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The large number of degrees of freedom involved in polaritonic chemistry processes considerably restricts the systems that can be described by any ab initio approach, due to the resulting high computational cost. Semiclassical methods that…

An implementation of the Hartree-Fock (HF) method capable of robust convergence for well-behaved arbitrary central potentials is presented. The Hartree-Fock equations are converted to a generalized eigenvalue problem by employing a B-spline…

Atomic Physics · Physics 2021-08-13 D. T. Waide , D. G. Green , G. F. Gribakin

We study the electronic structure of a strongly correlated d-wave superconducting state. Combining a renormalized mean field theory with direct calculation of matrix elements, we obtain explicit analytical results for the nodal Fermi…

Superconductivity · Physics 2009-11-11 Bernhard Edegger , V. N. Muthukumar , Claudius Gros , P. W. Anderson

Kohn-Sham spin-density functional theory provides an efficient and accurate model to study electron-electron interaction effects in quantum dots, but its application to large systems is a challenge. An efficient algorithm for the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Hong Jiang , Harold U. Baranger , Weitao Yang

Two of the most widely used electronic structure theory methods, namely Hartree-Fock and Kohn-Sham density functional theory, both requires the iterative solution of a set of Schr\"odinger-like equations. The speed of convergence of such…

Chemical Physics · Physics 2024-06-06 S. Hazra , U. Patil , S. Sanvito

This study presents a refined approach to computing the electronic structure of indium antimonide (InSb) using advanced \textit{ab initio} techniques with the In and Sb $4d^{10}$ semicore electrons included in the valence states. These…

Materials Science · Physics 2025-08-04 Ritwik Das , Anne-Sophie Grimault-Jacquin , Frédéric Aniel

The cranked relativistic Hartree+Bogoliubov theory has been applied for a systematic study of the nuclei around 254No, the heaviest elements for which detailed spectroscopic data are available. The deformation, rotational response, pairing…

Nuclear Theory · Physics 2009-11-10 A. V. Afanasjev , T. L. Khoo , S. Frauendorf , G. A. Lalazissis , I. Ahmad

We present a density matrix approach for computing global solutions of restricted open-shell Hartree-Fock theory, based on semidefinite programming (SDP), that gives upper and lower bounds on the Hartree-Fock energy of quantum systems.…

Chemical Physics · Physics 2014-04-22 Srikant Veeraraghavan , David A. Mazziotti

A systematic investigation of even-even superheavy elements in the region of proton numbers $100 \leq Z \leq 130$ and in the region of neutron numbers from the proton-drip line up to neutron number $N=196$ is presented. For this study we…

Nuclear Theory · Physics 2016-04-27 S. E. Agbemava , A. V. Afanasjev , T. Nakatsukasa , P. Ring

Hamiltonian and Schrodinger evolution equations on finite-dimensional projective space are analyzed in detail. Hartree-Fock (HF) manifold is introduced as a submanifold of many electron projective space of states. Evolution equations, exact…

Chemical Physics · Physics 2011-11-10 A. I. Panin

We benchmark angular-momentum projected{-after-variation} Hartree-Fock calculations as an approximation to full configuration-interaction results in a shell model basis. For such a simple approximation we find reasonably good agreement…

Nuclear Theory · Physics 2021-11-12 Stephanie M. Lauber , Hayden C. Frye , Calvin W. Johnson

Computing many-body ground state energies and resolving electronic structure calculations are fundamental problems for fields such as quantum chemistry or condensed matter. Several quantum computing algorithms that address these problems…

Quantum Physics · Physics 2023-01-12 Karen J. Morenz Korol , Kenny Choo , Antonio Mezzacapo

A systematic study of 160 heavy and super-heavy nuclei is performed in the Hartree-Fock-Bogoliubov approach with the finite range and density dependent Gogny force with the D1S parameter set. We show calculations in several approximations:…

Nuclear Theory · Physics 2015-06-04 M. Warda , J. L. Egido

We explore the existence and behaviour of holomorphic restricted Hartree-Fock (h-RHF) solutions for two-electron problems. Through algebraic geometry, the exact number of solutions with $n$ basis functions is rigorously identified as…

Chemical Physics · Physics 2018-01-15 Hugh G. A. Burton , Mark Gross , Alex J. W. Thom

Recent experimental progress in the field of cavity quantum electrodynamics allows to study the regime of strong interaction between quantized light and complex matter systems. Due to the coherent coupling between photons and matter-degrees…

Quantum Physics · Physics 2021-02-24 Florian Buchholz

Within the nuclear density functional theory (DFT) we study the effect of reflection-asymmetric shapes on ground-state binding energies and binding energy differences. To this end, we developed the new DFT solver AxialHFB that uses an…

Nuclear Theory · Physics 2013-03-05 E. Olsen , J. Erler , W. Nazarewicz , M. Stoitsov

Finding the ground state energy of electrons subject to an external electric field is a fundamental problem in computational chemistry. We prove that this electronic-structure problem, when restricted to a fixed single-particle basis and…

Quantum Physics · Physics 2021-03-16 Bryan O'Gorman , Sandy Irani , James Whitfield , Bill Fefferman

We formulate a new Hartree-Fock-Bogoliubov method applicable to weakly bound deformed nuclei using the coordinate-space Green's function technique. An emphasis is put on treatment of quasiparticle states in the continuum, on which we impose…

Nuclear Theory · Physics 2009-12-17 Hiroshi Oba , Masayuki Matsuo

We extend our analysis of two electrons on a sphere [Phys. Rev. A {\bf 79}, 062517 (2009); Phys. Rev. Lett. {\bf 103}, 123008 (2009)] to electrons on concentric spheres with different radii. The strengths and weaknesses of several…

Other Condensed Matter · Physics 2010-08-17 Pierre-François Loos , Peter M. W. Gill

Important features of low-frequency collective vibrational excitations in neutron drip line nuclei are studied. We emphasize that pairing anti-halo effect in the Hartree-Fock-Bogoliubov (HFB) theory play crucial roles to realize collective…

Nuclear Theory · Physics 2015-06-26 Masayuki Yamagami