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Motivated by contradicting reports in the literature, we have investigated the structural stability of tungsten nanoparticles using density functional theory calculations. The comparison of BCC, FCC, A15, disordered, and icosahedral…

Materials Science · Physics 2024-04-08 Laurent Pizzagalli , Sandrine Brochard , Julien Godet , Julien Durinck

Smalley and co-workers discovered that chemisorption reactivities of silicon clusters vary over three orders of magnitude as a function of cluster size. In particular, they found that \Si{33}, \Si{39}, and \Si{45} clusters are least…

chem-ph · Physics 2009-10-22 Mushti V. Ramakrishna , Jun Pan

A silicene-like polymorph of the Si111 7x7 surface is proposed that resolves numerous experimental paradoxes and inconsistencies arising over the past 34 years. An analysis of the three established surface state charge densities from atom…

Materials Science · Physics 2019-05-30 J. E. Demuth

The emergence of CsCl bulk structure in (CsCl)nCs+ cluster ions is investigated using a mixed quantum-mechanical/semiempirical theoretical approach. We find that rhombic dodecahedral fragments (with bulk CsCl symmetry) are more stable than…

Atomic and Molecular Clusters · Physics 2009-11-06 Andres Aguado

The search or design of silicon nanostructures similar to their carbon analogues has attracted great interest recently. In this work, density functional calculations are performed to systematically study a series of finite and infinite…

Mesoscale and Nanoscale Physics · Physics 2011-07-19 Lingju Guo , Xiaohong Zheng , Chunsheng Liu , Wanghuai Zhou , Zhi Zeng

A detailed microstructural investigation was performed to understand structural characteristics of a reaction-bonded B$_4$C/SiC ceramic composite. The state-of-the-art focused ion beam & scanning electron microscopy (FIB/SEM) and…

Materials Science · Physics 2017-06-07 Tianshi Wang , Chaoying Ni , Prashant Karandikar

The electrical and optical properties of flat and planar buckled siligraphene (SiC) monolayer are examined using a first principles approach. Buckling between the Si and the C atoms in SiC structures influences and impacts the properties of…

The four most stable structures of Ni$_N$ clusters with $N$ from 2 to 150 have been determined using a combination of the embedded-atom method in the version of Daw, Baskes and Foiles, the {\it variable metric/quasi-Newton} method, and our…

Atomic and Molecular Clusters · Physics 2016-09-08 V. G. Grigoryan , M. Springborg

The fcc-based structure of Yb2.75C60 is unique among metal-doped fullerene compounds, exhibiting long-range-ordered vacancies, significantly off-centered divalent Yb cations, and distorted, crystallographically inequivalent, orientationally…

Materials Science · Physics 2008-02-03 K. M. Rabe , P. H. Citrin

Silicon carbide (SiC) grains are a major dust component in carbon-rich AGB stars. The formation pathways of these grains are, however, not fully understood.\ We calculate ground states and energetically low-lying structures of (SiC)$_n$,…

Solar and Stellar Astrophysics · Physics 2017-05-18 David Gobrecht , Sergio Cristallo , Luciano Piersanti , Stefan T. Bromley

We report the spontaneous formation of a GaP fullerene cage in ab-initio Molecular Dynamics simulations starting from a bulk fragment. A systematic study of the geometric and electronic properties of neutral and ionized GaP clusters…

Chemical Physics · Physics 2009-11-06 V. Tozzini , F. Buda , A. Fasolino

Using first-principles density functional calculations, we have studied the structural stability of stoichiometric as well as non-stoichiometric CdS nanoclusters at ambient pressure with diameters ranging up to about 2.5 nm. Our study…

Atomic and Molecular Clusters · Physics 2011-06-07 Soumendu Datta , Mukul Kabir , Tanusri Saha-Dasgupta , D. D. Sarma

A crystalline form of LiBC is known which has been predicted to be superconducting, with a Tc comparable to that of MgB_2. In both compounds, superconductivity is enhanced by the presence of two electronic bands, one of which is close to a…

Atomic and Molecular Clusters · Physics 2007-05-23 G. M. Lombardo , A. Grassi , G. Forte , G. G. N. Angilella , R. Pucci , N. H. March

A symmetry analysis of the valence shell in the boron buckyball B80, shows a perfect match with the symmetry of the valence shell in C60 .The cap atoms participate in the bonding by 30 orbitals which transform as the sigma bonds along the…

Materials Science · Physics 2009-11-13 Arnout Ceulemans , Jules Tshishimbi Muya , G. Gopakumar , Minh Tho Nguyen

The possibility of the $^{14}$C cluster being a basic building block of medium mass nuclei is discussed. Although $\alpha$ cluster structures have been widely discussed in the light $N\approx Z$ mass region, the neutron to proton ratio…

Nuclear Theory · Physics 2020-03-18 N. Itagaki , A. V. Afanasjev , D. Ray

Enhancing the fracture toughness of diamond while preserving its hardness is a significant challenge. Traditional toughening strategies have primarily focused on modulating the internal microstructural units of diamonds, including…

The nature of metal silane sigma-bond interaction has been investigated in several key systems by a range of experimental and computational techniques. The structure of [Cp'Mn(CO)2(eta2-HSiHPh2)] 1 has been determined by single crystal…

The silicon-vacancy (SiV) and nitrogen-vacancy (NV) centers in diamond are commonly regarded as prototypical defects for solid-state quantum information processing. Here we show that when silicon and nitrogen are simultaneously introduced…

A class of silicon carbide cage clusters with two carbon atoms inside the silicon cage and with high stabilities are presented. The theoretical formalism used is Hartree-Fock theory followed by second order many body perturbation theory to…

Atomic and Molecular Clusters · Physics 2009-11-10 M. N. Huda , A. K. Ray

Stability and charge states of vacancy in Si$_{29}$ and Si$_{38}$ clusters have been calculated by non-conventional tight-binding method and molecular dynamics. Based on the theoretical calculations, it was shown that the vacancy in pure…

Soft Condensed Matter · Physics 2022-03-29 A. B. Normurodov , A. P. Mukhtarov , F. T. Umarova , M. Yu. Tashmetov , Sh. Makhkamov , N. T. Sulaymonov