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The finite basis optimized effective potential (OEP) method within density functional theory is examined as an ill-posed problem. It is shown that the generation of nonphysical potentials is a controllable manifestation of the use of…

Materials Science · Physics 2009-11-11 Tim Heaton-Burgess , Felipe A. Bulat , Weitao Yang

The optimized-effective-potential (OEP) method is a special technique to construct local Kohn-Sham potentials from general orbital-dependent energy functionals. In a recent publication [M. Betzinger, C. Friedrich, S. Bl\"ugel, A. G\"orling,…

Materials Science · Physics 2012-06-22 Markus Betzinger , Christoph Friedrich , Andreas Görling , Stefan Blügel

The optimized effective potential (OEP) is the exact Kohn-Sham potential for explicitly orbital-dependent energy functionals, e.g., the exact exchange energy. We give a proof for the OEP equation which does not depend on the chain rule for…

Materials Science · Physics 2009-11-10 Stephan Kümmel , John P. Perdew

For exchange-correlation functionals that depend explicitly on the Kohn-Sham orbitals, the potential $V_{\mathrm{xc}\sigma}(\re)$ must be obtained as the solution of the optimized effective potential (OEP) integral equation. This is very…

Materials Science · Physics 2009-11-07 Stephan Kümmel , John P. Perdew

The optimized effective potential (OEP) approach has so far mainly been used in benchmark studies and for the evaluation of band gaps. In this work, we extend the application of the OEP by determining the analytical ionic forces within the…

Materials Science · Physics 2024-09-13 Damian Contant , Maria Hellgren

The optimized effective potential (OEP) method allows for calculation of the local, effective single particle potential of density functional theory for explicitly orbital-dependent approximations to the exchange-correlation energy…

Materials Science · Physics 2015-06-25 P. Sule , S. Kurth , V. Van Doren

The exchange-only optimized effective potential method is implemented with the use of Slater-type basis functions, seeking for an alternative to the standard methods of solution with some computational advantages. This procedure has been…

Chemical Physics · Physics 2011-12-22 J. J. Fernandez , J. E. Alvarellos , P. Garcia-Gonzalez , M. Filatov

Arguments showing that exchange-only optimized effective potential (xOEP) methods, with finite basis sets, cannot in general yield the Hartree-Fock (HF) ground state energy, but a higher one, are given. While the orbital products of a…

Chemical Physics · Physics 2007-05-23 Andreas Goerling , Andreas Hesselmann , Martin Jones , Mel Levy

The optimized effective potential (OEP) method is a promising technique for calculating the ground state properties of a system within the density functional theory. However, it is not widely used as its computational cost is rather high…

Materials Science · Physics 2016-12-15 Taro Fukazawa , Hisazumi Akai

The accurate prediction of electronic response properties of extended molecular systems has been a challenge for conventional, explicit density functionals. We demonstrate that a self-interaction correction implemented rigorously within…

Materials Science · Physics 2009-11-13 T. Körzdörfer , M. Mundt , S. Kümmel

We present a spectral finite-element formulation of the optimized effective potential (OEP) method for atomic structure calculations in the random phase approximation (RPA). In particular, we develop a finite-element framework that employs…

Computational Physics · Physics 2026-01-28 Shubhang Krishnakant Trivedi , Phanish Suryanarayana

We introduce an orbital-optimized double-hybrid (DH) scheme using the optimized-effective-potential (OEP) method. The orbitals are optimized using a local potential corresponding to the complete exchange-correlation energy expression…

We apply a simple transformation method to construct a set of new exactly solvable potentials (ESP) which gives rise to bound state solution of $D$-dimensional Schr\"odinger equation. The important property of such exactly solvable quantum…

Mathematical Physics · Physics 2014-02-07 Nabaratna Bhagawati

Finite-range numerical atomic orbitals are the basis functions of choice for several first principles methods, due to their flexibility and scalability. Generating and testing such basis sets, however, remains a significant challenge for…

Chemical Physics · Physics 2013-11-12 Fabiano Corsetti , M. -V. Fernández-Serra , José M. Soler , Emilio Artacho

We present new quasi-exactly solvable models with inverse quartic, sextic, octic and decatic power potentials, respectively. We solve these models exactly via the functional Bethe ansatz method. For each case, we give closed-form solutions…

Mathematical Physics · Physics 2013-01-15 Davids Agboola , Yao-Zhong Zhang

In this article we show that the boundary of the Pareto critical set of an unconstrained multiobjective optimization problem (MOP) consists of Pareto critical points of subproblems considering subsets of the objective functions. If the…

Optimization and Control · Mathematics 2020-12-18 Bennet Gebken , Sebastian Peitz , Michael Dellnitz

An energy functional for orbital based $O(N)$ calculations is proposed, which depends on a number of non orthogonal, localized orbitals larger than the number of occupied states in the system, and on a parameter, the electronic chemical…

mtrl-th · Physics 2016-09-07 Jeongnim Kim , Francesco Mauri , Giulia Galli

Many real-world applications require solving families of expensive multi-objective optimization problems~(EMOPs) under varying operational conditions. This can be formulated as parametric expensive multi-objective optimization problems…

Machine Learning · Computer Science 2026-05-11 Tingyang Wei , Jiao Liu , Abhishek Gupta , Chin Chun Ooi , Puay Siew Tan , Yew-Soon Ong

The simplicity and the efficiency of a quasi-analytical method for solving nonlinear ordinary differential equations (ODE), is illustrated on the study of anharmonic oscillators (AO) with a potential $V(x) =\beta x^{2}+x^{2m}$ ($m>0$). The…

Mathematical Physics · Physics 2011-05-03 C. Bervillier

It is well known that every solution of an elliptic equation is analytic if its coefficients are analytic. However, less is known about the ultra-analyticity of such solutions. This work addresses the problem of elliptic equations with…

Analysis of PDEs · Mathematics 2024-09-12 Hongjie Dong , Ming Wang
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