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Electron transfer to an individual quantum dot promotes the formation of charged excitons with enhanced recombination pathways and reduced lifetimes. Excitons with only one or two extra charges have been observed and exploited for very…

We report correlation and cross-correlation measurements of photons emitted under continuous wave excitation by a single II-VI quantum dot (QD) grown by molecular-beam epitaxy. A standard technique of microphotoluminescence combined with an…

Quantum Physics · Physics 2016-08-16 C. Couteau , S. Moehl , F. Tinjod , J. M. Gérard , K. Kheng , H. Mariette , J. A. Gaj , R. Romestain , J. P. Poizat

Resonant photoluminescence excitation (RPLE) spectra of a neutral InGaAs quantum dot show an unconventional line-shape that depends on the detection polarization. We characterize this phenomenon by performing polarization-dependent RPLE…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Disheng Chen , Gary R. Lander , Glenn S. Solomon , Edward B. Flagg

The structure of the ground state exciton of Cd(Se,Te) quantum dots embedded in ZnTe matrix is studied experimentally using photoluminescence spectroscopy and theoretically using ${\bf k}\cdot{\bf p}$ and configuration interaction methods.…

Mesoscale and Nanoscale Physics · Physics 2022-05-04 Petr Klenovský , Piotr Baranowski , Piotr Wojnar

We present a direct experimental evidence of photo-ionized CdTe quantum dot core having luminescence "off" state at band-edge photo-excitation. We use the autocorrelation of fluorescence fluctuations from dilute colloidal solution of CdTe…

Mesoscale and Nanoscale Physics · Physics 2012-08-17 A. V. R. Murthy , Padmashri Patil , Shouvik Datta , Shivprasad Patil

The optical properties of single InAsP/InP quantum dots are investigated by spectrally-resolved and time-resolved photoluminescence measurements as a function of excitation power. In the short-wavelength region (below 1.45 $\mu$m), the…

Quantum dots (QDs), embedded in supercapacitors (S-C) cells exhibited capacitance amplification that peaked at certain QD concentration. More than 2.5 peak amplification was demonstrated with cyclic voltammetry (C-V) at a scan rate of 0.1…

Chemical Physics · Physics 2025-08-25 H. Grebel

The dephasing mechanisms of p-shell and s-shell excitons in an InAs self-assembled quantum dot ensemble are examined using two-dimensional coherent spectroscopy (2DCS). 2DCS provides a comprehensive picture of how the energy level structure…

Mesoscale and Nanoscale Physics · Physics 2019-08-16 Takeshi Suzuki , Rohan Singh , Galan Moody , Marc Aßmann , Manfred Bayer , Arne Ludwig , Andreas D. Wieck , and Steven T. Cundiff

We study the effect of Coulomb correlation on the emission properties of the ground state exciton in zincblende CdSe/ZnS core-shell and in wurtzite ZnO quantum dots. We validate our theory model by comparing results of computed exciton…

Mesoscale and Nanoscale Physics · Physics 2021-12-13 Petr Klenovský , Jakub Valdhans , Lucie Krejčí , Miroslav Valtr , Petr Klapetek , Olga Fedotova

Optical properties of multilayer semi-conductor nano-emitters are crucially dependent on the relative energy levelsof their different components. For core/shell quantum dots, the relative energy difference between conduction bandedge of…

We analyze time-resolved spontaneous emission from excitons confined in self-assembled $\mathrm{InAs}$ quantum dots placed at various distances to a semiconductor-air interface. The modification of the local density of optical states due to…

Other Condensed Matter · Physics 2010-11-05 Søren Stobbe , Jeppe Johansen , Philip Trøst Kristensen , Jørn M. Hvam , Peter Lodahl

The impact of variable Ti self-doping on the 1T-TiSe2 charge density wave (CDW) is studied by scanning tunneling microscopy. Supported by density functional theory we show that agglomeration of intercalated-Ti atoms acts as preferential…

Giant shell CdSe/CdS quantum dots are bright and flexible emitters, with near-unity quantum yield and suppressed blinking, but their single photon purity is reduced by efficient multiexcitonic emission. We report the observation, at the…

Mesoscale and Nanoscale Physics · Physics 2023-01-31 Sergii Morozov , Stefano Vezzoli , Alina Myslovska , Alessio Di Giacomo , N. Asger Mortensen , Iwan Moreels , Riccardo Sapienza

We introduce a method which enables to directly compare the impact of elastic strain on the optical properties of distinct quantum dots (QDs). Specifically, the QDs are integrated in a cross-section of a semiconductor core wire which is…

We report on stacked multiple quantum dots (QDs) formed inside inverted pyramidal recesses, which allow for the precise positioning of the QDs themselves. Specifically we fabricated double QDs with varying inter-dot distance and ensembles…

Mesoscale and Nanoscale Physics · Physics 2017-09-01 S. T. Moroni , T. H. Chung , G. Juska , A. Gocalinska , E. Pelucchi

We study the excitonic structure of CdSe/ZnSe self assembled quantum dots (SAQD) by magneto-photoluminescence (PL) spectroscopy. Using fixed 200 nm apertures through a metal film, we are able to probe single narrow (200 micro-eV)…

Materials Science · Physics 2007-05-23 K. P. Hewaparakrama , N. Mukolobwiez , L. M. Smith , H. E. Jackson , S. Lee , M. Dobrowolska , J. Furdyna

Intermittent photoluminescence of colloidal core/shell semiconductor nanocrystals of spherical and branched shape was studied under CW-laser excitation. Luminescent multichannel registration system was applied for the fluorescence detection…

Optics · Physics 2011-12-13 A. G. Vitukhnovsky , M. M. Kovalev , V. V. Lidsky , E. M. Khokhlov

The emission cascade of a single quantum dot is a promising source of entangled photons. A prerequisite for this source is the use of a symmetric dot analogous to an atom in a vacuum, but the simultaneous achievement of structural symmetry…

Mesoscale and Nanoscale Physics · Physics 2014-08-29 X. Liu , N. Ha , H. Nakajima , T. Mano , T. Kuroda , B. Urbaszek , H. Kumano , I. Suemune , Y. Sakuma , K. Sakoda

The photoluminescence (PL) spectrum of a two-dimensional electron gas (2DEG) in the fractional quantum Hall regime is studied as a function of the separation $d$ between the electron and valence hole layers. The abrupt change in the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Arkadiusz Wojs , John J. Quinn

Electrons and holes can spontaneously form excitons and condense in a semimetal or semiconductor, as predicted decades ago. This type of Bose condensation can happen at much higher temperatures in comparison with dilute atomic gases.…

Mesoscale and Nanoscale Physics · Physics 2023-02-24 Qiang Gao , Yang-hao Chan , Yuzhe Wang , Haotian Zhang , Jinxu Pu , Shengtao Cui , Yichen Yang , Zhengtai Liu , Dawei Shen , Zhe Sun , Juan Jiang , Tai C. Chiang , Peng Chen