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We show that classical molecular density functional theory (MDFT), here in the homogeneous reference fluid approximation in which the functional is inferred from the properties of the bulk solvent, is a powerful new tool to study, at a…

Vapor bubbles are formed in liquids by two mechanisms: evaporation (temperature above the boiling threshold) and cavitation (pressure below the vapor pressure). The liquid resists in these metastable (overheating and tensile, respectively)…

Soft Condensed Matter · Physics 2018-05-30 Mirko Gallo , Francesco Magaletti , Carlo Massimo Casciola

This is the second in a series of three papers in which we study a two-dimensional lattice gas consisting of two types of particles subject to Kawasaki dynamics at low temperature in a large finite box with an open boundary. Each pair of…

Probability · Mathematics 2015-05-28 Frank den Hollander , Francesca R. Nardi , Alessio Troiani

Nucleation is very common physical phenomena that occur at the microscopic scale. However, due to the presence of nucleation barriers, the time scale of nucleation is usually much longer than that of microscopic particle dynamics. These…

Chemical Physics · Physics 2023-08-08 Zihao Bai

Central nucleon-nucleon potentials involving forbidden states are obtained for the Gaussian, exponential, and Yukawa type. The parameters of interaction are obtained by fitting the scattering phase shifts for energies up to 500 MeV,…

Nuclear Theory · Physics 2007-05-23 S. B. Dubovichenko

Density functional theory (DFT) is an efficient instrument for describing a wide range of nanoscale phenomena: wetting transition, capillary condensation, adsorption, etc. In this paper, we suggest a method for obtaining the equilibrium…

Computational Physics · Physics 2021-06-18 Yuriy Kanygin , Irina Nesterova , Pavel Lomovitskiy , Aleksey Khlyupin

Dynamical density functional theory (DDFT) has been successfully derived and applied to describe on the one hand passive colloidal suspensions, including hydrodynamic interactions between individual particles. On the other hand, active…

Statistical Mechanics · Physics 2016-01-18 Andreas M. Menzel , Arnab Saha , Christian Hoell , Hartmut Löwen

Heterogeneous nucleation is studied by Monte Carlo simulations and phenomenological theory, using the two-dimensional lattice gas model with suitable boundary fields. A chemical inhomogeneity of length b at one boundary favors the liquid…

Statistical Mechanics · Physics 2018-04-04 Marta L. Trobo , Ezequiel V. Albano , Kurt Binder

The main goal of this paper is to assess the limits of validity, in the regime of low concentration and strong Coulomb coupling (high molecular charges), for a simple perturbative approximation to the radial distribution functions (RDF),…

Statistical Mechanics · Physics 2009-11-11 Achille Giacometti , Domenico Gazzillo , Giorgio Pastore , T. Kanti Das

The effective capillary interaction potentials for small colloidal particles trapped at the surface of liquid droplets are calculated analytically. Pair potentials between capillary monopoles and dipoles, corresponding to particles floating…

Soft Condensed Matter · Physics 2015-05-27 J. Guzowski , M. Tasinkevych , S. Dietrich

Despite its relevance in biology and engineering, the molecular mechanism driving cavitation in water remains unknown. Using computer simulations, we investigate the structure and dynamics of vapor bubbles emerging from metastable water at…

Using the formalism of the classical nucleation theory, we derive an expression for the reversible work $W_*$ of formation of a binary crystal nucleus in a liquid binary solution of non-stoichiometric composition (incongruent…

Chemical Physics · Physics 2017-04-26 Yuri S. Djikaev , Eli Ruckenstein

Thermodynamic perturbation theory for central-force (TPT-CF) type of associating potential is used to study the phase behavior of symmetric binary mixture of associating particles with spherically symmetric interaction. The model is…

Soft Condensed Matter · Physics 2013-12-18 Yu. V. Kalyuzhnyi , T. V. Hvozd

Nuclear density functional theory (DFT) is the tool of choice in describing properties of complex nuclei and intricate phases of bulk nucleonic matter. It is a microscopic approach based on an energy density functional representing the…

Nuclear Theory · Physics 2016-11-30 Bastian Schuetrumpf , Chunli Zhang , Witold Nazarewicz

The basic physics of nucleation in solid \hl{single-crystal} nanoparticles is revealed by a phase-field theory that includes surface energy, chemical reactions and coherency strain. In contrast to binary fluids, which form arbitrary contact…

Materials Science · Physics 2014-09-17 Daniel A. Cogswell , Martin Z. Bazant

We numerically study the effect of an active turbulent environment on a passive deformable droplet. The system is simulated using coupled hydrodynamic and nematodynamic equations for nematic liquid crystals with an active stress which is…

Soft Condensed Matter · Physics 2024-05-06 Chamkor Singh , Abhishek Chaudhuri

Results for the kinetics of vapor-liquid transitions, following temperature quenches with different densities, are presented from the molecular dynamics simulations of a Lennard-Jones system. For critical density, bicontinuous liquid and…

Statistical Mechanics · Physics 2018-03-09 Sutapa Roy , Subir K. Das

We analyze the depletion interaction between two hard colloids in a hard--sphere solvent and pay special attention to the limit of large size ratio between colloids and solvent particles which is governed by the well--known Derjaguin…

Soft Condensed Matter · Physics 2007-05-23 M. Oettel

Results from Monte Carlo simulations of wall-attached droplets in the three-dimensional Ising lattice gas model and in a symmetric binary Lennard-Jones fluid, confined by antisymmetric walls, are analyzed, with the aim to estimate the…

Soft Condensed Matter · Physics 2018-07-04 Subir K. Das , Sergei A. Egorov , Peter Virnau , David Winter , Kurt Binder

The profile of vapor around the droplet growing in the diffusion regime with known moving boundary have been calculated and expressed in terms of special functions.

Statistical Mechanics · Physics 2007-05-23 V. Kurasov