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Colloidal quantum dots (QDs) are an attractive medium for nonlinear optics and deterministic heterogeneous integration with photonic devices. Their intrinsic nonlinearities can be strengthened further by coupling QDs to low mode-volume…

Semiconductor superlattice multipliers have emerged as a nonlinear medium capable to generate radiation in a wide frequency range. This property facilitates the potential of sources suitable for sensing and spectroscopy applications. In…

Mesoscale and Nanoscale Physics · Physics 2021-01-06 Yuliia Shevchenko , Apostolos Apostolakis , Mauro F. Pereira

Nanoscale amplification of non-linear processes in solid-state devices opens novel applications in nano-electronics, nano-medicine or high energy conversion for example. Coupling few nano-joules laser energy at a nanometer scale for strong…

Second-harmonic generation in resonant structures is commonly evaluated in terms of intracavity field enhancement at the fundamental and harmonic frequencies. Here, we formulate nonlinear frequency conversion within a symmetry-resolved…

Nonlinear processes are at the core of many optical technologies including lasers, information processing, sensing, and security, and require optimised materials suitable for nanoscale integration. Here we demonstrate the emergence of a…

Optics · Physics 2018-01-03 B. Wells , A. Yu. Bykov , G. Marino , M. E. Nasir , A. V. Zayats , V. A. Podolskiy

We investigate type I second harmonic generation in III-V semiconductor wire waveguides aligned with a crystallographic axis. In this direction, because of the single nonzero tensor element of III-V semiconductors, only frequency conversion…

There is an active demand to develop efficient nanoscale nonlinear sources for applications in photonic circuitry, quantum optics and biosensing. To this end, plasmonic systems have been utilized to boost the nonlinear signal generation,…

Optics · Physics 2019-06-26 Feng Wang , Manoj Manjare , Robert Lemasters , Chentao Li , Hayk Harutyunyan

Harmonic generation mechanisms are of great interest in nanoscience and nanotechnology, since they allow generating visible light by using near-infrared radiation, which is particularly suitable for its endless applications in…

The simplest Lorentz-nonreciprocal medium has the constitutive relations (${\bf D} =\epso {\bf E} -{\bf \Gamma}\times {\bf H}$ and ${\bf B} =\muo {\bf H} + {\bf \Gamma}\times{\bf E}$). Scattering by a three-dimensional object composed of…

Second and third harmonic signals have been usually generated by using nonlinear crystals, but that method suffers from the low efficiency in small thicknesses. Metamaterials can be used to generate harmonic signals in small thicknesses.…

Optics · Physics 2016-07-28 Iman Sajedian , Inki Kim , Abdolnasser Zakery , Junsuk Rho

Nonlinear optical phenomena in nanostructured materials have been challenging our perceptions of nonlinear optical processes that have been explored since the invention of lasers. For example, the ability to control optical field…

Classical nonlocality in conducting nanostructures has been shown to dramatically alter the linear optical response, by placing a fundamental limit on the maximum field enhancement that can be achieved. This limit directly extends to all…

Mesoscale and Nanoscale Physics · Physics 2013-11-14 Cristian Ciracì , Michael Scalora , David R. Smith

Material systems with lone-pair electrons have long been a treasure trove in the search for large second harmonic generation effects. Revealing the origin of second harmonic generation in nonlinear optical materials can provide theoretical…

Materials Science · Physics 2025-05-13 Fuming Li , Shilie Pan , Zhihua Yang

Two-dimensional semiconductors have emerged as a new class of materials for nanophotonics for their strong exciton-photon interaction and flexibility for engineering and integration. Taking advantage of these properties, we engineer an…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Eunice Y. Paik , Long Zhang , G. William Burg , Rahul Gogna , Emanuel Tutuc , Hui Deng

High-harmonic generation (HHG) from a compact, solid-state medium is highly desirable for applications such as coherent attosecond pulse generation and extreme ultra-violet (EUV) spectroscopy, yet the typically weak conversion of pump light…

We observe strongly anisotropic third-harmonic generation mediated by resonant sum-frequency driving of Raman phonons with THz light, extending light-induced dual control of structural and optical properties in solids. Either strong…

Optics · Physics 2024-05-03 Jiaoyang Zheng , Guru Khalsa , Jeffrey Moses

In this paper, the detection of a small reflector in a randomly heterogenous medium using second-harmonic generation is investigated. The medium is illuminated by a time-harmonic plane wave at frequency omega. It is assumed that the…

Analysis of PDEs · Mathematics 2013-06-26 Habib Ammari , Josselin Garnier , Pierre Millien

We experimentally investigate second harmonic generation from strongly coupled localized and propagative phonon polariton modes in arrays of silicon carbide nanopillars. Our results clearly demonstrate the hybrid nature of the system's…

The discovery of second harmonic generation in 1961 marked the birth of nonlinear optics, unlocking a range of applications from frequency conversion to quantum light generation. Yet, phase matching in bulk nonlinear crystals remains a key…

Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light-matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are…