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Graphene is an ideal material for hot-electron bolometers, due to its low heat capacity and weak electron-phonon coupling. Nanostructuring graphene with quantum dot constrictions yields detectors with extraordinarily high intrinsic…

The GW plus Bethe-Salpeter equation (GW-BSE) formalism is a well-established approach for calculating excitation energies and optical spectra of molecules, nanostructures, and crystalline materials. We implement GW-BSE in the CP2K code and…

Computational Physics · Physics 2026-05-29 Maximilian Graml , Jan Wilhelm

Energy states below the bandgap of a semiconductor, such as trap states or charge transfer states in organic donor acceptor blends, can contribute to light absorption. Due to their low number density or ultrasmall absorption cross-section,…

Applied Physics · Physics 2019-11-27 Christina Kaiser , Stefan Zeiske , Paul Meredith , Ardalan Armin

One of the challenges of excitonic materials is the accurate determination of the exciton binding energy and bandgap. The difficulty arises from the overlap of the discrete and continuous excitonic absorption at the band edge. Many…

We calculate, as a function of temperature and conduction band electron density, the optical absorption of a weakly n-doped, idealized semiconductor quantum well. In particular, we focus on the absorption band due to the formation of a…

Strongly Correlated Electrons · Physics 2009-11-07 F. X. Bronold

We present a method for computing optical absorption spectra by means of a Bethe-Salpeter equation approach, which is based on a conserving linear response calculation for electron-hole coherences in the presence of an external…

Materials Science · Physics 2010-12-21 George Pal , Yaroslav Pavlyukh , Wolfgang Hübner , Hans Christian Schneider

We develop the tight-binding model to study electronic and optical properties of graphane. The strong sp3 chemical bondings among the carbon and hydrogen atoms induce a special band structure and thus lead to the rich optical excitations.…

Materials Science · Physics 2016-10-31 M. H. Lee , H. C. Chung , J. M. Lu , C. P. Chang , M. F. Lin

We address the question of the optimal broadband absorption of waves in an open, dissipative system. We develop a general framework for absorption induced by multiple overlapping resonances, based on quasi-normal modes and radiative and…

Optics · Physics 2024-07-30 Stéphane Collin , Maxime Giteau

Here we report the optical and x-ray absorption (XAS) spectra of the wide-band-gap oxide MgO using density functional theory (DFT) and many-body perturbation theory (MBPT). Our comprehensive study of the electronic structure shows that…

Other Condensed Matter · Physics 2021-05-19 Vijaya Begum , Markus E. Gruner , Christian Vorwerk , Claudia Draxl , Rossitza Pentcheva

Biased bilayer graphene (BBG) is a variable band gap semiconductor, with a strongly field-dependent band gap of up to $300 \, \text{meV}$, making it of particular interest for graphene-based nano-electronic and -photonic devices. The…

Mesoscale and Nanoscale Physics · Physics 2022-03-21 Mikkel Ohm Sauer , Thomas Garm Pedersen

The photoluminescence spectrum of a single-layer boron nitride remains elusive, marked by enigmatic satellites that hint at a significant but unidentified exciton-phonon coupling.Here, by employing a first principles approach based on the…

Materials Science · Physics 2024-06-03 Giovanni Marini , Matteo Calandra , Pierluigi Cudazzo

We investigate the role of electron-hole correlations in the absorption of freestanding monolayer and bilayer graphene using optical transmission spectroscopy from 1.5 to 5.5 eV. Line shape analysis demonstrates that the ultraviolet region…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Dong-Hun Chae , Tobias Utikal , Siegfried Weisenburger , Harald Giessen , Klaus. v. Klitzing , Markus Lippitz , Jurgen H. Smet

In the course of investigations of thermal neutron detection based on mixtures of $^{10}$BF$_3$ with other gases, knowledge was required of the photoabsorption cross sections of $^{10}$BF$_3$ for wavelengths between 135 and 205 nm. Large…

We examine the absorption spectrum of electromagnetic radiation from excitons, where an exciton in the $1s$ state absorbs a photon and makes a transition to the $2p$ state. We demonstrate that the absorption spectrum depends strongly on the…

Condensed Matter · Physics 2009-10-31 K. Johnsen , G. M. Kavoulakis

An ab initio approach to the calculation of excitonic effects in the optical absorption spectra of semiconductors and insulators is formulated. It starts from a quasiparticle bandstructure calculation and is based on the relevant…

Condensed Matter · Physics 2016-08-31 Stefan Albrecht , Lucia Reining , Rodolfo Del Sole , Giovanni Onida

The frequency-dependent conductivity is studied for the one-dimensional Hubbard model, using a selection rule, the Bethe ansatz, and symmetries associated with conservation laws. For densities where the system is metallic the absorption…

Strongly Correlated Electrons · Physics 2009-10-31 J. M. P. Carmelo , N. M. R. Peres , P. D. Sacramento

A study is presented of the electronic band structure and optical absorption spectrum of monolayer WSe$_2$ using an all-electron quasiparticle self-consistent $GW$ approach, QS$G\hat W$, in which the screened Coulomb interaction $\hat W$ is…

Materials Science · Physics 2024-02-29 Niloufar Dadkhah , Walter R. L. Lambrecht

The optical response functions and band structures of LiCoO$_2$ are studied at different levels of approximation, from density functional theory (DFT) in the generalized gradient approximation (GGA) to quasiparticle self-consistent QS$GW$…

The electronic properties of graphene are unique and are attracting increased attention to this novel 2-dimensional system. Its photonic properties are not less impressive. For example, this single atomic layer absorbs through direct…

Materials Science · Physics 2009-12-25 Fengnian Xia , Thomas Mueller , Yu-ming Lin , Alberto Valdes-Garcia , Phaedon Avouris

The strength of light-matter interaction is of central importance in photonics and optoelectronics. For many widely studied two-dimensional semiconductors, such as MoS2, the optical absorption due to exciton resonances increases with…

Mesoscale and Nanoscale Physics · Physics 2020-04-16 Guowei Zhang , Shenyang Huang , Fanjie Wang , Qiaoxia Xing , Chaoyu Song , Chong Wang , Yuchen Lei , Mingyuan Huang , Hugen Yan