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Related papers: Infrared dynamic polarizability of HD+ rovibration…

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We calculate the DC Stark effect for three molecular hydrogen ions in the non-relativistic approximation. The effect is calculated both in dependence on the rovibrational state and in dependence on the hyperfine state. We discuss special…

Atomic Physics · Physics 2015-06-19 Stephan Schiller , Dimitar Bakalov , Ashat K. Bekbaev , Vladimir I. Korobov

A systematic study of Ca+ atomic properties is carried out using high-precision relativistic all-order method where all single, double, and partial triple excitations of the Dirac-Fock wave functions are included to all orders of…

Atomic Physics · Physics 2015-05-20 M. S. Safronova , U. I. Safronova

An atom exposed to an electric field will experience Stark shifts of its internal energy levels, proportional to their polarizabilities. In optical frequency metrology, the Stark shift due to background black-body radiation (BBR) modifies…

The dynamic polarizabilities of the 4s, 3d and 4p states of Ca$^+$, are calculated using a relativistic structure model. The wavelengths at which the Stark shifts between different pairs of transitions are zero are computed. Experimental…

Atomic and Molecular Clusters · Physics 2015-06-15 Yong-Bo Tang , Hao-Xue Qiao , Ting-Yun Shi , J. Mitroy

The static and dynamic electric multipolar polarizabilities and second hyperpolarizabilities of the H$_2^+$, D$_2^+$, and HD$^+$ molecular ions in the ground and first excited states are calculated nonrelativistically using explicitly…

Atomic Physics · Physics 2014-09-23 Li-Yan Tang , Zong-Chao Yan , Ting-Yun Shi , James F. Babb

Homonuclear molecules have emerged as a crucial component in the pursuit of frequency standards, offering a promising avenue for the discovery of new physics phenomena that transcend the standard model. They also provide a unique approach…

Atomic Physics · Physics 2024-10-29 T. Zalialiutdinov , Y. Demidov , D. Solovyev

Precision measurements of transitions between singlet ($S=0$) Rydberg states of H$_2$ belonging to series converging on the $\mathrm{X}^+\,^2\Sigma_g^+(v^+=0,N^+=0)$ state of H$_2^+$ have been carried out by millimetre-wave spectroscopy…

Atomic Physics · Physics 2022-07-04 Nicolas Hölsch , Ioana Doran , Maximilian Beyer , Frédéric Merkt

The blackbody radiation (BBR) shift of the 5s - 4d_{5/2} clock transition in 88Sr+ is calculated to be 0.250(9) Hz at room temperature, T=300K, using the relativistic all-order method where all single and double excitations of the…

Atomic Physics · Physics 2015-05-13 Dansha Jiang , Bindiya Arora , M. S. Safronova , Charles W. Clark

The microwave clock frequency of the $|5s~^2S_{1/2}, F=0,m_F=0 \rangle \leftrightarrow |5s~^2S_{1/2}, F=1,m_F=0 \rangle$ transition in the $^{113}$Cd$^+$ ion has been reported as 15199862855.0192(10) Hz [Opt. Lett. {\bf 40}, 4249 (2015)].…

Atomic Physics · Physics 2017-11-29 Yan-mei Yu , B. K. Sahoo

We discuss possible search for optical transitions in Sm13+ and Sm14+ using ab initio calculations of differential dynamic polarizability. We calculate dynamic polarizability for M1 transition between first and second excited states of…

Atomic Physics · Physics 2015-06-17 A. Kozlov , V. A. Dzuba , V. Flambaum

We evaluated the static and dynamic polarizabilities of the 5s^2 ^1S_0 and 5s5p ^3P_0^o states of Sr using the high-precision relativistic configuration interaction + all-order method. Our calculation explains the discrepancy between the…

Atomic Physics · Physics 2015-06-11 M. S. Safronova , S. G. Porsev , U. I. Safronova , M. G. Kozlov , Charles W. Clark

We have measured the Stark shift of the $A^2\Pi_{1/2} - X^2\Sigma^+$ transition in YbF. We use a molecular beam triple resonance method, with two laser transitions acting as pump and probe, assisted by an rf transition that tags a single…

Atomic Physics · Physics 2009-11-11 P. C. Condylis , J. J. Hudson , M. R. Tarbutt , B. E. Sauer , E. A. Hinds

We present precise values of the dipole polarizabilities ($\alpha$) of the ground $\rm [4f^{14}6s] ~ ^2S_{1/2}$ and metastable $\rm [4f^{14} 5d] ~ ^2D_{3/2}$ states of Yb$^+$, that are %vital {\bf important} in reducing systematics in the…

Atomic Physics · Physics 2017-10-25 A. Roy , S. De , Bindiya Arora , B. K. Sahoo

Motivated by the prospect of an optical frequency standard based on 43Ca+, we calculate the blackbody radiation (BBR) shift of the 4s_1/2-3d_5/2 clock transition, which is a major component of the uncertainty budget. The calculations are…

Quantum Physics · Physics 2009-11-13 Bindiya Arora , M. S. Safronova , Charles W. Clark

We report the theoretical evaluations of the static scalar polarizability of the 133Cs ground state and of the black body radiation shift induced on the transition frequency between the two hyperfine levels with m_F = 0. This shift is of…

Atomic Physics · Physics 2009-11-10 S. Micalizio , A. Godone , D. Calonico , F. Levi , L. Lorini

We apply relativistic many-body methods to compute static differential polarizabilities for transitions inside the ground-state hyperfine manifolds of monovalent atoms and ions. Knowing this transition polarizability is required in a number…

Atomic Physics · Physics 2011-07-13 V. A. Dzuba , V. V. Flambaum , K. Beloy , A. Derevianko

The present work reports the spectroscopic parameters and molecular properties for the ground electronic state, $^1\Sigma^+$, of CdH$^+$, HgH$^{+}$, and YbH$^{+}$ molecular ions. We have used the state-of-the-art relativistic coupled…

Atomic Physics · Physics 2025-11-20 Ankush Thakur , Renu Bala , H. S. Nataraj

Molecular lattice clocks enable the search for new physics, such as fifth forces or temporal variations of fundamental constants, in a manner complementary to atomic clocks. Blackbody radiation (BBR) is a major contributor to the systematic…

Atomic Physics · Physics 2024-02-05 B. Iritani , E. Tiberi , W. Skomorowski , R. Moszynski , M. Borkowski , T. Zelevinsky

A comparative study of the effect of a static homogeneous electric field on the rovibrational spectra of several polar dimers in their $\textrm{X}^1\Sigma^+$ electronic ground state is performed. Focusing upon the rotational ground state…

Atomic Physics · Physics 2008-10-03 R. Gonzalez-Ferez , M. Mayle , P. Sanchez-Moreno , P. Schmelcher

We present a measurement of the dynamic scalar and tensor polarizabilities of the excited state 3D1 in atomic ytterbium. The polarizabilities were measured by analyzing the spectral lineshape of the 408-nm 1S0->3D1 transition driven by a…

Atomic Physics · Physics 2010-12-15 D. R. Dounas-Frazer , K. Tsigutkin , A. Family , D. Budker
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