared towards the demands of atomic, molecular, and chemical physics experiments. By utilizing a novel…
The optical absorption spectra of cyclo[n]carbons (n=10, 14, 18) are investigated in the framework of time-dependent density functional theory. The collective plasmon excitations well develop as the increases of the ring size and the…
We examine the light and color evolution of the T Tauri binary KH 15D through photometry obtained at wavelengths between 0.55 and 8.0 $\mu$m. The data were collected with ANDICAM on the 1.3 m SMARTS telescope at Cerro-Tololo Inter-American…
We report the detection of the polycyclic aromatic hydrocarbon (PAH) 1H-cyclopent[cd]indene (c-C11H8) in TMC-1 with the QUI- JOTE line survey. We detected 22 independent lines corresponding to 88 rotational transitions with quantum numbers…
We use ultrafast x-ray pulses to characterize the lattice response of SrTiO3 when driven by strong terahertz (THz) fields. We observe transient changes in the diffraction intensity with a delayed onset with respect to the driving field.…