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We present an efficient method for propagating the time-dependent Kohn-Sham equations in free space, based on the recently introduced Fourier contour deformation (FCD) approach. For potentials which are constant outside a bounded domain,…

Chemical Physics · Physics 2023-07-10 Jason Kaye , Alex Barnett , Leslie Greengard , Umberto De Giovannini , Angel Rubio

We describe linear and nonlinear transport across a single impurity Anderson model quantum dot with intermediate coupling to the leads, i.e., with tunnel coupling of the order of the thermal energy k_B T. The coupling is large enough that…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Johannes Kern , Milena Grifoni

An argument is given showing that Coulomb attraction between conduction electrons and impurity ions in a dilute magnetic alloy (DMA) can be disregarded, provided the system's inverse temperature beta is replaced by an effective inverse…

Statistical Mechanics · Physics 2007-05-23 Jan Mackowiak

We investigate the time an electronic excitation travels in a supermolecular setup using a measurement process in an open quantum-system framework. The approach is based on the stochastic Schr\"odinger equation and uses a Hamiltonian from…

Materials Science · Physics 2013-12-09 Dirk Hofmann , Heiko Appel , Massimiliano Di Ventra , Stephan Kümmel

The formally exact framework of equilibrium Density Functional Theory (DFT) is capable of simultaneously and consistently describing thermodynamic and structural properties of interacting many-body systems in arbitrary external potentials.…

We present here a theoretical method to determine the phononic contribution to the thermal conductance of nanoscale systems in the phase-coherent regime. Our approach makes use of classical molecular dynamics (MD) simulations to calculate…

Mesoscale and Nanoscale Physics · Physics 2022-11-09 Fabian Müller , Peter Nielaba , Juan Carlos Cuevas , Fabian Pauly

The splitting of the Kondo resonance in the density of states of an Anderson impurity in finite magnetic field is calculated from the exact Bethe-ansatz solution. The result gives an estimate of the electron spectral function for nonzero…

Strongly Correlated Electrons · Physics 2009-10-31 Joel E. Moore , Xiao-Gang Wen

The zero-bias resonance in the dI/dV tunneling spectrum recorded using a scanning tunneling microscope above a spin-1/2 magnetic adatom (such as Ti) adsorbed on a decoupling layer on metal surface can be accurately fitted using the…

Mesoscale and Nanoscale Physics · Physics 2012-02-24 Rok Zitko

We present a perturbative approach within the scope of Kohn-Sham density functional theory (DFT). The method is based on the exact exchange-only optimized effective potential method, and correlation is included via perturbation expansion…

Chemical Physics · Physics 2007-05-23 P. Sule

Above the Kondo temperature, the Kohn-Sham zero-bias conductance of an Anderson junction has been shown to completely miss the Coulomb blockade. Within a standard model for the spectral function, we deduce a parameterization for both the…

Strongly Correlated Electrons · Physics 2015-07-30 Zhenfei Liu , Kieron Burke

Recently, thermally-assisted-occupation density functional theory (TAO-DFT) [J.-D. Chai, J. Chem. Phys. 136, 154104 (2012)] has been demonstrated to be an efficient and accurate electronic structure method for studying the ground-state…

Chemical Physics · Physics 2026-03-03 Shaozhi Li , Jeng-Da Chai

The Kondo zero bias anomaly of Co adatoms probed by scanning tunneling microscopy is known to depend on the height of the tip above the surface, and this dependence is different on different low index Cu surfaces. On the (100) surface, the…

Strongly Correlated Electrons · Physics 2019-07-24 P. P. Baruselli , R. Requist , A. Smogunov , M. Fabrizio , E. Tosatti

This chapter presents controlled approximations of Kohn-Sham density functional theory (DFT) that enable very large scale simulations. The work is motivated by the study of defects in crystalline solids, though the ideas can be used in…

Materials Science · Physics 2021-12-14 Kaushik Bhattacharya , Vikram Gavini , Michael Ortiz , Mauricio Ponga , Phanish Suryanarayana

We study non-perturbative aspects of QCD Kondo effect, which has been recently proposed for the finite density and strong magnetic field systems, using conformal field theory describing the low energy physics near the IR fixed point. We…

High Energy Physics - Phenomenology · Physics 2019-02-06 Taro Kimura , Sho Ozaki

We study the Kondo effect in a model system of a quantum dot embedded in an Aharanov-Bohm ring connected to two leads. By transforming to the scattering basis of the direct inter-lead tunneling, we are able to describe precisely how the…

Mesoscale and Nanoscale Physics · Physics 2010-10-15 Justin Malecki , Ian Affleck

We calculate the energy deposition by very short laser pulses in SiO_2 (alpha-quartz) with a view to establishing systematics for predicting damage and nanoparticle production. The theoretical framework is time-dependent density functional…

Materials Science · Physics 2015-11-18 S. A. Sato , K. Yabana , Y. Shinohara , T. Otobe , K. M. Lee , G. F. Bertsch

It was recently shown [Y. Suzuki, L. Lacombe, K. Watanabe, and N. T. Maitra, Phys. Rev. Lett. 119, 263401 (2017)] that peak and valley structures in the exact exchange-correlation potential of time-dependent density functional theory are…

Chemical Physics · Physics 2018-07-04 Lionel Lacombe , Yasumitsu Suzuki , Kazuyuki Watanabe , Neepa T. Maitra

Traditional finite-temperature Kohn-Sham density functional theory (KSDFT) has an unfavorable scaling with respect to the electron number or at high temperatures. The evaluation of the ground-state density in KSDFT can be replaced by the…

Computational Physics · Physics 2022-10-05 Qianrui Liu , Mohan Chen

We present a {\it nonequilibrium nonperturbative} field theory for the Kondo effect in strongly interacting quantum dots at finite temperatures. Unifying the slave-boson representation with the Keldysh field integral an effective Keldysh…

Mesoscale and Nanoscale Physics · Physics 2011-09-08 Sergey Smirnov , Milena Grifoni

A microscopic finite-temperature model based on time-dependent nuclear density functional theory (TDDFT), is employed to study the induced-fission process of $^{226}$Th. The saddle-to-scission dynamics of this process is explored, starting…

Nuclear Theory · Physics 2024-09-11 B. Li , D. Vretenar , T. Nikšić , P. W. Zhao , J. Meng