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We propose a theory of the dynamics of polymers in dilute solution, in which the popular Zimm and Rouse models are limiting cases of infinitely large and small draining parameter. The equation of motion for the polymer segments beads) is…

Soft Condensed Matter · Physics 2007-05-23 V. Lisy , J. Tothova , A. V. Zatovsky

We consider a single Rouse polymer chain in two dimensions in presence of a transverse shear flow along the $x$ direction and calculate the persistence probability $P_0(t)$ that the $x$ coordinate of a bead in the bulk of the chain does not…

Statistical Mechanics · Physics 2009-11-13 Somnath Bhattacharya , Dibyendu Das , Satya N. Majumdar

We investigate spatial and temporal cross-correlations between streamwise and normal velocity components in three shear flows: a low-dimensional model for vortex-streak interactions, direct numerical simulations for a nearly homogeneous…

Chaotic Dynamics · Physics 2009-11-11 A. Jachens , J. Schumacher , B. Eckhardt , K. Knobloch , H. H. Fernholz

The influence of an external flow on the relaxation dynamics of a single polymer is investigated theoretically and numerically. We show that a pronounced dynamical slowdown occurs in the vicinity of the coil-stretch transition, especially…

Chaotic Dynamics · Physics 2007-05-23 Antonio Celani , Alberto Puliafito , Dario Vincenzi

We briefly review the recent advances in the rheology of entangled polymers and identify emerging research trends and outstanding challenges, especially with respect to branched polymers. Emphasis is placed on the role of well-characterized…

Soft Condensed Matter · Physics 2016-04-12 F. Snijkers , R. Pasquino , P. D. Olmsted , D. Vlassopoulos

We study the two-dimensional (2D) shear flow of amorphous solids within variants of an elastoplastic model, paying particular attention to spatial correlations and time fluctuations of, e.g., local stresses. The model is based on the local…

Soft Condensed Matter · Physics 2014-03-27 Alexandre Nicolas , Kirsten Martens , Lydéric Bocquet , Jean-Louis Barrat

A theoretical model is developed for predicting dynamic polymer depletion effects under the influence of fluid flow. The results are established by combining the two-fluid model and the self-consistent field theory. We consider a uniform…

Soft Condensed Matter · Physics 2012-08-02 Takashi Taniguchi , Yuichiro Arai , Remco Tuinier , Tai-Hsi Fan

By quantitative studies of statistics of polymer stretching in a random flow and of a flow field we demonstrate that the stretching of polymer molecules in a 3D random flow occurs rather sharply via the coil-stretch transition at the value…

Chaotic Dynamics · Physics 2009-11-10 S. Gerashchenko , C. Chevallard , V. Steinberg

We study the conformation and dynamics of a single polymer chain that is pulled by a constant force applied at its one end with the other end free. Such a situation is relevant to the growing technology of manipulating individual…

Soft Condensed Matter · Physics 2015-06-04 Takahiro Sakaue , Takuya Saito , Hirofumi Wada

The file is a Chapter from my review volume "Polymer Physics: Phenomenology of Polymeric Fluid Simulations". The chapter treats literature tests of the Rouse model, which is widely invoked as a description of polymer motion in melts. In…

Soft Condensed Matter · Physics 2024-08-27 George D. J. Phillies

Many physical systems exhibit plastic flow when subjected to slow steady shear. A unified picture of plastic flow is still lacking; however, there is an emerging theoretical understanding of such flows based on irreversible motions of the…

Soft Condensed Matter · Physics 2007-05-23 Michael Dennin

Motivated by the reported peculiar dynamics of a red blood cell in shear flow, we develop an analytical theory for the motion of a nearly--spherical fluid particle enclosed by a visco--elastic incompressible interface in linear flows. The…

Fluid Dynamics · Physics 2010-07-06 Petia M. Vlahovska , Yuan-nan Young , Gerrit Danker , Chaouqi Misbah

We investigate conformations and dynamics of a polymer considering its monomers to be active Brownian particles. This active polymer shows very intriguing physical behavior which is absent in an active Rouse chain. The chain initially…

Soft Condensed Matter · Physics 2020-04-13 Shalabh K. Anand , Sunil P. Singh

We investigate turbulence in dilute polymer solutions when polymers are strongly stretched by the flow. We establish power-law spectrum of velocity, which is not associated with a flux of a conserved quantity, in two cases. The first case…

Chaotic Dynamics · Physics 2009-11-07 A. Fouxon , V. Lebedev

We experimentally investigate the flow of a viscoelastic fluid in a parallel shear geometry at low Reynolds number. As the flow becomes unstable via a nonlinear subcritical instability, velocimetry measurements show non-periodic…

Fluid Dynamics · Physics 2017-07-26 Boyang Qin , Paulo E. Arratia

The slip phenomena in thin polymer films confined by either flat or periodically corrugated surfaces are investigated by molecular dynamics and continuum simulations. For atomically flat surfaces and weak wall-fluid interactions, the shear…

Soft Condensed Matter · Physics 2008-10-15 Anoosheh Niavarani , Nikolai V. Priezjev

The purpose of this paper is to investigate several analytical methods of solving first passage (FP) problem for the Rouse model, a simplest model of a polymer chain. We show that this problem has to be treated as a multi-dimensional…

Soft Condensed Matter · Physics 2015-12-09 Jing Cao , Jian Zhu , Zuowei Wang , Alexei E. Likhtman

Bead spring models for polymers in solution are nonlinear if either the finite extensibility of the polymer, excluded volume effects or hydrodynamic interactions between polymer segments are taken into account. For such models we use a…

Soft Condensed Matter · Physics 2009-11-07 Roland Rzehak , Walter Zimmermann

We report results of molecular-dynamics simulations for a glassy polymer melt consisting of short, linear bead-spring chains. It was shown in previous work that this onset of the glassy slowing down is compatible with the predictions of the…

Soft Condensed Matter · Physics 2009-10-31 C. Bennemann , J. Baschnagel , W. Paul , K. Binder

The interaction of polymers with small-scale velocity gradients can trigger a coil-stretch transition in the polymers. We analyze this transition within a direct numerical simulation of shear turbulence with an Oldroyd-B model for the…

Chaotic Dynamics · Physics 2009-11-07 Bruno Eckhardt , Jochen Kronjaeger , Joerg Schumacher