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This work describes the development of a third-generation charge optimized many-body (COMB3) potential for Al-C and its application to the investigation of aluminum/graphene nanostructures. In particular, the new COMB3 potential was used to…

Materials Science · Physics 2019-12-04 Difan Zhang , Alexandre F. Fonseca , Tao Liang , Simon R. Phillpot , Susan B. Sinnott

Although many graphene derivatives have sizable band gaps, their electrical or mechanical properties are significantly degraded due to the low degree of {\pi}-conjugation. Besides the {\pi}-{\pi} conjugation, there exists hyperconjugation…

Materials Science · Physics 2019-12-06 Gui-Lin Zhu , Xiao-Juan Ye , Chun-Sheng Liu

In a recent Letter, Fujii et. al. [Phys. Rev. Lett. 125, 016001] predicted a new carbon allotrope, pentadiamond, with remarkable mechanical properties: elastic moduli comparable or larger than diamond, and negative Poisson's ratio $\mu$ =…

Materials Science · Physics 2020-07-21 Santanu Saha , Wolfgang von der Linden , Lilia Boeri

We report pure carbon-based superlattices that exhibit direct band gaps and excellent optical absorption and emission properties at the threshold energy. The structures are nearly identical to that of cubic diamond except that defective…

Materials Science · Physics 2016-03-23 Young Jun Oh , Sunghyun Kim , In-Ho Lee , Jooyoung Lee , K. J. Chang

The adsorption of an alkali-metal submonolayer on graphene occupying every third hexagon of the honeycomb lattice in a commensurate $(\sqrt{3}\times\sqrt{3})R30^\circ$ arrangement induces an energy gap in the spectrum of graphene. To…

Materials Science · Physics 2009-01-27 M. Farjam , H. Rafii-Tabar

Magnetic order emerging in otherwise non-magnetic materials as carbon is a paradigmatic example of a novel type of s-p electron magnetism predicted to be of exceptional high-temperature stability. It has been demonstrated that atomic scale…

We report a room-temperature optical reflectivity study performed on [112]-oriented Cd$_3$As$_2$ single crystals over a broad energy range under external pressure up to 10 GPa. The abrupt drop of the band dispersion parameter…

Materials Science · Physics 2018-05-23 E. Uykur , R. Sankar , D. Schmitz , C. A. Kuntscher

Angle-resolved photoemission and X-ray diffraction experiments show that multilayer epitaxial graphene grown on the SiC(000-1) surface is a new form of carbon that is composed of effectively isolated graphene sheets. The unique rotational…

The cyanides $M$CN, $M$=Cu, Ag, Au, have experimentally a structure with hexagonally packed, infinite -$M$-CN-$M$-CN- chains. Following our earlier study for AuCN, we now predict that all three $M$CN could have an alternative…

Materials Science · Physics 2009-11-13 P. Zaleski-Ejgierd , P. Pyykkö , M. Hakala

Hybrid two-dimensional (2D) materials have attracted increasing interest as platforms for tailoring electronic properties through interfacial design. Very recently, a novel hybrid 2D material termed glaphene, which combines monolayers of 2D…

T-carbon has been proposed as a new carbon allotrope in 2011, which was successfully synthesized in recent experiments. Because of its fluffy structure, several kinds of atoms can be intercalated into T-carbon, making it a versatile…

Superconductivity · Physics 2020-06-04 Jing-Yang You , Bo Gu , Gang Su

Graphene is the first example of truly two-dimensional crystals - it's just one layer of carbon atoms. It turns out to be a gapless semiconductor with unique electronic properties resulting from the fact that charge carriers in graphene…

Mesoscale and Nanoscale Physics · Physics 2011-11-09 M. I. Katsnelson , K. S. Novoselov

The transition between gapped (semiconducting) and gapless (metallic) phases and tunability of bandgap in materials is a very lucrative yet considerably challenging goal for new-age device preparation. For bulk materials and for…

Strongly Correlated Electrons · Physics 2022-02-08 Rudranil Basu , Swastibrata Bhattacharyya

Graphite oxide is an amorphous insulator. Although several models have been suggested, its structure remains controversial. To elucidate this issue, 5 samples were prepared by the Brodie process and the Staudenmaier process. The electronic…

Materials Science · Physics 2011-03-03 D. W. Lee , J. W. Seo

We introduce carbon Kagome nanotubes (CKNTs) -- a new allotrope of carbon formed by rolling up sheets of Kagome graphene, and investigate the properties of this material using first principles calculations. Based on the direction of…

Materials Science · Physics 2023-12-15 Hsuan Ming Yu , Shivam Sharma , Shivang Agarwal , Olivia Liebman , Amartya S. Banerjee

We present a density functional theory study of low density bromination of graphene and graphite, finding significantly different behaviour in these two materials. On graphene we find a new Br2 form where the molecule sits perpendicular to…

Mesoscale and Nanoscale Physics · Physics 2011-03-18 A. Yaya , C. P. Ewels , I. Suarez-Martinez , Ph. Wagner , S. Lefrant , A. Okotrub , L. Bulusheva , P. R. Briddon

Graphene+, a novel carbon monolayer with sp2-sp3 hybridization, is recently reported to exhibit graphene-like Dirac properties and unprecedented out-of-plane half-auxetic behavior [Yu et al, Cell Reports Physical Science, 3 100790 (2022)].…

Materials Science · Physics 2022-10-26 Linfeng Yu , Ailing Chen , Xiaoxia Wang , Huimin Wang , Zhenzhen Qin , Guangzhao Qin

Several 2D carbon-based materials have been computationally designed in the last years due to the success achieved by graphene. Here, we propose a new 2D all-sp$^2$ carbon allotrope, named Irida-Graphene (IG), using a bottom-up approach. IG…

Rhombohedral dense forms of carbon, rh-C2 (or hexagonal h-C6), and boron nitride, rh-BN (or hexagonal h-B3N3), are derived from rhombohedral 3R graphite based on original crystal chemistry scheme backed with full cell geometry optimization…

Materials Science · Physics 2021-09-29 Samir F. Matar , Vladimir L. Solozhenko

Allotropes of carbon, including one-dimensional carbon nanotubes and two-dimensional graphene sheets, continue to draw attention as promising platforms for probing the physics of electrons in lower dimensions. Recent research has shown that…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 Benedetta Flebus , Allan H. MacDonald