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The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of great debate. We conducted 17-O single crystal NMR…

Strongly Correlated Electrons · Physics 2015-11-09 M. Fu , T. Imai , T. -H. Han , Y. S. Lee

We report measurements of the specific heat and magnetization of single crystal samples of the spin-1/2 kagome compound ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ (herbertsmithite), a promising quantum spin-liquid candidate, in high magnetic fields and…

We report muSR experiments on Mg{x}Cu{4-x}(OH)6Cl2 with x \sim 1, a new material isostructural to Herbertsmithite exhibiting regular kagome planes of spin 1/2 (Cu^{2+}), and therefore a candidate for a spin liquid ground state. We evidence…

Strongly Correlated Electrons · Physics 2014-10-06 E. Kermarrec , P. Mendels , F. Bert , R. H. Colman , A. S. Wills , P. Strobel , P. Bonville , A. Hillier , A. Amato

The field of frustrated magnetism has been enriched significantly by the discovery of various kagome lattice compounds. These materials exhibit a great variety of macroscopic behaviours ranging from magnetic orders to quantum spin liquids.…

Strongly Correlated Electrons · Physics 2015-08-10 Tsezar F. Seman , Cheng-Chien Chen , Rajiv R. P. Singh , Michel van Veenendaal

We present a Raman spectroscopic investigation of the Herbertsmithite ZnCu3(OH)6Cl2, the first realization of a Heisenberg s=1/2 antiferromagnet on a perfect kagome lattice. The magnetic excitation spectrum of this compound is dominated by…

Herbertsmithite, ZnCu3(OH)6Cl2, is the prototype candidate for a spin liquid behavior on a geometrically perfect kagome lattice. Its discovery and the absence of any evidence for spin-freezing down to the lowest probed temperature to-date…

Strongly Correlated Electrons · Physics 2015-05-28 P. Mendels , F. Bert

Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the…

Strongly Correlated Electrons · Physics 2016-12-05 M. R. Norman

Quantum antiferromagnets based on the square-kagome lattice are proving to be a fertile platform for realizing nontrivial phenomena in frustrated magnetism. Recently, several decorated square-kagome compounds of the nabokoite family have…

Strongly Correlated Electrons · Physics 2025-05-19 Matías G. Gonzalez , Yasir Iqbal , Johannes Reuther , Harald O. Jeschke

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

Strongly Correlated Electrons · Physics 2021-06-15 H. Murayama , T. Tominaga , T. Asaba , A. de Oliveira Silva , Y. Sato , H. Suzuki , Y. Ukai , S. Suetsugu , Y. Kasahara , R. Okuma , I. Kimchi , Y. Matsuda

The quantum spin liquid material herbertsmithite is described by an antiferromagnetic Heisenberg model on the kagome lattice with non-negligible Dzyaloshinskii-Moriya interaction~(DMI). A well established phase transition to the $\mathbf…

Strongly Correlated Electrons · Physics 2017-07-04 Laura Messio , Samuel Bieri , Claire Lhuillier , Bernard Bernu

Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel…

Strongly Correlated Electrons · Physics 2017-01-06 A. Zorko , M. Herak , M. Gomilšek , J. van Tol , M. Velázquez , P. Khuntia , F. Bert , P. Mendels

The spin-1/2 kagome lattice antiferromagnet herbertsmithite, ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, is a candidate material for a quantum spin liquid ground state. We show that the magnetic response of this material displays an unusual scaling…

Strongly Correlated Electrons · Physics 2010-04-07 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Qiu , D. G. Nocera , Y. S. Lee

We performed 23Na NMR measurements on a single-domain crystal of the Kitaev material Na3Co2SbO6, with magnetic field applied along the crystalline a axis. A positive Curie-Weiss constant is obtained from the NMR Knight shift, which suggests…

Strongly Correlated Electrons · Physics 2024-02-14 Ze Hu , Yue Chen , Yi Cui , Shuo Li , Cong Li , Xiaoyu Xu , Ying Chen , Xintong Li , Yuchen Gu , Rong Yu , Rui Zhou , Yuan Li , Weiqiang Yu

There is growing evidence from both experiment and numerical studies that low half-odd integer quantum spins on a kagome lattice with predominant antiferromagnetic near neighbor interactions do not order magnetically or break lattice…

Strongly Correlated Electrons · Physics 2009-11-13 S. Ryu , O. I. Motrunich , J. Alicea , Matthew P. A. Fisher

The dc-magnetization of the unique S=1/2 kagome antiferromagnet Herbertsmithite has been measured down to 0.1K. No sign of spin freezing is observed in agreement with former muSR and ac-susceptibility results. The low temperature magnetic…

Strongly Correlated Electrons · Physics 2009-11-13 F. Bert , S. Nakamae , F. Ladieu , D. L'Hôte , P. Bonville , F. Duc , J. -C. Trombe , P. Mendels

The intrinsic magnetic susceptibility and local magnetization of the near-kagome quantum magnet vesignieite, Cu3BaV2O8(OH)2, are presented as measured using 51V NMR. The NMR line shift gives an accurate measurement of the intrinsic…

Strongly Correlated Electrons · Physics 2015-05-28 J. A. Quilliam , F. Bert , R. H. Colman , D. Boldrin , A. S. Wills , P. Mendels

A preponderance of evidence suggests that the ground state of the nearest-neighbor $S = 1/2$ antiferromagnetic Heisenberg model on the kagome lattice is a gapless spin liquid. Many candidate materials for the realization of this model…

Strongly Correlated Electrons · Physics 2018-12-13 Chih-Yuan Lee , B. Normand , Ying-Jer Kao

To capture the high-field magnetization process of herbertsmithite (ZnCu3(OH)6Cl2), Faraday rotation (FR) measurements were carried out on a single crystal in magnetic fields of up to 190 T. The magnetization data evaluated from the FR…

Strongly Correlated Electrons · Physics 2020-09-29 Ryutaro Okuma , Daisuke Nakamura , Shojiro Takeyama

Nearest-neighbor interacting S = 1/2 spins on the ideal Kagom\'{e} lattice are predicted to form a variety of novel quantum entangled states, including quantum spin-liquid (SL) and valence bond solid (VBS) phases. In real materials, the…

Strongly Correlated Electrons · Physics 2019-10-31 N. J. Laurita , A. Ron , J. W. Han , A. Scheie , J. P. Sheckelton , R. W. Smaha , W. He , J. -J. Wen , J. S. Lee , Y. S. Lee , M. R. Norman , D. Hsieh

We present thermodynamic studies of a new spin-1/2 antiferromagnet containing undistorted kagome lattices---barlowite Cu$_{4}$(OH)$_{6}$FBr. Magnetic susceptibility gives $\theta_{CW}$ = $-$136 K, while long-range order does not happen…

Strongly Correlated Electrons · Physics 2014-12-05 Tian-Heng Han , John Singleton , John A. Schlueter
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