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In quantum science applications, ranging from many-body physics to quantum metrology, dipolar interactions in spin ensembles are controlled via Floquet engineering. However, this technique typically reduces the interaction strength between…

Nanodiamonds containing nitrogen vacancy (NV-) centers show promise for a number of emerging applications including targeted in vivo imaging and generating nuclear spin hyperpolarization for enhanced NMR spectroscopy and imaging. Here, we…

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

Diamond-based quantum sensors have enabled high-resolution NMR spectroscopy at the microscale in scenarios where fast molecular motion averages out dipolar interactions among target nuclei. However, in samples with low-diffusion, ubiquitous…

Quantum Physics · Physics 2025-08-26 Carlos Munuera-Javaloy , Ander Tobalina , Jorge Casanova

Nitrogen-vacancy (NV) centers in diamond have emerged as valuable tools for sensing and polarizing spins. Motivated by potential applications in chemistry, biology, and medicine, we show that NV-based sensors are capable of detecting single…

Quantum Physics · Physics 2016-03-10 M. Bruderer , P. Fernández-Acebal , R. Aurich , M. B. Plenio

We use tunable dipolar-interactions between the spins of nitrogen-vacancy (NV) centers in diamond to rotate a diamond crystal. Specifically, we employ cross-relaxation between the electronic spin of pairs of NV centers in a trapped diamond…

Mesoscale and Nanoscale Physics · Physics 2021-09-22 C. Pellet-Mary , P. Huillery , M. Perdriat , G. Hétet

The use of the nuclear spins surrounding electron spin qubits as quantum registers and long-lived memories opens the way to new applications in quantum information and biological sensing. Hence, there is a need for generic and robust forms…

Quantum Physics · Physics 2021-07-06 O. T. Whaites , J. Randall , T. H. Taminiau , T. S. Monteiro

The nitrogen-vacancy (NV) centre in diamond has emerged as a candidate to non-invasively hyperpolarise nuclear spins in molecular systems to improve the sensitivity of nuclear magnetic resonance (NMR) experiments. Several promising proof of…

Mesoscale and Nanoscale Physics · Physics 2021-05-26 A. J. Healey , L. T. Hall , G. A. L. White , T. Teraji , M. -A. Sani , F. Separovic , J. -P. Tetienne , L. C. L. Hollenberg

The Nitrogen Vacancy Center in diamond coupled to addressable surrounding nuclear spins forms a versatile building block for future quantum technologies. While previous activities focused on sensing with only a single or very few spins in…

Quantum Physics · Physics 2024-08-20 Dominik Maile , Joachim Ankerhold

Precise characterization of a hyperfine interaction is a prerequisite for high fidelity manipulations of electron and nuclear spins belonging to a hybrid qubit register in diamond. Here, we demonstrate a novel scheme for determining a…

Quantum Physics · Physics 2013-09-11 J. H. Shim , B. Nowak , I. Niemeyer , J. Zhang , F. D. Brandao , D. Suter

Quantum networks will rely on photons entangled to robust, local quantum registers for computation and error correction. We demonstrate control of and entanglement in a fully connected three-qubit $^{13}\mathrm{C}$ nuclear spin register in…

Quantum Physics · Physics 2025-08-08 Marco Klotz , Andreas Tangemann , David Opferkuch , Alexander Kubanek

Solid state spins in diamond, in particular negatively charged nitrogen-vacancy centers (NV), are leading contenders in the field of quantum sensing. While addressing of single NVs offers nanoscale spatial resolution, many implementations…

Quantum Physics · Physics 2023-01-11 Yuchun Zhu , Elena Losero , Christophe Galland , Valentin Goblot

We propose an approach to realize a hybrid quantum system composed of a diamond nitrogen-vacancy (NV) center spin coupled to a magnon mode of the low-damping, low-moment organic ferrimagnet vanadium tetracyanoethylene. We derive an…

Mesoscale and Nanoscale Physics · Physics 2025-04-22 Denis R. Candido , Gregory D. Fuchs , Ezekiel Johnston-Halperin , Michael E. Flatté

We propose a novel architecture for scalable quantum computation based on quantum actuated decoherence-free (DF) qubits. Each qubit is encoded by the DF subspace of a nuclear spin pair and has long coherence time. A nitrogen-vacancy center…

Quantum Physics · Physics 2017-12-06 Xing Rong , Lihong Dong , Jianpei Geng , Fazhan Shi , Zhaokai Li , Changkui Duan , Jiangfeng Du

A negatively charged nitrogen vacancy (NV) center in diamond has been recognized as a good solid-state qubit. A system consisting of the electronic spin of the NV center and hyperfine-coupled nitrogen and additionally nearby carbon nuclear…

Quantum Physics · Physics 2015-05-21 Yi Chou , Shang-Yu Huang , Hsi-Sheng Goan

Theoretical study of the indirect coupling of nuclear spins (qubits) embedded into a mesoscopic ring and in a finite length quantum wire in a magnetic field is presented. It is found that the hyperfine interaction, via the conduction…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Yu. V. Pershin , I. D. Vagner , P. Wyder

We show that electric field noise from surface charge fluctuations can be a significant source of spin decoherence for near-surface nitrogen-vacancy (NV) centers in diamond. This conclusion is based on the increase in spin coherence…

Mesoscale and Nanoscale Physics · Physics 2015-08-26 M. Kim , H. J. Mamin , M. H. Sherwood , K. Ohno , D. D. Awschalom , D. Rugar

The nitrogen-vacancy (NV) centre in diamond is a leading platform for nanoscale sensing and imaging, as well as quantum information processing in the solid state. To date, individual control of two NV electronic spins at the nanoscale has…

Electron and nuclear spins are very promising candidates to serve as quantum bits (qubits) for proposed quantum computers, as the spin degrees of freedom are relatively isolated from their surroundings, and can be coherently manipulated…

Quantum Physics · Physics 2010-08-24 J. van Tol , G. W. Morley , S. Takahashi , D. R. McCamey , C. Boehme , M. E. Zvanut

Hybrid qubit systems combining electronic spins with nearby ("proximate") nuclear spin registers offer a promising avenue towards quantum information processing, with even multi-spin error correction protocols recently demonstrated in…

Quantum Physics · Physics 2015-06-16 R. Guichard , S. J. Balian , G. Wolfowicz , P. A. Mortemousque , T. S. Monteiro