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Electromigrated nanoscale junctions have proven very useful for studying electronic transport at the single-molecule scale. However, confirming that conduction is through precisely the molecule of interest and not some contaminant or metal…

Mesoscale and Nanoscale Physics · Physics 2008-09-04 D. R. Ward , G. D. Scott , Z. K. Keane , N. J. Halas , D. Natelson

Electrically connected and plasmonically enhanced molecular junctions combine the optical functionalities of high field confinement and enhancement (cavity function), and of high radiative efficiency (antenna function) with the electrical…

The accurate determination of electronic temperatures in metallic nanostructures is essential for many technological applications, like plasmon-enhanced catalysis or lithographic nanofabrication procedures. In this Letter we demonstrate…

Understanding and controlling the flow of heat is a major challenge in nanoelectronics. When a junction is driven out of equilibrium by light or the flow of electric charge, the vibrational and electronic degrees of freedom are, in general,…

Mesoscale and Nanoscale Physics · Physics 2011-06-29 Daniel R. Ward , David A. Corley , James M. Tour , Douglas Natelson

Temperature imaging of nanoscale systems is a fundamental problem which has myriad potential technological applications. For example, nanoscopic cold spots can be used for spot cooling electronic components while hot spots could be used for…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 Abhay Shastry , Sosuke Inui , Charles A. Stafford

Thermal transport in nanostructures plays a critical role in modern technologies. As devices shrink, techniques that can measure thermal properties at nanometer and nanosecond scales are increasingly needed to capture transient,…

Plasmonic absorption of light can lead to significant local heating in metallic nanostructures, an effect that defines the sub-field of thermoplasmonics and has been leveraged in diverse applications from biomedical technology to…

Mesoscale and Nanoscale Physics · Physics 2014-02-21 Joseph B. Herzog , Mark W. Knight , Douglas Natelson

Surface plasmon enhanced processes and hot-carrier dynamics in plasmonic nanostructures are of great fundamental interest to reveal light-matter interactions at the nanoscale. Using plasmonic tunnel junctions as a platform supporting both…

Understanding the electronic and phononic transport properties of junctions consisting of a scattering region such as a nanoscale matters or molecules connected to two or more electrodes is the central basis for future nano and molecular…

Mesoscale and Nanoscale Physics · Physics 2016-07-11 Hatef Sadeghi

The search for the signature of non-thermal (so-called ``hot'') electrons in illuminated plasmonic nanostructures requires a detailed understanding of the non-equilibrium electron distribution under illumination, as well as a careful design…

Mesoscale and Nanoscale Physics · Physics 2023-03-31 Yonatan Dubi , Ieng-Wai Un , Yonatan Sivan

While the thermal and electromagnetic properties of plasmonic nanostructures are well understood, nanoscale thermometry still presents an experimental and theoretical challenge. Plasmonic structures can confine electromagnetic energy at the…

Noise measurements are a probe beyond simple electronic transport that can reveal additional information about electronic correlations and inelastic processes. Here we report noise measurements in individual electromigrated nanojunctions,…

Mesoscale and Nanoscale Physics · Physics 2013-06-28 P. J. Wheeler , Ruoyu Chen. , D. Natelson

Plasmonic molecular nanojunctions exhibit opto-mechanical coupling at the nanoscale, enabling intertwined optical, vibrational and electronic phenomena. Here, we demonstrate plasmon-mediated phonon pumping, driven by inelastic electron…

Metal nanostructures act as powerful optical antennas[1, 2] because collective modes of the electron fluid in the metal are excited when light strikes the surface of the nanostructure. These excitations, known as plasmons, can have…

Mesoscale and Nanoscale Physics · Physics 2011-04-04 Daniel R. Ward , Falco Hueser , Fabian Pauly , Juan Carlos Cuevas , Douglas Natelson

We investigate the thermopower of a metal-molecule-metal junction taking into account thermal effects on the junction. Based on analytical expressions and numerical simulations we show that the thermoelectric potential reveals valuable…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Dvira Segal

Plasmons --the collective oscillations of electrons in conducting materials-- play a pivotal role in nanophotonics because of their ability to couple electronic and photonic degrees of freedom. In particular, plasmons in graphene --the…

Materials Science · Physics 2018-05-08 Renwen Yu , F. Javier García de Abajo

Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub{\aa}ngstrom and femtosecond spatiotemporal resolution. We present a theory predicting that…

Leveraging thermal losses as a useful consequence of surface plasmons in metal nanostructures has gained traction in recent years. This thermalization of hot electrons also induces a resistance change to an applied bias current, which we…

Optics · Physics 2024-12-23 Alec R. Cheney , Borui Chen , Tim Thomay

Energy and charge transfer between molecules and metal surfaces underpin heterogeneous catalysis, surface-enhanced spectroscopies and plasmon-driven chemistry, yet the microscopic origins of vibrational excitation at metal interfaces remain…

Mesoscale and Nanoscale Physics · Physics 2026-01-26 Bing Gao , Jameel Damoah , Wassie M. Takele , Terefe G. Habteyes

We have developed an efficient scalable kernel method for thermal transport in open systems, with which we have computed the thermal conductance of a junction between bulk silicon and silicon nanowires with diameter up to 10 nm. We have…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Ivan Duchemin , Davide Donadio
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