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Spin correlations of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by using inelastic neutron scattering on single crystalline samples ($x=-0.007, 0.000,$ and $0.003$), which have the putative…

Strongly Correlated Electrons · Physics 2019-01-08 Hiroaki Kadowaki , Mika Wakita , Björn Fåk , Jacques Ollivier , Seiko Ohira-Kawamura , Kenji Nakajima , Jeffrey W. Lynn

We present a comprehensive experimental investigation of the temperature evolution of magnetic states in triangular-lattice delafossite YbCuSe$_2$. Magnetization measurements on high-quality single crystals reveal easy-plane anisotropy.…

Strongly Correlated Electrons · Physics 2026-04-08 K. Bhattacharya , Y. Tokiwa , M. Majumder

Spin correlations in the pyrochlore antiferromagnet Y_2Ru_2O_7 with Curie-Weiss temperature $\Theta_{CW}=-1100$ K and critical temperature T_N=77 K were examined through neutron scattering. For $T_N<T<\Theta_{CW}/3$ the data show spin…

Strongly Correlated Electrons · Physics 2014-07-03 J. van Duijn , N. Hur , J. W. Taylor , Y. Qiu , Q. Z. Huang , S. -W. Cheong , C. Broholm , T. G. Perring

We have investigated the spin fluctuations and their interplay with lattice instabilities in a layered S=1/2 quantum spin system TiOCl. Our Ti and Cl NMR data demonstrate a pseudo spin-gap behavior below T*=135 K, followed by successive…

Strongly Correlated Electrons · Physics 2007-05-23 T. Imai , F. C. Chou

Muon spin rotation (muSR) experiments reveal unconventional spin freezing and dynamics in the two-dimensional (2D) triangular lattice antiferromagnet NiGa2S4. Long-lived disordered Ni-spin freezing (correlation time > 10-6 s at 2 K) sets in…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Nambu , S. Nakatsuji , R. H. Heffner , Lei Shu , O. O. Bernal , K. Ishida

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

Statistical Mechanics · Physics 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

By performing time-of-flight neutron scattering measurements on a large amount of single crystals of Sr$_2$RuO$_4$, we studied detailed structure of the imaginary part of the dynamic spin susceptibility over a wide range of phase space. In…

Strongly Correlated Electrons · Physics 2015-05-28 K. Iida , M. Kofu , N. Katayama , J. Lee , R. Kajimoto , Y. Inamura , M. Nakamura , M. Arai , Y. Yoshida , M. Fujita , K. Yamada , S. -H. Lee

The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in La$_{1.93}$Sr$_{0.07}$CuO$_4$, a superconductor…

Superconductivity · Physics 2015-11-25 H. Jacobsen , I. A. Zaliznyak , A. T. Savici , B. L. Winn , S. Chang , M. Huecker , G. D. Gu , J. M. Tranquada

After several decades of studies of high-temperature superconductivity, there is no compelling theory for the mechanism yet; however, the spin fluctuations have been widely believed to play a crucial role in forming the superconducting…

We have performed neutron scattering experiments on the heavy fermion superconductor URu$_2$Si$_2$ to search for the orbital currents predicted to exist in the ordered phase below {\Tn} = 17.5 K. Elastic scans in the (H, K, 0) and (H, 0, L)…

Strongly Correlated Electrons · Physics 2007-05-23 C. R. Wiebe , G. M. Luke , Z. Yamani , A. A. Menovsky , W. J. L. Buyers

We report on diffuse neutron scattering experiments providing evidence for the presence of random strains in the quantum spin ice candidate Pr2Zr2O7. Since Pr is a non-Kramers ion, the strain deeply modifies the picture of Ising magnetic…

Strongly Correlated Electrons · Physics 2017-08-08 N. Martin , P. Bonville , E. Lhotel , S. Guitteny , A. Wildes , C. Decorse , M. Ciomaga Hatnean , G. Balakrishnan , I. Mirebeau , S. Petit

We interpret recent measurements of the zero field muon relaxation rate in the frustrated magnetic pyrochlore Dy$_2$Ti$_2$O$_7$ as resulting from the quantum diffusion of muons in the substance. In this scenario, the plateau observed at low…

Strongly Correlated Electrons · Physics 2015-06-04 P. Quémerais , P. McClarty , R. Moessner

Experimental investigation of the resistivity $\rho$, susceptibility $\chi$, specific heat C$_p$, and Hall coefficient R$_H$ of the pyrochlore Cd$_2$Re$_2$O$_7$ reveals the presence of a continuous phase transition of uncertain origin with…

Strongly Correlated Electrons · Physics 2016-08-31 R. Jin , J. He , J. R. Thompson , M. F. Chisholm , B. C. Sales , D. Mandrus

We present a model which accounts for the high field magnetisation at very low temperature in two pyrochlore frustrated systems, Er2Ti2O7 and Tb2Ti2O7. The two compounds present very different ground states: Er2Ti2O7, which has a planar…

Strongly Correlated Electrons · Physics 2015-06-15 Pierre Bonville , Sylvain Petit , Isabelle Mirebeau , Julien Robert , Elsa Lhotel , Carley Paulsen

We present neutron scattering spectra taken from a single crystal of Na0.75CoO2, the precursor to a novel cobalt-oxide superconductor. The data contain a prominent inelastic signal at low energies (~10 meV), which is localized in wavevector…

Strongly Correlated Electrons · Physics 2009-11-10 A. T. Boothroyd , R. Coldea , D. A. Tennant , D. Prabhakaran , L. M. Helme , C. D. Frost

Muon spin relaxation measurements on Bi2Ir2O7 show that it undergoes a bulk magnetic transition at 1.84(3) K. This is accompanied by increases in the muon spin relaxation rate and the amplitude of the non-relaxing part of the signal. The…

Strongly Correlated Electrons · Physics 2013-06-13 P. J. Baker , J. S. Moeller , F. L. Pratt , W. Hayes , S. J. Blundell , T. Lancaster , T. F. Qi , G. Cao

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

Neutron scattering measurements were performed to investigate magnetic excitations in a single-crystal sample of the ternary iron arsenide BaFe2As2, a parent compound of a recently discovered family of Fe-based superconductors. In the…

Strongly Correlated Electrons · Physics 2009-02-28 K. Matan , R. Morinaga , K. Iida , T. J. Sato

Frustration in magnetic interactions can give rise to disordered ground states with subtle and beautiful properties. The spin ices Ho2Ti2O7 and Dy2Ti2O7 exemplify this phenomenon, displaying a classical spin liquid state, with…

Strongly Correlated Electrons · Physics 2017-12-11 Mathieu Taillefumier , Owen Benton , Han Yan , L. D. C. Jaubert , Nic Shannon

Conventional crystalline magnets are characterized by symmetry breaking and normal modes of excitation called magnons with quantized angular momentum $\hbar$. Neutron scattering correspondingly features extra magnetic Bragg diffraction at…

Strongly Correlated Electrons · Physics 2018-10-31 K. W. Plumb , Hitesh J. Changlani , A. Scheie , Shu Zhang , J. W. Kriza , J. A. Rodriguez-Rivera , Yiming Qiu , B. Winn , R. J. Cava , C. L. Broholm