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Cavity-free lasing in atmospheric air has stimulated intense research towards fundamental understanding of underlying physical mechanisms. In this Letter, we identify a new mechanism -- third harmonic photon mediated resonant energy…

A cavity-free laser in the sky could lead to revolutionary improvements in optical remote sensing for atmospheric science. Abundant in air, nitrogen molecules are prime candidates as an active medium for such a laser. Nitrogen molecules,…

Singly ionized nitrogen molecules in ambient air pumped by near-infrared femtosecond laser give rise to superradiant emission. Here we demonstrate coherent control of this superradiance by injecting a pair of resonant seeding pulses inside…

We experimentally demonstrate generation of strong narrow-bandwidth emissions with excellent coherent properties at ~391 nm and ~428 nm from molecular ions of nitrogen inside a femtosecond filament in air by an orthogonally polarized…

Filamentation of ultrashort laser pulses in the atmosphere offers unique opportunities for long-range transmission of high-power laser radiation and standoff detection. With the critical power of self-focusing scaling as the laser…

Recently, S. Mitryukovskiy et al. presented experimental evidence showing that backward stimulated radiation at 337 nm can be obtained from plasma filaments in nitrogen gas pumped by circularly polarized 800 nm femtosecond pulses (Opt.…

We report on the lasing in air and pure nitrogen gas pumped by a single 800 nm femtosecond laser pulse. Depending on gas pressure, incident laser power and beam convergence, different lasing lines are observed in the forward direction with…

The need for molecular standoff detection has motivated the development of a remotely pumped, high gain air laser that produces lasing in the backward direction and can sample the air as the beam returns. High gain is achieved in the near…

Optics · Physics 2015-05-20 Arthur Dogariu , James Michael , Marlan O. Scully , Richard B. Miles

We report on experimental realization of impulsive rotational Raman scattering from neutral nitrogen molecules in a femtosecond laser filament using an intense self-induced white-light seeding "air laser" generated during the filamentation…

We experimentally investigate generation of backward 357 nm N2 laser in a gas mixture of N2/Ar using 800-nm femtosecond laser pulses, and examine the involved gain dynamics based on pump-probe measurements. Our findings show that a minimum…

Optics · Physics 2015-04-09 Hongqiang Xie , Guihua Li , Wei chu , Bin Zeng , Jinping Yao , Chenrui Jing , Ziting Li , Ya Cheng

Molecular rotational spectroscopy based on strong-field-ionization-induced nitrogen laser is employed to investigate the time evolution of the rotational wave packet composed by a coherent superposition of quantum rotational states created…

We report, for what we believe to be the first time, on the generation of remote self-seeding laser amplification by using only one 800 nm Ti:Sapphire femtosecond laser pulse. The laser pulse (~ 40 fs) is first used to generate a filament…

We report on an investigation of simultaneous generation of several narrow-bandwidth laser-like coherent emissions from nitrogen molecular ions ( ) produced in intense mid-infrared laser fields. With systematic examinations on the…

Optics · Physics 2017-09-12 Jinping Yao , Wei Chu , Zhaoxiang Liu , Bo Xu , Jinming Chen , Ya Cheng

Gaseous ammonia has previously been demonstrated as a compelling gain medium for a quantum cascade laser pumped molecular laser (QPML), exhibiting good power efficiency but limited tunability. Here we explore the potential of the ammonia…

Repetition-rate-scanned lasers are practical in accordion frequency comb generation that serves as a variable gearbox connecting optical and radio wave domains. Rapid and wide-range scanned repetition rate can benefit versatile purposes,…

Recent studies have demonstrated the possibility of accelerating electrons to MeV energies in ambient air using tightly focused laser configurations. In this article, we explore possible strategies to control and optimize the resulting…

We report on the observation of backward lasing at 391.4 nm of nitrogen ions pumped by linearly polarized intense femtosecond pulses at 800 nm. The strongly enhanced spectral intensity at 391.4 nm, as well as the amplification of an…

We report on strong backward stimulated emission at 337 nm in Nitrogen gas pumped by circularly polarized femtosecond laser pulses at 800 nm. A distinct dependence of the backward UV spectrum on pump laser polarization and intensity is…

We demonstrate that pulsed THz radiation produced in air by a focused ultrashort laser pulse can be steered to large angles or even in the backward direction with respect to the laser propagation axis. The emission angle is adjusted by the…

Enhancement of methane emission measurement techniques is necessary to address the need for greenhouse gas emissions monitoring. Here we introduce a gas analyzer designed for remote sensing of atmospheric methane aboard unmanned aerial…

Instrumentation and Detectors · Physics 2024-11-07 Viacheslav Meshcherinov , Viktor Kazakov , Maxim Spiridonov , Gennady Suvorov , Alexander Rodin
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