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We derive an analytical expression that describes the complete three-dimensional carrier-envelope phase (CEP) distribution of in the focal volume of ultrashort pulsed Gaussian beams focused by spherical mirrors or lenses. The focal CEP map…

Optics · Physics 2018-12-19 M. A. Porras , Zoltán L. Horváth , Balázs Major

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

Recent interest in the role of quantum mechanics in the primary events of photosynthetic energy transfer has led to a convergence of nonlinear optical spectroscopy and quantum optics on the topic of energy-transfer dynamics in…

Quantum Physics · Physics 2014-01-23 Agata M. Branczyk , Daniel B. Turner , Gregory D. Scholes

Interferometers are essential tools to measure and shape optical fields, and are widely used in optical metrology, sensing, laser physics, and quantum mechanics. They superimpose waves with a mutual phase delay, resulting in a change in…

The term two-dimensional coherent spectroscopy (2DCS) usually refers to experimental setups where a coherently generated electric field in a sample is recorded over many runs as a function of two time variables: the delay $\tau$ between two…

Superconductivity · Physics 2025-09-30 Jacopo Fiore , Niccolò Sellati , Mattia Udina , Lara Benfatto

X-ray free-electron lasers (FEL) deliver ultrabright X-ray pulses, but not the sequences of phase-coherent pulses required for time-domain interferometry and control of quantum states. For conventional split-and-delay schemes to produce…

Accelerator Physics · Physics 2022-02-11 S. Reiche , G. Knopp , B. Pedrini , E. Prat , G. Aeppli , S. Gerber

We report on tunnel ionization of Xe by 2-cycle, intense, infrared laser pulses and its dependence on carrier-envelope-phase (CEP). At low values of optical field ($E$), the ionization yield is maximum for cos-like pulses with the…

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

We introduce a wide field hyperspectral microscope using the Fourier-transform approach. The interferometer is based on the Translating-Wedge-Based Identical Pulses eNcoding System (TWINS) [Opt. Lett. 37, 3027 (2012)], a common-path…

Instrumentation and Detectors · Physics 2019-09-26 A. Candeo , B. E. Nogueira de Faria , M. Erreni , G. Valentini , A. Bassi , A. M. de Paula , G. Cerullo , C. Manzoni

Spectro-microscopy is an experimental technique which can be used to observe spatial variations in chemical state and changes in chemical state over time or under experimental conditions. As a result it has broad applications across areas…

Medical Physics · Physics 2026-02-05 Maike Meier , Lorenzo Lazzarino , Boris Shustin , Hussam Al Daas , Paul Quinn

Time-domain sampling of arbitrary electric fields with sub-cycle resolution enables a complete time-frequency analysis of a system's response to electromagnetic illumination. This provides access to dynamic information that is not provided…

Spectroscopic mapping refers to the massive recording of spectra whilst varying an additional degree of freedom, such as: magnetic field, location, temperature, or charge carrier concentration. As this involves two serial tasks,…

Materials Science · Physics 2021-11-15 Berk Zengin , Jens Oppliger , Danyang Liu , Lorena Niggli , Tohru Kurosawa , Fabian Donat Natterer

Two-dimensional (2D) fluorescence-excitation (2D-FLEX) spectroscopy is a recently proposed nonlinear femtosecond technique for the detection of photoinduced dynamics. The method records a time-resolved fluorescence signal in its excitation-…

Chemical Physics · Physics 2024-06-24 Sebastian V. Pios , Maxim F. Gelin , Luis Vasquez , Jürgen Hauer , Lipeng Chen

The phase space structure of certain quantum states reveals structure on a scale that is small compared to the Planck area. Using an analog between the wavefunction of a single photon and the electric field of a classical ultrashort optical…

Optics · Physics 2015-05-14 Dane R. Austin , Tobias Witting , Ian A. Walmsley

We propose and demonstrate an interferometric scheme for measuring the two-dimensional two-point cross-spectral density function in a two-shot manner. Our scheme comprises a Michelson interferometer with a converging lens in one of the arms…

Instrumentation and Detectors · Physics 2018-08-01 Abhinandan Bhattacharjee , Shaurya Aarav , Anand K. Jha

In high-performance solar cells based on polymeric semiconductors, the mechanism of photocarrier generation on $<100$-fs timescales is yet to be unravelled. In particular the dynamics of early-time electronic coupling between excitons on…

We demonstrate and characterize that a carrier-envelope-phase (CEP)-controlled ultrashortchirped field is an efficient and robust mechanism to modify the dissociation dynamics of molecularhydrogen. Different dissociation pathways are…

Atomic Physics · Physics 2019-12-11 S. A. Karakaş , P. Rosenberger , M. F. Ciappina , M. F. Kling , İ. Yavuz

Two-dimensional superconductivity has become a major frontier in condensed matter physics. It holds the key to the mechanism of high-temperature superconductors and offers an exceptional arena to stabilize emergent quantum states enabled by…

Superconductivity · Physics 2026-03-16 Qiang-Jun Cheng , Xu-Cun Ma , Qi-Kun Xue , Can-Li Song

Imaging spectroscopy is intended to be coupled with adaptive optics (AO) on large telescopes, such as EST, in order to produce high spatial and temporal resolution measurements of velocities and magnetic fields upon a 2D FOV. We propose a…

Instrumentation and Methods for Astrophysics · Physics 2023-10-10 Jean-Marie Malherbe , Frédéric Sayède , Pierre Mein

Driving laser wakefield acceleration with extremely short, near single-cycle laser pulses is crucial to the realisation of an electron source that can operate at kHz-repetition rate while relying on modest laser energy. It is also…

Plasma Physics · Physics 2021-04-14 Julius Huijts , Igor Andriyash , Lucas Rovige , Aline Vernier , Jerome Faure