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Related papers: Molecular imaging using high-order harmonic genera…

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Real-space picture of electron recollision with the parent ion guides our understanding of the highly nonlinear response of atoms and molecules to intense low-frequency laser fields. It is also among several leading contestants for the…

Optics · Physics 2019-11-06 Mrudul M. S. , Adhip Pattanayak , Misha Ivanov , Gopal Dixit

Although it seems that obtaining quantum properties of light from classical calculations is a self-contradictory claim, it is shown here that a unified mechanism governs the three distinct measurements of high harmonic generation spectra…

Quantum Physics · Physics 2024-09-18 Nimrod Moiseyev

This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly…

Strongly Correlated Electrons · Physics 2022-04-06 R. E. F. Silva , Igor V. Blinov , Alexey N. Rubtsov , O. Smirnova , M. Ivanov

Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…

Strongly Correlated Electrons · Physics 2022-06-29 Takeshi Suzuki , Shik Shin , Kozo Okazaki

We present theoretical predictions of high-order harmonic generation (HHG) resulting from the interaction of short femtosecond laser pulses with metal nanotips. It has been demonstrated that high energy electrons can be generated using…

In conditions where the interaction betweeen an atom and a short high-frequency extreme ultraviolet laser pulse is a perturbation, we show that a simple theoretical approach, based on Coulomb-Volkov-type states, can make reliable…

Atomic Physics · Physics 2009-11-07 Guillaume Duchateau , Eric Cormier , Robert Gayet

In strong laser-atom interactions, the Coulomb potential can affect the trajectories of rescattering electron in high-order harmonic generation (HHG). Here, by constructing a semi-analytical Coulomb-included model and comparing it with…

Atomic Physics · Physics 2025-12-16 Yigen Peng , Jiayin Che , Ruihua Xu , Shang Wang , Xuejiao Xie , Yanjun Chen

We characterize the temporal profile of the high-order harmonic emission from ablation plasma plumes using cross-correlations with the infrared (IR) laser beam provided by 2-photon harmonic+IR ionization of rare gas atoms. We study both…

A theoretical optimization method of high-harmonic-generation (HHG) is developed in the framework of optimal-control-theory (OCT). The target of optimization is the emission radiation of a particular frequency. The OCT formulation includes…

Quantum Physics · Physics 2020-02-19 Ido Schaefer , Ronnie Kosloff

Alignment and orientation of molecules by intense, ultrashort laser fields are crucial for a variety of applications in physics and chemistry. These include control of high harmonics generation, molecular orbitals tomography, control of…

We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

We establish how the intensities of the higher harmonics that arise when a photoelectron recombines with a parent ion depend functionally on the parameters of the laser wave and atomic medium, and estimate the limiting values of these…

Optics · Physics 2017-04-19 M. A. Kutlan

We investigate how short and long electron trajectory contributions to high harmonic emission and their interferences give access to intra-molecular dynamics. In the case of unaligned molecules, we show experimental evidences that the long…

By using Bohmian trajectory method, we investigate the dynamic interference in diatomic molecular high-order harmonic generation progress. It is demonstrated that the main characteristics of the molecular harmonic spectrum can be well…

Atomic Physics · Physics 2013-08-05 Yang Song , Bing-Bing Wang , Fu-Ming Guo , Su-Yu Li , Xue-Shen Liu , Ji-Gen Chen , Si-Liang Zeng , Yu-Jun Yang

Globally optimal solution describing a phase conjugated field of Raman scattering on the resonant $B\gets X$ transition of iodine $I_2$ is studied. Maximum optical coherence is found as a top eigenvalue problem. A reversibility theorem has…

Optics · Physics 2009-09-29 V. M. Akulin , V. A. Dubovitskii , A. M. Dykhne , A. G. Rudavets

We perform a detailed analysis of high-order harmonic generation (HHG) in atoms within the strong field approximation (SFA) by considering spatially inhomogeneous monochromatic laser fields. We investigate how the individual pairs of…

Atomic Physics · Physics 2015-06-05 T. Shaaran , M. F. Ciappina , M. Lewenstein

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

We investigate high-order harmonic generation in inhomogeneous media for reduced dimensionality models. We perform a phase-space analysis, in which we identify specific features caused by the field inhomogeneity. We compute high-order…

Atomic Physics · Physics 2016-05-25 C. Zagoya , M. Bonner , H. Chomet , E. Slade , C. Figueira de Morisson Faria

The irradiation of atoms by a strong IR laser field of frequency $\omega$ results in the emission of odd-harmonics of $\omega$ ("IR harmonics") up to some maximal cut-off frequency. The addition of an XUV field of frequency…

Atomic Physics · Physics 2008-02-04 Avner Fleischer , Nimrod Moiseyev