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We experimentally demonstrate a one-color two-photon transition from the $5\mathit{S}_{1/2}$ ground state to the $6\mathit{S}_{1/2}$ excited state in rubidium (Rb) vapor using a continuous wave laser at 993 nm. The Rb vapor contains both…

Atomic Physics · Physics 2019-02-22 Thomas Nieddu , Tridib Ray , Krishnapriya S. Rajasree , Ritayan Roy , Síle Nic Chormaic

We report on Doppler-free laser spectroscopy in a Cs vapor cell using a dual-frequency laser system tuned on the Cs D$_1$ line. Using counter-propagating beams with crossed linear polarizations, an original sign-reversal of the usual…

Atomic Physics · Physics 2016-05-31 Moustafa Abdel Hafiz , Grégoire Coget , Emeric De Clercq , Rodolphe Boudot

Femtosecond high-order harmonic transient absorption spectroscopy is used to observe electromagnetically induced transparency-like behavior as well as induced absorption in the extreme ultraviolet by laser dressing of the He 2s2p (1Po) and…

Atomic Physics · Physics 2009-11-13 Zhi-Heng Loh , Chris H. Greene , Stephen R. Leone

Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb…

The $3p^{4}$ $^{3}$P$_{J}$ - $3p^{3}4p$ $^{3}$P$_{J}$ transition in the sulphur atom is investigated in a precision two-photon excitation scheme under Doppler-free and collision-free circumstances yielding an absolute accuracy of 0.0009…

Atomic Physics · Physics 2020-06-23 K. -F. Lai , E. J. Salumbides , W. Ubachs

Direct evidence of excitation of the 5p3/2 -> 6p3/2 electric dipole forbidden transition in atomic rubidium is presented. The experiments were performed in a room temperature rubidium cell with continuous wave extended cavity diode lasers.…

We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe…

We report measurements of absolute transition frequencies and hyperfine coupling constants for the 8S_{1/2}, 9S_{1/2}, 7D_{3/2}, and 7D_{5/2} states in ^{133}Cs vapor. The stepwise excitation through either the 6P_{1/2} or 6P_{3/2}…

We have performed high resolution spectroscopy of rubidium with a single mode continuous wave distributed feedback (DFB) laser diode. The saturation spectrum of the D_2-line of 85Rb and 87Rb was recorded with a resolution close to the…

Atomic Physics · Physics 2015-06-26 S. Kraft , A. Deninger , Ch. Truck , J. Fortagh , F. Lison , C. Zimmermann

The $6S_{1/2}-5D_{5/2}$ electric quadrupole transition is investigated in Cesium vapor at room temperature via nonlinear Doppler-free 6P-6S-5D three-level spectroscopy. Frequency-resolved studies of individual E2 hyperfine lines allow one…

We present experiments on two-photon excitation of ${\rm ^{87}}$Rb atoms to Rydberg states. For this purpose, two continuous-wave (cw)-laser systems for both 780 nm and 480 nm have been set up. These systems are optimized to a small…

Quantum Physics · Physics 2016-08-16 Axel Grabowski , Rolf Heidemann , Robert Löw , Jürgen Stuhler , Tilman Pfau

We perform a beat-frequency-resolved analysis for two-dimensional electronic spectroscopy using a high-speed and stable 2D electronic spectrometer and few-cycle visible laser pulses to disentangle the vibrational coherences in an artificial…

We demonstrate two techniques for studying the features of three-level systems driven by two lasers (called control and probe), when the transitions are Doppler broadened as in room-temperature vapor. For $\Lambda$-type systems, the probe…

Optics · Physics 2007-05-23 Umakant D. Rapol , Vasant Natarajan

The hybrid Stimulated Raman Scattering - Two Plasmon Decay instability had shown to play the dominant role for plasma waves excitation and energy absorption at interaction of very intense femtosecond obliquely incident $p$-polarized laser…

Plasma Physics · Physics 2021-01-04 I. Tsymbalov , D. Gorlova , A. Savel'ev

We demonstrate a new simple technique to measure IR frequencies near 30 THz using a femtosecond (fs) laser optical comb and sum-frequency generation. The optical frequency is directly compared to the distance between two modes of the fs…

In this work, we consider a three-level ladder-type atom driven by a coherent field, inspired by the experimental work of Gasparinetti et al. [Phys. Rev. A 100, 033802 (2019)]. When driven on two-photon resonance, the atom is excited into…

Quantum Physics · Physics 2025-10-06 Jacob Ngaha , Scott Parkins , Howard J. Carmichael

We demonstrate a technique to lock the frequency of a laser to a transition between two excited states in Rb vapor in the presence of a weak magnetic field. We use a ladder configuration from specific hyperfine sublevels of the 5S 1/2, 5P…

Optics · Physics 2015-05-13 F. E. Becerra , R. T. Willis , S. L. Rolston , L. A. Orozco

We investigate the prospects of using two-mode intensity squeezed twin-beams, generated in Rb vapor, to improve the sensitivity of spectroscopic measurements by engaging two-photon Raman transitions. As a proof of principle demonstration,…

Atomic Physics · Physics 2021-04-21 Nikunjkumar Prajapati , Ziqi Niu , Irina Novikova

Utilizing two-photon excitation in hot Rb vapor we demonstrate the generation of collimated optical fields at 420 nm and 1324 nm. Input laser beams at 780 nm and 776 nm enter a heated Rb vapor cell collinear and circularly polarized,…

Atomic Physics · Physics 2015-06-17 J. F. Sell , M. A. Gearba , B. D. DePaola , R. J. Knize

We have studied the resonance fluorescence of a room-temperature rubidium vapor exited to the atomic 5P3/2 state (D2 line) by powerful single-frequency cw laser radiation (1.25 W/cm^2) in the presence of a magnetic field. In these studies,…

Atomic Physics · Physics 2009-11-13 A. Atvars , M. Auzinsh , E. A. Gazazyan , A. V. Papoyan , S. V. Shmavonyan