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We present a general-purpose parameterization of the atomic cluster expansion (ACE) for magnesium. The ACE shows outstanding transferability over a broad range of atomic environments and captures physical properties of bulk as well as…

Materials Science · Physics 2023-05-08 Eslam Ibrahim , Yury Lysogorskiy , Matous Mrovec , Ralf Drautz

Orthogonal systems in $\mathrm{L}_2(\mathbb{R})$, once implemented in spectral methods, enjoy a number of important advantages if their differentiation matrix is skew-symmetric and highly structured. Such systems, where the differentiation…

Numerical Analysis · Mathematics 2019-11-14 Arieh Iserles , Marcus Webb

The adaptively compressed exchange (ACE) method provides an efficient way for solving Hartree-Fock-like equations in quantum physics, chemistry, and materials science. The key step of the ACE method is to adaptively compress an operator…

Numerical Analysis · Mathematics 2017-11-22 Lin Lin , Michael Lindsey

We propose a simple linear scaling expression in reciprocal space for evaluating the ion--electron potential of crystalline solids. The expression replaces the long-range ion--electron potential with an equivalent localized charge…

Materials Science · Physics 2016-12-21 Xuecheng Shao , Wenhui Mi , Qiang Xu , Yanchao Wang , Yanming Ma

In this paper we describe a new approach to implement the O(N) fast multipole method and $O(N\log N)$ tree method, which uses pseudoparticles to express the potential field. The new method is similar to Anderson's method, which uses the…

Astrophysics · Physics 2009-10-30 Junichiro Makino

We present a combination of the incremental expansion of potential energy surfaces (PESs), known as n-mode expansion, with the incremental evaluation of the electronic energy in a many-body approach. The application of semi-local…

Chemical Physics · Physics 2016-08-15 Carolin König , Ove Christiansen

A three-dimensional (3D) Poisson solver with longitudinal periodic and transverse open boundary conditions can have important applications in beam physics of particle accelerators. In this paper, we present a fast efficient method to solve…

Accelerator Physics · Physics 2017-09-13 Ji Qiang

Treating electron correlation more accurately and efficiently is at the heart of the development of electronic structure methods. In the present work, we explore the use of stochastic approaches to evaluate high-order electron correlation…

Chemical Physics · Physics 2020-01-29 Zhendong Li

The need to understand the structure of hierarchical or high-dimensional data is present in a variety of fields. Hyperbolic spaces have proven to be an important tool for embedding computations and analysis tasks as their non-linear nature…

Human-Computer Interaction · Computer Science 2024-01-26 Martin Skrodzki , Hunter van Geffen , Nicolas F. Chaves-de-Plaza , Thomas Höllt , Elmar Eisemann , Klaus Hildebrandt

Over the last two decades, several fast, robust, and high-order accurate methods have been developed for solving the Poisson equation in complicated geometry using potential theory. In this approach, rather than discretizing the partial…

Numerical Analysis · Mathematics 2024-09-19 Fredrik Fryklund , Leslie Greengard , Shidong Jiang , Samuel Potter

We describe a new, adaptive solver for the two-dimensional Poisson equation in complicated geometries. Using classical potential theory, we represent the solution as the sum of a volume potential and a double layer potential. Rather than…

Numerical Analysis · Mathematics 2022-11-29 Fredrik Fryklund , Leslie Greengard

Large-scale atomistic simulations rely on interatomic potentials providing an efficient representation of atomic energies and forces. Modern machine-learning (ML) potentials provide the most precise representation compared to electronic…

Computational Physics · Physics 2025-04-23 David Immel , Ralf Drautz , Godehard Sutmann

We present a new method to accelerate real time-time dependent density functional theory (rt-TDDFT) calculations with hybrid exchange-correlation functionals. For large basis set, the computational bottleneck for large scale calculations is…

Computational Physics · Physics 2019-07-24 Weile Jia , Lin Lin

We develop several efficient algorithms for the classical \emph{Matrix Scaling} problem, which is used in many diverse areas, from preconditioning linear systems to approximation of the permanent. On an input $n\times n$ matrix $A$, this…

Data Structures and Algorithms · Computer Science 2017-04-10 Zeyuan Allen-Zhu , Yuanzhi Li , Rafael Oliveira , Avi Wigderson

In this paper we consider calculation of two-centre exchange integrals over Slater-type orbitals (STOs). We apply the Neumann expansion of the Coulomb interaction potential and consider calculation of all basic quantities which appear in…

Quantum Physics · Physics 2016-11-04 Michał Lesiuk , Robert Moszynski

A number of problems arise when long-range forces, such as those governed by Bessel functions, are used in particle-particle simulations. If a simple cut-off for the interaction is used, the system may find an equilibrium configuration at…

Computational Physics · Physics 2009-11-06 Hans Fangohr , Andrew R. Price , Simon J. Cox , Peter A. J. de Groot , Geoffrey J. Daniell , Ken S. Thomas

The Atomic Cluster Expansion (ACE) (Drautz, Phys. Rev. B 99, 2019) has been widely applied in high energy physics, quantum mechanics and atomistic modeling to construct many-body interaction models respecting physical symmetries.…

Numerical Analysis · Mathematics 2024-01-08 Cheuk Hin Ho , Timon S. Gutleb , Christoph Ortner

The space nonlocal Allen-Cahn equation is a famous example of fractional reaction-diffusion equations. It is also an extension of the classical Allen-Cahn equation, which is widely used in physics to describe the phenomenon of two-phase…

Numerical Analysis · Mathematics 2025-02-05 Yuxin Zhang , Hengfei Ding

Artificial neural network (ANN) potentials enable the efficient large-scale atomistic modeling of complex materials with near first-principles accuracy. For molecular dynamics simulations, accurate energies and interatomic forces are a…

Computational Physics · Physics 2020-05-05 April M. Cooper , Johannes Kästner , Alexander Urban , Nongnuch Artrith

Matrix exponentiation (ME) is widely used in various fields of science and engineering. For example, the unitary dynamics of quantum systems is described by exponentiation of Hamiltonian operators. However, despite a significant attention,…

Quantum Physics · Physics 2017-07-10 Gaurav Bhole , T. S. Mahesh
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