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We study the coupling between the structural dynamics and rheological response of charged colloidal monolayers at water/oil interfaces, driven into steady shear by a microdisk rotating at a controlled angular velocity. The flow causes…

Soft Condensed Matter · Physics 2015-09-14 Ivo Buttinoni , Zachary A. Zell , Todd M. Squires , Lucio Isa

Glass transition is accompanied by a rapid growth of the structural relaxation time and a concomitant decrease of configurational entropy. It remains unclear whether the transition has a thermodynamic origin, and whether the dynamic arrest…

Soft Condensed Matter · Physics 2015-10-28 Chengjie Xia , Jindong Li , Yixin Cao , Binquan Kou , Xinaghui Xiao , Kamel Fezzaa , Tiqiao Xiao , Yujie Wang

We analyse the relationship between dynamics and configuration space structure of Ising spin glass systems. The exact knowledge of the structure of the low--energy landscape is used to study the relaxation of the system by random walk in…

Disordered Systems and Neural Networks · Physics 2009-11-07 S. Kobe , J. Krawczyk

Enormous enhancement in the viscosity of a liquid near its glass transition is generally connected to the growing many-body static correlations near the transition, often coined as `amorphous ordering'. Estimating the length scales of such…

Particle tracking is a key to single-particle-level confocal microscopy observation of colloidal suspensions, emulsions, and granular matter. The conventional tracking method has not been able to provide accurate information on the size of…

Soft Condensed Matter · Physics 2013-01-31 Mathieu Leocmach , Hajime Tanaka

Aging in an attraction-driven colloidal glass is studied by computer simulations. The system is equilibrated without attraction and instantaneously ``quenched'', at constant colloid volume fraction, to one of two states beyond the glass…

Soft Condensed Matter · Physics 2015-06-25 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

In soft amorphous materials, shear cessation after large shear deformation leads to structures having residual shear stress. The origin of these states and the distribution of the local shear stresses within the material is not well…

Soft Condensed Matter · Physics 2021-08-31 Vishwas V. Vasisht , Pinaki Chaudhuri , Kirsten Martens

We employ parallel superposition rheology to study the dynamics of an aging colloidal glass in the presence of a mean field stress. Over a range of intermediate stresses, the loss modulus exceeds the storage modulus at short times but…

Soft Condensed Matter · Physics 2010-03-10 Ajay Singh Negi , Chinedum O. Osuji

Contact-based vibrations play a critical role in the dynamics of granular materials. Significant insights into vibrational granular dynamics have been obtained with reduced-dimensional systems containing macroscale particles. We study…

Mesoscale and Nanoscale Physics · Physics 2016-05-18 Morgan Hiraiwa , Maroun Abi Ghanem , Samuel P. Wallen , Amey Khanolkar , Alexei A. Maznev , Nicholas Boechler

New metallic glasses containing La or Ce have been introduced that have dynamic properties bordering on extremes of conventional metallic glasses. This provides opportunity to test trends or correlations established before in molecular and…

Materials Science · Physics 2015-06-15 K. L. Ngai , Z. Wang , X. Q. Gao , H. B. Yu , W. H. Wang

We have measured depolarized light scattering in liquid benzene over the whole accessible temperature range and over four decades in frequency. Between 40 and 180 GHz we find a susceptibility peak due to structural relaxation. This peak…

Soft Condensed Matter · Physics 2011-04-05 Sabine Wiebel , Joachim Wuttke

The transient behaviour of highly concentrated colloidal liquids and dynamically arrested states (glasses) under time-dependent shear is reviewed. This includes both theoretical and experimental studies and comprises the macroscopic…

Soft Condensed Matter · Physics 2013-09-03 K J Mutch , M Laurati , C P Amann , M Fuchs , S U Egelhaaf

Understanding relaxation of supercooled fluids is a major challenge and confining such systems can lead to bewildering behaviour. Here we exploit an optically confined colloidal model system in which we use reduced pressure as a control…

Soft Condensed Matter · Physics 2020-11-10 Ian Williams , Erdal C. Oğuz , Paul Bartlettl , Hartmut Löwen , C. Patrick Royall

The influence of structural constraints on the relaxation dynamics of three polyurea networks with varying degree of crosslinking, has been studied by means of a thorough analysis of broadband dielectric spectroscopy measurements. Two…

Soft Condensed Matter · Physics 2018-10-03 Nerea Sebastián , Christophe Contal , Antoni Sánchez-Ferrer , Marco Pieruccini

For several atomistic models of glass formers, at conditions below their glassy dynamics onset temperatures, ${T_\mathrm{o}}$, we use importance sampling of trajectory space to study the structure, statistics and dynamics of excitations…

Statistical Mechanics · Physics 2014-05-08 Aaron S. Keys , Lester O. Hedges , Juan P. Garrahan , Sharon C. Glotzer , David Chandler

We study numerically the configuration space at low energy of electron glasses. We consider systems with Coulomb interactions, short-range interactions and no interactions. First, we calculate the integrated density of configurations as a…

Strongly Correlated Electrons · Physics 2007-05-23 A. Perez-Garrido , M. Ortuno , A. M. Somoza , A. Diaz-Sanchez

The precise nature of complex structural relaxation as well as an explanation for the precipitous growth of relaxation time in cooling glass-forming liquids are essential to the understanding of vitrification of liquids. The dramatic…

Materials Science · Physics 2017-06-14 Kaikin Wong , Rithin P. Krishnan , Changjiu Chen , Qing Du , Dehong Yu , Zhaoping Lu , Suresh M. Chathoth

Atomistic deformation simulations in the nominally elastic regime are performed for a model binary glass with strain rates as low as $10^{4}$/sec (corresponding to 0.01 shear strain per 1$\mu$sec). A robust elasticity is revealed that…

Soft Condensed Matter · Physics 2020-11-21 P. M. Derlet , R. Maass

When stressed sufficiently, solid materials yield and deform plastically via reorganization of microscopic constituents. Indeed, it is possible to alter the micro-structure of materials by judicious application of stress, an empirical pro-…

Soft Condensed Matter · Physics 2021-08-09 K. L. Galloway , Xiaoguang Ma , Nathan C. Keim , Douglas J. Jerolmack , Arjun G. Yodh , Paulo E. Arratia

The replica theory of glasses predicts that in the infinite dimensional mean field limit there exist two distinct glassy phases of matter: stable glass and marginal glass. We have developed a technique to experimentally probe these phases…

Soft Condensed Matter · Physics 2020-03-05 Andrew P. Hammond , Eric I Corwin
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