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As the emerging ferroelectric (FE) materials, the ultrathin two-dimensional (2D) sliding ferroelectrics without phase-matching bottleneck, usually exhibit the pronounced second harmonic generation (SHG) responses. Despite the structural…

Materials Science · Physics 2025-12-02 Fengfeng Ye , Qiankun Li , Zhuocheng Lu , Xinfeng Chen , Yang Li , Hua Wang , Lu You , Gaoyang Gou

Ferroelectricity can exist in elemental phases as a result of charge transfers between atoms occupying inequivalent Wyckoff positions. We investigate the emergence of ferroelectricity in two-dimensional elemental materials with buckled…

Polar metals based on binary and ternary compounds have been demonstrated in literature. Here, we propose a design principle for ferroelectric-like elemental polar metals and relate it to real materials. The design principle is that, to be…

Materials Science · Physics 2022-05-17 Hu Zhang , Bei Deng , Wei-Chao Wang , Xing-Qiang Shi

While ferroelectric hafnia ($\mathrm{HfO_2}$) has become a technically important material for microelectronics, the physical origin of its ferroelectricity remains poorly understood. The tetragonal $P4_2/nmc$ phase is commonly assigned as…

Materials Science · Physics 2024-09-17 Heng Yu , Kan-Hao Xue , Nan Feng , Yunzhe Zheng , Yan Cheng , Ben Xu , Xiangshui Miao

Ferroelectricity in crystals is associated with the displacement of ions or rotations of polar units. Here we consider the dipole created by donor doping ($D^+$) and the corresponding bound polaron ($e^-$).A dipole of 6.15 Debye is…

Materials Science · Physics 2022-07-06 Kazuki Morita , Yu Kumagai , Fumiyasu Oba , Aron Walsh

We analyze the equilibrium states of quantum lattice model with local multi-well potentials for Sn$_2$P$_2$S$_6$ ferroelectric crystals using the mean and Gaussian curvatures ($H$, $K$), curvedness ($C$) and shape index ($S$). From the…

Materials Science · Physics 2025-12-29 S. Özüm , T. Akkurt , R. Erdem , N. Güçlü

Using first-principles methods, we predict the energy landscape and ferroelectric states of double perovskites of the form AA$'$BB$'$O$_6$ in which the atoms on both the A and B sites are arranged in rock-salt order. While we are not aware…

Materials Science · Physics 2011-04-25 Anindya Roy , David Vanderbilt

Vertical ferroelectricity where a net dipole moment appears as a result of in-plane ionic displacements has gained enormous attention following its discovery in transition metal dichalcogenides. Based on first-principles calculations, we…

Materials Science · Physics 2021-10-29 Xiaonan Ma , Chang Liu , Wei Ren , Sergey A. Nikolaev

The switching of electric polarization induced by electric fields -a fundamental functionality of ferroelectrics- is closely associated with the motions of the domain walls that separate regions with distinct polarization directions.…

Materials Science · Physics 2014-01-10 F. Kagawa , S. Horiuchi , N. Minami , S. Ishibashi , K. Kobayashi , R. Kumai , Y. Murakami , Y. Tokura

We demonstrate the formation of ferroelectric domain-wall polarons in a minimal two-dimensional lattice model of electrons interacting with rotating dipoles. Along the domain-wall, the rotors polarize in opposite directions, causing the…

Mesoscale and Nanoscale Physics · Physics 2025-03-20 Florian Kluibenschedl , Georgios M. Koutentakis , Ragheed Alhyder , Mikhail Lemeshko

We study a simple microscopic model for thin, ferromagnetic, metallic layers on semi-infinite bulk superconductor. We find that for certain values of the exchange spliting, on the ferromagnetic side, the ground states of such structures…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 M. Krawiec , B. L. Gyorffy , J. F. Annett

We investigate the ferrimagnetism and ferroelectricity of bulk NiFe$_2$O$_4$ with tetragonal $P4_122$ ~symmetry by means of density functional calculations using generalized gradient approximation + Hubbard $U$ approach. Special attention…

Materials Science · Physics 2017-09-20 Un-Gi Jong , Chol-Jun Yu , Yong-Su Park , Chong-Suk Ri

The design of the interfacial bondings at metal-oxide interfaces yields exciting new phenomena and can be a route to sustain, and even promote, ferroelectricity at the nanoscale. We study the impact of these interfaces on the nature of the…

Materials Science · Physics 2014-08-12 A. Cano , A. P. Levanyuk

When two BN layers are stacked in parallel in an AB or BA arrangement, a spontaneous out-of-plane electric polarization arises due to charge transfer in the out-of-plane B-N bonds. The ferroelectric switching from AB to BA (or BA to AB) can…

The possibility that metals may support ferroelectricity is an open issue. Anderson and Blount showed that certain martensitic transitions involve inversion symmetry breaking and the formal existence of a polar axis, so 'metallic…

Materials Science · Physics 2016-04-08 Alessio Filippetti , Vincenzo Fiorentini , Francesco Ricci , Pietro Delugas , Jorge Íñiguez

We carry out X-ray absorption spectroscopy experiment at oxygen K-edge in croconic acid (C5H2O5) crystal as a prototype of ferroelectric organic molecular solid, whose electric polarization is generated by proton transfer. The experimental…

A conceptual problem of the electric-field mediated polarization correlations during a stochastic formation of polarization domain structure in ferroelectrics is addressed by using an exactly solvable stochastic model of polarization…

Materials Science · Physics 2023-10-05 Yuri A. Genenko , Olga Y. Mazur , Leonid I. Stefanovich

A variety of compounds, for example doped paraelectrics and polar metals, exhibit both ferroelectricity and correlated electronic phenomena such as low-density superconductivity and anomalous transport. Characterizing such properties is…

Strongly Correlated Electrons · Physics 2023-07-19 Avraham Klein , Vladyslav Kozii , Jonathan Ruhman , Rafael M. Fernandes

The concept of a polar metal proposes new approach of current-induced polarization control for ferroelectrics. We fabricate SnSe/WTe$_2$ heterostructure to experimentally investigate charge transport between two ferroelectric van der Waals…

Mesoscale and Nanoscale Physics · Physics 2022-12-16 N. N. Orlova , A. V. Timonina , N. N. Kolesnikov , E. V. Deviatov

The central goal of crystal engineering is to develop precise control over material function \emph{via} rational design of structure. A particularly successful realisation of this paradigm is the example of hybrid improper ferroelectricity…

Materials Science · Physics 2017-12-06 Hanna L B Boström , Mark S Senn , Andrew L Goodwin