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We present an \emph{ab initio} study of the role of interference effects in the thermal conductance of single-molecule junctions. To be precise, using a first-principles transport method based on density functional theory, we analyze the…

Mesoscale and Nanoscale Physics · Physics 2017-12-27 J. C. Klöckner , J. C. Cuevas , F. Pauly

We present a theory of tunneling and resonant transitions in one-dimensional molecular systems which is based on Green's function theory of electron sub-barrier scattering off the structural units (or functional groups) of a molecular…

Other Condensed Matter · Physics 2007-05-23 I. I. Oleynik , M. A. Kozhushner , V. S. Posvyanskii

This work concerns the theoretical description of the quantum dynamics of molecular junctions with thermal fluctuations and probability losses To this end, we propose a theory for describing non-Hermitian quantum systems embedded in…

Quantum Physics · Physics 2021-02-24 Andrea Grimaldi , Alessandro Sergi , Antonino Messina

In this work, a theoretical study of spin transport in a pseudovalve spin (PSV) heterostructure is conducted. For the semiconductor (SC), the conduction band at the $\Gamma$ point of reciprocal space and spin-orbit coupling (SOC) are…

Materials Science · Physics 2026-03-24 Julián A. Zúñiga , Arles V. Gil Rebaza , Diego F. Coral Coral

Employing the nonequilibrium Green's function method, we develop a fully quantum mechanical model to study the coupled electron-phonon transport in one-dimensional atomic junctions in the presence of a weak electron-phonon interaction. This…

Mesoscale and Nanoscale Physics · Physics 2008-03-04 J. T. Lü , Jian-Sheng Wang

A self-consistent method for calculating electron transport through a molecular device is proposed. It is based on density functional theory electronic structure calculations under periodic boundary conditions and implemented in the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

Here, we employ a numerical approach to investigate the transport and conductance characteristics of a quantum point contact. A quantum point contact is a narrow constriction of a width comparable to the electron wavelength defined in a…

Mesoscale and Nanoscale Physics · Physics 2015-12-08 G. Bilgec Akyüz , A. Siddiki

Atomic quantum point contacts accommodate a small number of conduction channels. Their number N and transmission coefficients {T_n} can be determined by analyzing the subgap structure due to multiple Andreev reflections in the…

Superconductivity · Physics 2009-10-31 E. Scheer , J. C. Cuevas , A. Levy Yeyati , A. Martin-Rodero , P. Joyez , M. H. Devoret , D. Esteve , C. Urbina

The study of electron transport through single molecules is essential to the development of molecular electronics. Indeed, trends in electronic conductance through organic nanowires have emerged with the increasing reliability of electron…

Mesoscale and Nanoscale Physics · Physics 2007-05-24 Jordan R. Quinn , Frank W. Foss , Latha Venkataraman , Mark S. Hybertsen , Ronald Breslow

Thermal conductance of single molecular junctions at room temperature has been measured recently using picowatt-resolution scanning probes. However, fully understanding thermal transport in a much wider temperature range is needed for the…

Mesoscale and Nanoscale Physics · Physics 2022-02-15 Gen Li , Bing-Zhong Hu , Nuo Yang , Jing-Tao Lü

Electron transport through a quantum dot coupled to superconducting leads shows a sharp conductance onset when a quantum dot orbital level crosses the superconducting coherence peak of one lead. We study superconducting single electron…

Mesoscale and Nanoscale Physics · Physics 2019-02-06 D. M. T. van Zanten , H. Courtois , C. B. Winkelmann

We study the variation of electron transmission through Au-S-benzene-S-Au junctions and related systems as a function of the structure of the Au:S contacts. For junctions with semi-infinite flat Au(111) electrodes, the highly coordinated…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 A. Grigoriev , J. Skoeldberg , G. Wendin , Z. Crljen

Recent STM molecular break-junction experiments have revealed multiple series of peaks in the conductance histograms of alkanedithiols. To resolve a current controversy, we present here an in-depth study of charge transport properties of…

Materials Science · Physics 2008-02-19 Chen Li , Ilya Pobelov , Thomas Wandlowski , Alexei Bagrets , Andreas Arnold , Ferdinand Evers

A comprehensive review is presented of single molecule junction conductance measurements across families of molecules measured while breaking a gold point contact in a solution of molecules with amine end groups. A theoretical framework…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Mark S. Hybertsen , Latha Venkataraman , Jennifer E. Klare , Adam C. Whalley , Michael L. Steigerwald , Colin Nuckolls

We study ballistic interfacial thermal transport across atomic junctions. Exact expressions for phonon transmission coefficients are derived for thermal transport in one-junction and two-junction chains, and verified by numerical…

Materials Science · Physics 2011-03-02 Lifa Zhang , Pawel Keblinski , Jian-Sheng Wang , Baowen Li

We consider tunneling transport through a Mn$_{12}$ molecular magnet using spin density functional theory. A tractable methodology for constructing many-body wavefunctions from Kohn-Sham orbitals allows for the determination of…

Mesoscale and Nanoscale Physics · Physics 2010-02-08 L. Michalak , C. M. Canali , M. R. Pederson , M. Paulsson , V. G. Benza

This thesis describes the measurement and analysis of the transmission matrix (TM) for microwave radiation propagating through multichannel random waveguides in the crossover to Anderson localization. Eigenvalues of the transmission matrix…

Disordered Systems and Neural Networks · Physics 2014-02-17 Zhou Shi

We present a theoretical analysis aimed at understanding electrical conduction in molecular tunnel junctions. We focus on discussing the validity of coherent versus incoherent theoretical formulations for single-level tunneling to explain…

Mesoscale and Nanoscale Physics · Physics 2016-06-06 Alvar R. Garrigues , Li Yuan , Lejia Wang , Eduardo R. Mucciolo , Damien Thompson , Enrique del Barco , Christian A. Nijhuis

Coherent electronic transport through individual molecules is crucially sensitive to quantum interference. Using exact diagonalization techniques, we investigate the zero-bias and zero-temperature conductance through $\pi$-conjugated…

Strongly Correlated Electrons · Physics 2015-05-14 Julian Rincon , K. Hallberg , S. Ramasesha

We study the model of a molecular switch comprised of a molecule with a soft vibrational degree of freedom coupled to metallic leads. In the presence of strong electron-ion interaction, different charge states of the molecule correspond to…

Mesoscale and Nanoscale Physics · Physics 2008-12-18 Fabio Pistolesi , Yaroslav M. Blanter , Ivar Martin
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