Related papers: Polarization spectroscopy of an excited state tran…
We describe a method to observe the dynamics of an excited-state transition in a room temperature atomic vapor using hyperfine quantum beats. Our experiment using cesium atoms consists of a pulsed excitation of the D2 transition, and…
The $6S_{1/2}-5D_{5/2}$ electric quadrupole transition is investigated in Cesium vapor at room temperature via nonlinear Doppler-free 6P-6S-5D three-level spectroscopy. Frequency-resolved studies of individual E2 hyperfine lines allow one…
We report on a study of modulation transfer spectroscopy of the $4\textrm{S}_{1/2}\rightarrow 4\textrm{P}_{1/2}$ ($D_{1}$) transition of naturally abundant potassium in a room-temperature vapour cell. This transition is critical for laser…
We investigate, theoretically and experimentally, absorption on an excited-state atomic transition in a thermal vapor where the lower state is coherently pumped. We find that the transition linewidth can be sub-natural, i.e. less than the…
We experimentally demonstrate the cesium electric quadrupole transition from the 6S1/2 ground state to the 7D3/2,5/2 excited state through a virtual level by using a single laser at 767 nm. The excited state energy level population is…
We study modulation spectroscopy of the potassium D2 transitions at 766.7 nm. The vapour pressure, controlled by heating a commercial reference cell, is optimized using conventional saturated absorption spectroscopy. Subsequent heterodyne…
We study modulation-free methods for producing sub-Doppler, dispersive line shapes for laser stabilization near the potassium D2 transitions at 767 nm. Polarization spectroscopy is performed and a comparison is made between the use of a…
We report on the demonstration of Doppler-free polarization spectroscopy of the D2 line of 6Li atoms. Counterintuitively, the presence of an Ar buffer gas, in a certain pressure range, causes a drastic enhancement of the polarization…
We characterize the anisotropic differential ac-Stark shift for the Dy $626$ nm intercombination transition, induced in a far-detuned $1070$ nm optical dipole trap, and observe the existence of a "magic polarization" for which the…
Photoionization spectroscopy of cold cesium dimers obtained by photoassociation of cold atoms in a magneto-optical trap is reported here. In particular, we report on the observation and on the spectroscopic analysis of all the excited…
The impact of the optical field polarization on the spectrum of magnetically-induced transitions, a class of transitions forbidden at zero magnetic field, is studied with a weak-probe sub-Doppler technique. The high spectral resolution of…
We have completed a measurement of the Stark shift within the $^{115}$In $6s_{1/2} \rightarrow 6p_{1/2}$ excited-state transition using two-step laser spectroscopy in an indium atomic beam. Combining this measurement with recent…
The relaxation of atomic polarization in buffer-gas-free, paraffin-coated cesium vapor cells is studied using a variation on Franzen's technique of ``relaxation in the dark'' [Franzen, Phys. Rev. {\bf 115}, 850 (1959)]. In the present…
We develop a theoretical treatment of polarization spectroscopy and use it to make predictions about the general form of polarization spectra in the alkali atoms. Using our model, we generate theoretical spectra for the D2 transitions in…
We demonstrate a laser frequency stabilization technique for laser cooling of Potassium atoms, based on saturated absorption spectroscopy in the C-Band optical telecommunication window, using ro-vibrationel transitions of the acetylene…
We report on studies of simultaneous continuous-wave mirrorless lasing on multiple optical transitions, realized by pumping hot cesium vapor with laser light resonant with the 6$S_{1/2}\rightarrow 8$P$_{3/2}$ transition. The multiplicity of…
A novel polarization-modulation transient method has been developed for studying fast anisotropic relaxation in electronic excited states of polyatomic and biologically relevant molecules under excitation with femtosecond laser pulses. The…
We present a combined theoretical and experimental study of magnetic resonance transitions induced by polarization-modulated light in cesium vapor exposed to a transverse magnetic field. Signals are obtained by phase-sensitive analysis of…
Selective Reflection (SR) spectroscopy of the $6s$ $^2S_{1/2} \rightarrow$ $7p$ $^2P_{3/2}$ electric dipole transition of Cesium ($\lambda~=~456$ nm) is performed for the first time using a nanometric-thin cell ($L=50 - 1500$~nm). We…
In this work we perform polarization spectroscopy of erbium atoms in a hollow cathode lamp (HCL) for the stabilization of a diode laser to the 401-nm transition. We review the theory behind Doppler-free polarization spectroscopy,…