Related papers: Doppler-free two-photon resonances for atom detect…
We explore a single-photon approach to Rydberg state excitation and Rydberg blockade. Using detailed theoretical models, we show the feasibility of direct excitation, predict the effect of background electric fields, and calculate the…
Dual-comb spectroscopy is a rapidly developing technique enabling ultraprecise broadband optical diagnostics of atoms and molecules. This powerful tool typically requires two phase-locked femtosecond lasers, yet it has been shown that it…
We introduce the first method to enable an optical amplification of a coherent Raman spectroscopy signal called radio frequency Doppler Raman spectroscopy. Doppler Raman measurements amplify the optical signals in coherent Raman…
We study the feasibility of nearly-degenerate two-photon rovibrational spectroscopy in ensembles of trapped, sympathetically cooled hydrogen molecular ions using a resonance-enhanced multiphoton dissociation (REMPD) scheme. Taking advantage…
Although Rydberg atoms have shown promise for use in novel types of radio frequency receivers, they have generally not been considered phase sensitive without the use of closed-loop interferometry or auxiliary radio frequency fields. Here,…
We report a direct measurement of the $7s\ ^2S_{1/2}\rightarrow$ $7p\ ^2P_{3/2}$ electric dipole transition frequency in $^{226}$Ra$^{+}$. With a single laser-cooled radium ion we determine the transition frequency to be 785722.11(3) GHz by…
We show that two-photon absorption (TPA) in Rubidium atoms can be greatly enhanced by the use of a hollow-core photonic bandgap fiber. We investigate off-resonant, degenerate Doppler-free TPA on the 5S1/2 - 5D5/2 transition and observe 1%…
Vacuum-stimulated Raman transitions are driven between two magnetic substates of a rubidium-87 atom strongly coupled to an optical cavity. A magnetic field lifts the degeneracy of these states, and the atom is alternately exposed to laser…
Dynamic stabilization of atomic hydrogen against ionization in high-frequency single- and two-color, circularly polarized laser pulses is observed by numerically solving the three-dimensional, time-dependent Schr\"odinger equation. The…
In this study, a dual-interrogation (DI) method was used to suppress the light shift in the Rb 778 nm 5S1/2-5D5/2 two-photon transition (TPT) optical frequency standard. The approach used an auxiliary system to calibrate the light shift of…
A three-step laser excitation scheme is used to make absolute frequency measurements of highly excited nF7/2 Rydberg states in 85Rb for principal quantum numbers n=33-100. This work demonstrates the first absolute frequency measurements of…
Photoionization of the rubidium (Rb) atoms cooled in a magneto-optical trap, characterized by the coexistence of the ground 5$S_{1/2}$ and the excited 5$P_{3/2}$ states, is investigated experimentally and theoretically with the 400 nm…
We present a space and time resolved interferometric plasma diagnostic for use on plasmas where neutral-bound electron contribution to the refractive index cannot be neglected. By recording simultaneously the plasma optical index at 532 and…
We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly…
Two-photon states generated through degenerate spontaneous parametric down-conversion (SPDC) can exhibit sharp correlations in the transverse spatial coordinates. This property leads to unique free-space propagation features. Here, we show…
We report measurements of an intensity-field correlation function of the resonance fluorescence of a single trapped Ba+ ion. Detection of a photon prepares the atom in its ground state and we observe its subsequent evolution under…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
We demonstrate a dual wavelength optical frequency standard based on the dual optical transition modulation transfer spectroscopy (DOTMTS) between different quantum transitions of the rubidium D1 (795 nm) and D2 (780 nm) lines. In a single…
We report on the demonstration of Doppler-free polarization spectroscopy of the D2 line of 6Li atoms. Counterintuitively, the presence of an Ar buffer gas, in a certain pressure range, causes a drastic enhancement of the polarization…
Semiconductor lasers offer native bifunctionality enabling coherent light emission and linear photodetection. They can also operate as sensitive two-photon absorption detectors due to the third-order nonlinearity of the heterostructure…