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The linear energy dispersion of graphene electrons leads to a strongly nonlinear electromagnetic response of this material. We develop a general quantum theory of the third-order nonlinear local dynamic conductivity of graphene…

Mesoscale and Nanoscale Physics · Physics 2016-02-04 S. A. Mikhailov

Graphene is emerging as a viable alternative to conventional optoelectronic, plasmonic, and nanophotonic materials. The interaction of light with carriers creates an out-of-equilibrium distribution, which relaxes on an ultrafast timescale…

Mesoscale and Nanoscale Physics · Physics 2013-06-25 D. Brida , A. Tomadin , C. Manzoni , Y. J. Kim , A. Lombardo , S. Milana , R. R. Nair , K. S. Novoselov , A. C. Ferrari , G. Cerullo , M. Polini

We present the first experimental investigation of nonlinear optical properties of graphene flakes. We find that at near infrared frequencies a graphene monolayer exhibits a remarkably high third-order optical nonlinearity which is…

Materials Science · Physics 2011-01-13 E. Hendry , P. J. Hale , J. J. Moger , A. K. Savchenko , S. A. Mikhailov

A non-perturbative model for graphene optical nonlinearity is developed for the study of ultrafast pulse propagation along a monolayer, as in the case of graphene-comprising nanophotonic integrated waveguides. This graphene `hot electron'…

Optics · Physics 2022-03-18 Alexandros Pitilakis , Emmanouil E. Kriezis

We present here a general formulation for the interband dynamical optical conductivity in the nonlinear regime of graphene in the presence of a quantum bath comprising phonons and electrons. Our main focus is the relaxation behavior of the…

Mesoscale and Nanoscale Physics · Physics 2023-07-10 Bristi Ghosh , Sushanta Dattagupta , Malay Bandyopadhyay

Graphene placed in a magnetic field possesses an extremely high mid/far-infrared optical nonlinearity originating from its unusual band structure and selection rules for the optical transitions near the Dirac point. Here we study the linear…

Mesoscale and Nanoscale Physics · Physics 2016-11-26 Xianghan Yao , Alexey Belyanin

The ability of graphene to support long-lived, electrically tunable plasmons that interact strongly with light, combined with its highly nonlinear optical response, has generated great expectations for application of the atomically-thin…

Mesoscale and Nanoscale Physics · Physics 2017-04-12 Joel D. Cox , Iván Silveiro , F. Javier García de Abajo

We present perturbation theory for analysis of generic third-order nonlinear processes in graphene integrated photonic structures. Optical response of graphene is treated as the nonlinear boundary condition in Maxwell equations. The derived…

Optics · Physics 2016-07-13 Andrey V. Gorbach , Edouard Ivanov

An electromagnetic response of a single graphene layer to a uniform, arbitrarily strong electric field $E(t)$ is calculated by solving the kinetic Boltzmann equation within the relaxation-time approximation. The theory is valid at low…

Mesoscale and Nanoscale Physics · Physics 2018-04-26 S. A. Mikhailov

Graphene is a two-dimensional material with strongly nonlinear electrodynamics and optical properties. We present some of our recent theoretical results on the quantum and non-perturbative quasi-classical theories of nonlinear effects in…

Mesoscale and Nanoscale Physics · Physics 2018-10-02 S. A. Mikhailov , N. A. Savostianova

We develop a microscopic large-$N$ theory of electron-electron interaction corrections to multi-legged Feynman diagrams describing second- and third-order nonlinear response functions. Our theory, which reduces to the well-known random…

Materials Science · Physics 2017-01-25 Habib Rostami , Mikhail I. Katsnelson , Marco Polini

Hot electron effects in graphene are significant because of graphene's small electronic heat capacity and weak electron-phonon coupling, yet the dynamics and cooling mechanisms of hot electrons in graphene are not completely understood. We…

Nonperturbative approach based on exact solution of Boltzmann kinetic equation in the relaxation time approximation is developed for the study of nonlinear response of electron-doped few-layer graphene to a high-frequency electromagnetic…

Mesoscale and Nanoscale Physics · Physics 2020-03-06 D. V. Fil

Position measurements at the quantum level are vital for many applications, but also challenging. Typically, methods based on optical phase shifts are used, but these methods are often weak and difficult to apply to many materials. An…

Intense efforts have been made in recent years to realize nonlinear optical interactions at the single-photon level. Much of this work has focused on achieving strong third-order nonlinearities, such as by using single atoms or other…

Mesoscale and Nanoscale Physics · Physics 2015-08-25 Marco T. Manzoni , Iván Silveiro , F. Javier García de Abajo , Darrick E. Chang

Graphene exhibits extremely strong optical nonlinearity when a strong perpendicular magnetic field is applied, the response current shows strong field dependence even for moderate light intensity, and the perturbation theory fails. We…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 J. L. Cheng , C. Guo

Understanding the ultrafast carrier dynamics of graphene on a substrate is a fundamental step in the development of graphene based opto-electronic devices. Here, we present ultrafast pump-probe measurements of supported graphene on quartz…

Mesoscale and Nanoscale Physics · Physics 2021-02-16 Rustam Gatamov , Andrey Baydin , Halina Krzyzanowska , Norman Tolk

Nonlinear-optical refraction is typically described by means of perturbation theory near the material's equilibrium state. Graphene, however, can easily move far away from its equilibrium state upon optical pumping, yielding strong…

Optics · Physics 2020-02-14 David Castello-Lurbe , Hugo Thienpont , Nathalie Vermeulen

An electrodynamic response of graphene to a strong electromagnetic radiation is considered. A hot electron model (HEM) is introduced and a corresponding system of nonlinear equations is formulated. Solutions of this system are found and…

Mesoscale and Nanoscale Physics · Physics 2019-09-18 S. A. Mikhailov

Graphene is a recently discovered carbon based material with unique physical properties. This is a monolayer of graphite, and the two-dimensional electrons and holes in it are described by the effective Dirac equation with a vanishing…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 S. A. Mikhailov , K. Ziegler
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