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The structural and electronic properties of the clathrate compounds Ba$_{8}$Al$_{x}$Si$_{46-x}$ and Sr$_{8}$Al$_{x}$Si$_{46-x}$ are studied from first principles, considering an Al content $x$ between 6 and 16. Due to the large number of…

Materials Science · Physics 2017-08-29 Maria Troppenz , Santiago Rigamonti , Claudia Draxl

The technological performances of metallic compounds are largely influenced by atomic ordering. Although there is a general consensus that successful theories of metallic systems should account for the quantum nature of the electronic glue,…

Materials Science · Physics 2015-05-13 Ezio Bruno , Francesco Mammano , Beniamino Ginatempo

In the Al-Co-Cu alloy system, both the decagonal quasicrystal with the space group of $P\overline{10}m2$ and its approximant Al$_{13}$Co$_4$ phase with monoclinic $Cm$ symmetry are present around 20 at.% Co-10 at.% Cu. In this study, we…

Materials Science · Physics 2016-10-13 K. Nakayama , A. Mizutani , Y. Koyama

Using density-functional-theory calculations, we have identified new stable configurations for tri-, tetra-, and penta-vacancies in silicon. These new configurations consist of combinations of a ring-hexavacancy with three, two, or one…

Materials Science · Physics 2009-11-10 D. V. Makhov , Laurent J. Lewis

A computational approach to determine the equilibrium structures of nanoclusters in the whole temperature range from 0 K to melting is developed. Our approach relies on Parallel Tempering Molecular Dynamics (PTMD) simulations complemented…

Atomic and Molecular Clusters · Physics 2023-08-16 Manoj Settem , Riccardo Ferrando , Alberto Giacomello

A formalism for the vacancy formation energies in random alloys within the single-site mean-filed approximation, where vacancy-vacancy interaction is neglected, is outlined. It is shown that the alloy configurational entropy can…

Computational Physics · Physics 2016-05-04 Andrei V. Ruban

The structure and transport properties of SiO2-Al2O3 melts containing 13 mol% and 47 mol% Al2O3 are investigated by means of large scale molecular dynamics computer simulations. The interactions between the atoms are modelled by a pair…

Disordered Systems and Neural Networks · Physics 2007-05-23 Patrick Pfleiderer , Juergen Horbach , Kurt Binder

Machine learning is changing how we design and interpret experiments in materials science. In this work, we show how unsupervised learning, combined with ab initio modeling, improves our understanding of structural metastability in…

We have carried out \textit{ab-initio} calculations of local structure of Mn and Ni in Mn$_{2}$Ni$_{1.5}$In$_{0.5}$ alloy with different site occupancies in order to understand the similarities in martensitic and magnetic properties of…

Materials Science · Physics 2017-01-31 D. N. Lobo , K. R. Priolkar , A. Koide , S. Emura

In a recent paper, Zhang et al. [Acta Materialia 152 (2018) 96] studied the in-plane ordering of the long-period stacking ordered (LPSO) structure in Mg-Al-Y alloys. In addition to the well-known L12 type building cluster, they proposed…

Materials Science · Physics 2018-05-21 Xin-Fu Gu , Tadashi Furuhara , Leng Chen , Ping Yang

Segregation engineering has emerged as a promising pathway towards designing thermally stable nanocrystalline alloys with enhanced mechanical properties. However, the compositional and processing space for solute stabilized microstructures…

Materials Science · Physics 2023-08-31 W. Streit Cunningham , Jungho Shin , Tianjiao Lei , Timothy J Rupert , Daniel S. Gianola

We report on the structure and adsorption properties of Pd$_n$ ($n=1-4$) clusters supported on the rutile TiO$_2$ (110) surfaces with the possible presence of a surface oxygen vacancy or a subsurface Ti-interstitial atom. As predicted by…

Materials Science · Physics 2012-04-12 Jin Zhang , Anastassia N. Alexandrova

By applying a genetic algorithm in a cascade approach of increasing accuracy, we calculate the composition and structure of MgMOx clusters at realistic temperatures and oxygen pressures. The stable and metastable systems are identified by…

Layered Li(Ni,Mn,Co,)O$_2$ (NMC) presents an intriguing ternary alloy design space for optimization as a cathode material in Li-ion batteries. Recently, the high cost and resource limitations of Co have added a new design constraint and…

Materials Science · Physics 2020-02-17 Gregory Houchins , Venkatasubramanian Viswanathan

Using an effective genetic algorithm, we uncover the structure of a metastable Al41Sm5 phase that supplements its family sharing similar short-range orders. The phase evolves upon heating an amorphous Al-9.7at.%Sm ribbon, produced by…

Materials Science · Physics 2017-12-29 Z. Ye , F. Meng , F. Zhang , Y. Sun , L. Yang , S. H. Zhou , R. E. Napolitano , M. I. Mendelev , R. T. Ott , M. J. Kramer , C. Z. Wang , K. M. Ho

In order to clarify thermodynamic stability of Mg-based long-period stacking ordered (LPSO) structure, we systematically study energetic preference for alloys on multiple stacking with different composition for random mixing of constituent…

Materials Science · Physics 2015-09-15 Ryohei Tanaka , Koretaka Yuge

Laser-based additive manufacturing offers a promising route for 3D printing of metallic parts. We evidence experimentally a particular columnar solidification microstructure in a Laser Powder-Bed Fusion processed Inconel 718 nickel-based…

Materials Science · Physics 2019-01-23 G. Boussinot , M. Apel , J. Zielinski , U. Hecht , J. H. Schleifenbaum

Near the melting temperature, equilibrium bismuth melt is characterized by structural features that are absent in equilibrium monatomic simple liquids. In the present work, the structure of bismuth melt is studied by X-ray diffraction…

Materials Science · Physics 2023-06-16 B. N. Galimzyanov , A. A. Tsygankov , A. V. Suslov , V. I. Lad'yanov , A. V. Mokshin

Homogeneous nucleation from aluminum (Al) melt was investigated by million-atom molecular dynamics (MD) simulations utilizing the second nearest neighbor modified embedded atom method (MEAM) potentials. The natural spontaneous homogenous…

Materials Science · Physics 2019-05-02 Avik Mahata , Mohsen Asle Zaeem , Michael I. Baskes

We have investigated the crystal and magnetic structure of Mn${}_{2}$PtPd alloy using powder x-ray and neutron diffraction experiments. This compound is believed to belong to the Heusler family having crystal symmetry…

Materials Science · Physics 2020-03-27 Vivek Kumar , Manfred Reehuis , Andreas Hoser , Peter Adler , Claudia Felser