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Related papers: Two-center minima in harmonic spectra from aligned…

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We theoretically investigate the interference effect of high-order harmonics generated from molecules at different alignment angles. It is shown that the interference of the harmonic emissions from molecules aligned at different angles can…

Optics · Physics 2015-02-27 Meiyan Qin , Xiaosong Zhu , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We present a theoretical investigation into the two-center interference in aligned H$_2^+$. The influence of the laser field on the recombination step is investigated by comparing laser-induced harmonic generation with harmonic generation…

Atomic Physics · Physics 2015-05-19 Elmar V. van der Zwan , Manfred Lein

We report theoretical calculations on the effect of the multiple orbital contribution in high-order harmonic generation (HHG) from aligned CO$_2$ with inclusion of macroscopic propagation of harmonic fields in the medium. Our results show…

Atomic Physics · Physics 2011-05-10 Cheng Jin , Anh-Thu Le , C. D. Lin

We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center interference condition for elliptically polarized fields,…

Atomic Physics · Physics 2015-06-16 T. Das , B. B. Augstein , C. Figueira de Morisson Faria

We utilize few-level model systems to analyze the polarization and phase properties of below-threshold harmonics generated from aligned molecules. In a two-level system, we find that the phase of emitted harmonics undergoes a distinct…

Quantum Physics · Physics 2026-05-06 Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

We investigate high-order harmonic spectra from aligned diatomic molecules in intense driving fields whose components have orthogonal polarizations. We focus on how the driving-field ellipticity influences structural interference patterns…

We investigate the alignment-dependent high-order harmonic spectrum generated from nonadiabatically aligned molecules around the first half rotational revival. It is found that the evolution of the molecular alignment is encoded in the…

Atomic Physics · Physics 2014-03-13 Meiyan Qin , Xiaosong Zhu , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…

We study the Cooper minimum in high harmonic generation from argon atoms using long wavelength laser pulses. We find that the minimum in high harmonic spectra is systematically shifted with respect to total photoionization cross section…

We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic…

Atomic Physics · Physics 2009-11-13 Xibin Zhou , Robynne Lock , Wen Li , Nick Wagner , Margaret. M. Murnane , Henry C. Kapteyn

Proposals for quantum computing using rotational states of polar molecules as qubits have previously considered only diatomic molecules. For these the Stark effect is second-order, so a sizable external electric field is required to produce…

Quantum Physics · Physics 2015-05-30 Qi Wei , Sabre Kais , Bretislav Friedrich , Dudley Herschbach

We analyze the influence of different recombination scenarios, involving one or two centers, on high-order harmonic generation (HHG) in diatomic molecules, for different values of the internuclear separation. We work within the strong-field…

Atomic Physics · Physics 2015-05-13 C. Figueira de Morisson Faria

We study the effect of an electric-field on an electron-hole pair in an asymmetric system of vertically coupled self-assembled quantum dots taking into account their non-perfect alignment. We show that the non-perfect alignment does not…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 B. Szafran , F. M. Peeters , S. Bednarek

An improved quantum trajectory Monte Carlo method involving the Stark shift of the initial state, Coulomb potential, and multielectron polarization-induced dipole potential is used to revisit the origin of the low-energy interference…

Atomic Physics · Physics 2021-05-12 Weifeng Yang , Jie Li , Wenbin Jia , Hongdan Zhang , Xiwang Liu , Ming Zhu , Xiaohong Song , Jing Chen

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

Atomic Physics · Physics 2011-11-10 C. Figueira de Morisson Faria

We consider electronic transport through break-junctions bridged by a single molecule in the Kondo regime. We describe the system by a two-channel Anderson model. We take the tunneling matrix elements to depend on the position of the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Jernej Mravlje , Anton Ramsak

We show that combined permanent and induced electric dipole interactions of polar and polarizable molecules with collinear electric fields lead to a sui generis topology of the corresponding Stark energy surfaces and of other observables -…

Chemical Physics · Physics 2023-02-09 Burkhard Schmidt , Bretislav Friedrich

A theoretical study of the rotational dynamics of a linear polar molecule in a two-color non-resonant cw laser field is presented. By systematically considering the interactions of this field with the electric dipole moment, polarizability…

Quantum Physics · Physics 2020-08-26 David Mellado-Alcedo , Niurka R. Quintero , Rosario González-Férez

We present single-molecule and macroscopic calculations showing that laser-induced Stark shifts contribute significantly to the phase of high-order harmonics from polar molecules. This is important for orbital tomography, where phases of…

Quantum Physics · Physics 2015-06-05 Adam Etches , Mette B. Gaarde , Lars Bojer Madsen
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