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Electronic Structure Theory (EST) describes the behavior of electrons in matter and is used to predict material properties. Conventionally, this involves forming a Hamiltonian and solving the Schr\"odinger equation through discrete…

Signal Processing · Electrical Eng. & Systems 2024-04-02 Aakash Yadav , Daniel Hedman , Hongsik Jeong

We carry out highly accurate \emph{ab initio} path integral Monte Carlo (PIMC) simulations to directly estimate the free energy of various warm dense matter systems including the uniform electron gas and hydrogen without any nodal…

Quantum Gases · Physics 2024-07-02 Tobias Dornheim , Zhandos Moldabekov , Sebastian Schwalbe , Jan Vorberger

Mapping methods, including the Meyer-Miller-Stock-Thoss (MMST) mapping and spin-mapping, are commonly utilised to simulate nonadiabatic dynamics by propagating classical mapping variable trajectories. Recent work confirmed the Momentum…

Chemical Physics · Physics 2026-03-13 Lauren E. Cook , James R. Rampton , Timothy J. H. Hele

Path integrals are usually formulated in discrete Euclidean time using the Trotter formula. We propose a new method to study discrete quantum systems, in which we work directly in the Euclidean time continuum. The method is of general…

Condensed Matter · Physics 2014-10-13 B. B. Beard , U. -J. Wiese

The book deals with a stochastic formulation of path integration in real time, by rotating the_space_ variables over exp(i pi/4). Preliminary chapters deal with quantum and classical mechanics, probability theory and stochastic calculus,…

Quantum Physics · Physics 2007-05-23 Alec Maassen van den Brink

A novel method for simulating the statistical mechanics of molecular systems in which both nuclear and electronic degrees of freedom are treated quantum mechanically is presented. The scheme combines a path integral description of the…

Computational Physics · Physics 2009-10-31 Ruben O. Weht , Jorge Kohanoff , Dario A. Estrin , Charusita Chakravarty

A new methodology of simulating nonadiabatic dynamics using frozen-width Gaussian wavepackets within the moving crude adiabatic representation with the on-the-fly evaluation of electronic structure is presented. The main feature of the new…

Chemical Physics · Physics 2018-04-04 Loïc Joubert-Doriol , Artur F. Izmaylov

An exact quantum master equation formalism is constructed for the efficient evaluation of quantum non-Markovian dissipation beyond the weak system-bath interaction regime in the presence of time-dependent external field. A novel truncation…

Quantum Physics · Physics 2009-11-10 Rui-Xue Xu , Ping Cui , Xin-Qi Li , Yan Mo , YiJing Yan

Statistical mechanics of the discrete nonlinear Schr\"odinger equation is studied by means of analytical and numerical techniques. The lower bound of the Hamiltonian permits the construction of standard Gibbsian equilibrium measures for…

Statistical Mechanics · Physics 2009-10-31 K. Ø. Rasmussen , T. Cretegny , P. G. Kevrekidis , N. Grønbech-Jensen

Mean-field molecular dynamics based on path integrals is used to approximate canonical quantum observables for particle systems consisting of nuclei and electrons. A computational bottleneck is the sampling from the Gibbs density of the…

Numerical Analysis · Mathematics 2023-11-30 Xin Huang , Petr Plechac , Mattias Sandberg , Anders Szepessy

Recent investigations show that the statistical mechanics of a finite number of particles in ideal harmonic systems predicts different results for the same physical properties, depending on the ensemble under consideration. Path integral…

Statistical Mechanics · Physics 2009-10-31 L. F. Lemmens , F. Brosens , J. T. Devreese

We apply the restricted-path-integral (RPI) theory of non-minimally disturbing continuous measurements for correct description of frictional Brownian motion. The resulting master equation is automatically of the Lindblad form, so that the…

Quantum Physics · Physics 2009-11-07 Michael B. Mensky , Stig Stenholm

We propose a new method for simulating electron dynamics in open quantum systems out of equilibrium, using a finite atomistic model. The proposed method is motivated by the intuitive and practical nature of the driven Liouville von-Neumann…

Mesoscale and Nanoscale Physics · Physics 2014-09-23 Tamar Zelovich , Leeor Kronik , Oded Hod

We develop an efficient algorithm for a spatially inhomogeneous matrix-valued quantum Boltzmann equation derived from the Hubbard model. The distribution functions are $2 \times 2$ matrix-valued to accommodate the spin degree of freedom,…

Computational Physics · Physics 2015-05-15 Jianfeng Lu , Christian B. Mendl

Non commutative quantum mechanics can be viewed as a quantum system represented in the space of Hilbert-Schmidt operators acting on non commutative configuration space. Taking this as departure point, we formulate a coherent state approach…

High Energy Physics - Theory · Physics 2015-05-13 Sunandan Gangopadhyay , Frederik G Scholtz

Geometric integrators of the Schr\"{o}dinger equation conserve exactly many invariants of the exact solution. Among these integrators, the split-operator algorithm is explicit and easy to implement, but, unfortunately, is restricted to…

Chemical Physics · Physics 2024-09-26 Seonghoon Choi , Jiří Vaníček

We generalize and extend the stochastic path integral formalism and action principle for continuous quantum measurement introduced in [A. Chantasri, J. Dressel and A. N. Jordan, Phys. Rev. A {\bf 88}, 042110 (2013)], where the optimal…

Quantum Physics · Physics 2015-09-23 Areeya Chantasri , Andrew N. Jordan

Direct dynamics methods using Gaussian wavepackets have to rely only on local properties, such as gradients and hessians at the center of the wavepacket, so as to be compatible with the usual quantum chemistry methods. Matrix elements of…

Chemical Physics · Physics 2016-04-26 Alexander Humeniuk , Roland Mitric

In this work, we present a compact analytical approximation for the quantum partition function of systems composed of quantum oscillators. The proposed formula is general and applicable to an arbitrary number of oscillators described by a…

Statistical Mechanics · Physics 2025-07-08 Michel Caffarel

From the key composite quantum system made of a two-level system (qubit) and a harmonic oscillator (photon) with resonant or dispersive interactions, one derives the corresponding quantum Stochastic Master Equations (SME) when either the…

Quantum Physics · Physics 2022-09-12 Pierre Rouchon