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Using state-of-the-art rare-event sampling simulations, we precisely characterize the nucleation of liquid droplets from a supersaturated Lennard-Jones gas and uncover a key physical feature: critical clusters nucleate with a density that…

Chemical Physics · Physics 2026-01-07 Yijian Wu , Thomas Philippe , Aymane Graini , Julien Lam

Particles dispersed in a liquid crystal above the nematic-isotropic phase transition are wetted by a surface-induced corona of paranematic order. Such coronas give rise to pronounced two-particle interactions. In this article, we report…

Soft Condensed Matter · Physics 2009-11-10 Paolo Galatola , Jean-Baptiste Fournier , Holger Stark

We introduce a simple model consisting of two or three coupled one-dimensional channels of particles with Yukawa interactions. For the two channel system, when an external drive is applied only to the top or primary channel, we find a…

Soft Condensed Matter · Physics 2015-05-20 C. Reichhardt , C. Bairnsfather , C. J. Olson Reichhardt

Monte Carlo simulations of mono-- and polydisperse two--dimensional crystals are reported. The particles in the studied system, interacting through hard--core repulsive Yukawa potential, form a solid phase of hexagonal lattice. The elastic…

Computational Physics · Physics 2023-07-19 Jakub W. Narojczyk , P. M. Piglowski , K. W. Wojciechowski , K. V. Tretiakov

Systems with long-range interactions when quenced into a metastable state near the pseudo-spinodal exhibit nucleation processes that are quite different from the classical nucleation seen near the coexistence curve. In systems with…

Materials Science · Physics 2009-11-07 W. Klein , T. Lookman , A. Saxena , D. Hatch

We examine the nanoscale behavior of an equilibrium three-phase contact line in the presence of long-ranged intermolecular forces by employing a statistical mechanics of fluids approach, namely density functional theory (DFT) together with…

Fluid Dynamics · Physics 2014-08-05 Andreas Nold , David N. Sibley , Benjamin D. Goddard , Serafim Kalliadasis

A common approach to study nucleation rates is the estimation of free-energy barriers. This usually requires knowledge about the shape of the forming droplet, a task that becomes notoriously difficult in macromolecular setups starting with…

Statistical Mechanics · Physics 2017-03-28 Johannes Zierenberg , Philipp Schierz , Wolfhard Janke

The depletion potential between two hard spheres in a solvent of thin hard disclike platelets is investigated by using either the Derjaguin approximation or density functional theory. Particular attention is paid to the density dependence…

Soft Condensed Matter · Physics 2009-11-10 L. Harnau , S. Dietrich

Brownian particles interacting via repulsive soft-core potentials can spontaneously aggregate, despite repelling each other, and form periodic crystals of particle clusters. We study this phenomenon in low-dimensional situations (one and…

Density functional theory (DFT) is a powerful theoretical tool widely used in such diverse fields as computational condensed matter physics, atomic physics, and quantum chemistry. DFT establishes that a system of $N$ interacting electrons…

Plasma Physics · Physics 2020-04-29 Giovanni Manfredi

Classical density functional theory (DFT) is a statistical mechanical theory for calculating the density profiles of the molecules in a liquid. It is widely used, for example. to calculate the density distribution of the molecules in the…

Statistical Mechanics · Physics 2015-07-08 Adam P. Hughes , Uwe Thiele , Andrew J. Archer

Colloidal particles that are confined to an interface effectively form a two-dimensional fluid. We examine the dynamics of such colloids when they are subject to a constant external force, which drives them in a particular direction over…

Soft Condensed Matter · Physics 2011-06-24 Andrew J. Archer , Alexandr Malijevsky

Using classical density functional theory (DFT) the effect of bringing a liquid crystal (LC) into contact with a porous substrate or matrix is investigated. The DFT used is a combination of the Onsager approximation to evaluate the excess…

Soft Condensed Matter · Physics 2007-05-23 David L. Cheung

Phase diagrams of some globular proteins have a fluid-fluid transition as well as a fluid-crystal transition. Homogeneous nucleation of the crystal from the fluid phase near the critical point of the fluid-fluid transition is examined. As…

Soft Condensed Matter · Physics 2009-10-31 Richard P. Sear

We present some new results on heavy-element nuclear-structure properties calculated on the basis of the finite-range droplet model and folded-Yukawa single-particle potential. Specifically, we discuss calculations of nuclear ground-state…

Nuclear Theory · Physics 2007-05-23 Peter Möller , J. Rayford Nix

Particle beams are important tools for probing atomic and molecular interactions. Here we demonstrate that particle beams also offer a unique opportunity to investigate interactions in macroscopic systems, such as granular media. Motivated…

Soft Condensed Matter · Physics 2015-05-19 Scott R. Waitukaitis , Helge F. Gruetjen , John R. Royer , Heinrich M. Jaeger

Hard-sphere fluids confined between parallel plates a distance $D$ apart are studied for a wide range of packing fractions, including also the onset of crystallization, applying Monte Carlo simulation techniques and density functional…

Statistical Mechanics · Physics 2011-10-10 Debabrata Deb , Alexander Winkler , Mohammad Hossein Yamani , Martin Oettel , Peter Virnau , Kurt Binder

This study proposes a dynamic model to reflect the physical image of the droplet breakup process in two-phase detonation flows. This breakup model is implemented in a two-phase detonation solver developed based on an open-source…

Fluid Dynamics · Physics 2024-04-05 Wenhao Wang , Miao Yang , Zongmin Hu , Peng Zhang

The effective pair potential between mesoscopic charged particles in a neutralising background medium takes a Yukawa form $\exp(-\lambda r)/r$ with screening length $\lambda^{-1}$. We consider a dilute suspension of such Yukawa particles…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer , P. Hopkins , R. Evans

For isotropic fluids, classical nucleation theory predicts the nucleation rate, barrier height and critical droplet size by accounting for the competition between bulk energy and interfacial tension. The nucleation process in liquid…

Soft Condensed Matter · Physics 2017-08-01 Amit Kumar Bhattacharjee
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