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Motivated by the discovery of multiferroicity in the geometrically frustrated triangular antiferromagnet CuCrO$_2$ below its N\'eel temperature $T_N$, we investigate its magnetic and ferroelectric properties using ab initio calculations and…

Materials Science · Physics 2017-10-23 Ahmed Albaalbaky , Yaroslav Kvashnin , Denis Ledue , Renaud Patte , Raymond Frésard

Evidence for the quasi one-dimensional (1D) antiferromagnetism of CuO is presented in a framework of Heisenberg model. We have obtained an experimental absolute value of the paramagnetic spin susceptibility of CuO by subtracting the orbital…

Strongly Correlated Electrons · Physics 2009-11-10 T. Shimizu , T. Matsumoto , A. Goto , T. V. Chandrasekhar Rao , K. Yoshimura , K. Kosuge

We present a theoretical and experimental study of a quasi-one-dimensional zigzag antiferromagnet (N_2H_5)CuCl_3, which can be viewed as weakly coupled Heisenberg chains with a frustrated interaction. We first discuss generic features of…

Strongly Correlated Electrons · Physics 2009-11-07 N. Maeshima , M. Hagiwara , Y. Narumi , K. Kindo , T. C. Kobayashi , K. Okunishi

CuTeO4 has been proposed as a crystallographically distinct, yet electronic structure analog, of the superconducting cuprates. Here, we present detailed characterization of the of the physical properties of CuTeO4 to address this proposal.…

Strongly Correlated Electrons · Physics 2024-05-31 Zubia Hasan , Eli Zoghlin , Michal J. Winiarski , Kathryn E. Arpino , Thomas Halloran , Thao T. Tran , Tyrel M. McQueen

The magnetic properties of a new family of molecular-based quasi-two dimension $S=1/2$ Heisenberg antiferromagnets are reported. Three compounds, ($Cu(pz)_2(ClO_4)_2$, $Cu(pz)_2(BF_4)_2$, and $[Cu(pz)_2(NO_3)](PF_6)$) contain similar planes…

Based on density functional calculations, we present a detailed theoretical study of the electronic structure and the magnetic properties of the quasi-one dimensional chain cuprate Li_2ZrCuO_4 (Li_2CuZrO_4). For the relevant ratio of the…

Strongly Correlated Electrons · Physics 2015-05-14 M. Schmitt , J. Malek , S. -L. Drechsler , H. Rosner

We report on high-field magnetization, specific-heat and electron spin resonance (ESR) studies of the quasi-two-dimensional spin-1/2 Heisenberg antiferromagnet [Cu(pyz)2(HF2)]PF6. The frequency-field diagram of ESR modes below TN = 4.38 K…

Strongly Correlated Electrons · Physics 2011-03-10 E. Cizmar , S. A. Zvyagin , R. Beyer , M. Uhlarz , M. Ozerov , Y. Skourski , J. L. Manson , J. A. Schlueter , J. Wosnitza

Magnetic properties of AMoOPO$_4$Cl (A = K, Rb) with Mo$^{5+}$ ions in the 4$d^1$ electronic configuration are investigated by magnetization, heat capacity and NMR measurements on single crystals, combined with powder neutron diffraction…

Temperature dependent EPR studies were performed on a single crystal of CuSiO3.This recently discovered compound is isostructural with the spin-Peierls compound CuGeO3. The EPR signals show different characteristics than those of CuGeO3 and…

Strongly Correlated Electrons · Physics 2007-05-23 J. Sichelschmidt , A. Loidl , M. Baenitz , H. H. Otto , C. Geibel , F. Steglich

Magnetic properties of a quasi one-dimensional magnet CuV_2O_6 have been studied by means of susceptibility measurement, NMR and powder neutron diffraction. Cu^{2+} spins (S=1/2) order antiferromagnetically below 22.6 K, and the saturation…

Strongly Correlated Electrons · Physics 2009-10-31 Jun Kikuchi , Kazuhiro Ishiguchi , Kiyoichiro Motoya , Masayuki Itoh , Kazunori Inari , Naotoshi Eguchi , Jun Akimitsu

From experimental and theoretical analyses of magnetic and specific-heat properties, we present the complete magnetic phase diagram of the quasi-one-dimensional antiferromagnet Cu(N$_2$H$_5$)$_2$(SO$_4$)$_2$. On cooling and at zero magnetic…

Strongly Correlated Electrons · Physics 2016-11-23 A. Paduan-Filho , A. P. Vieira , J. G. A. Ramon , R. S. Freitas

This paper presents results of a recent study of multiferroic \CCO\ by means of single crystal neutron diffraction. This system has two close magnetic phase transitions at $T\nsub{N1}=24.2$ K and $T\nsub{N2}=23.6$ K. The low temperature…

Materials Science · Physics 2015-05-30 M. Frontzek , G. Ehlers , A. Podlesnyak , H. Cao , M. Matsuda , O. Zaharko , N. Aliouane , S. Barilo , S. V. Shiryaev

In a frustrated J_1-J_2 chain with the nearest-neighbor ferromagnetic interaction J_1 and the next-nearest-neighbor antiferromagnetic interaction J_2, novel magnetic states such as a spin-nematic state are theoretically expected. However,…

The minimal model to describe many spin chain materials with ferroelectric properties is the Heisenberg model with ferromagnetic nearest neighbor coupling J1 and antiferromagnetic next-nearest neighbor coupling J2. Here we study the…

Strongly Correlated Electrons · Physics 2010-02-17 J. Sirker

We report the results of muon-spin relaxation measurements on the low-dimensional antiferromagnet Rb4Cu(MoO4)3. No long-range magnetic order is observed down to 50 mK implying a ratio T_N/J<0.005 (where J is the principal exchange strength…

Strongly Correlated Electrons · Physics 2014-01-17 T. Lancaster , P. J. Baker , F. L. Pratt , S. J. Blundell , W. Hayes , D. Prabhakaran

We report structural and magnetic properties of the spin-$\frac12$ quantum antiferromagnet Cu[C$_6$H$_2$(COO)$_4$][C$_2$H$_5$NH$_3$]$_2$ by means of single-crystal x-ray diffraction, magnetization, heat capacity, and electron spin resonance…

Experimental data for the magnetic susceptibility and magnetostriction of CuGeO_3 are analyzed within a one-dimensional antiferromagnetic model with nearest ({J_1}) and next-nearest neighbour interactions ({J_2}). We show that the ratio of…

Strongly Correlated Electrons · Physics 2016-08-31 K. Fabricius , A. Klümper , U. Löw , B. Büchner , T. Lorenz

CuSiO_3, isotypic to the spin - Peierls compound CuGeO_3, was discovered recently as a metastable decomposition product of the silicate mineral dioptase, Cu_6Si_6O_{18}\cdot6H_2O. We investigated the physical properties of CuSiO_3 using…

Strongly Correlated Electrons · Physics 2009-10-31 M. Baenitz , C. Geibel , M. Dischner , G. Sparn , F. Steglich , H. H. Otto , M. Meibohm , A. A. Gippius

The magnetic susceptibility and magnetization of two new layered S=1/2 Heisenberg antiferromagnets with moderate exchange are reported. The two isostructural compounds, (2-amino-5-chloropyridinium)2CuBr4 ((5CAP)2CuBr4) and…

Materials Science · Physics 2009-11-07 F. M. Woodward , A. S. Albrecht , C. M. Wynn , C. P. Landee , M. M. Turnbull

We report an experimental and theoretical study of the low-temperature specific heat $C$ and magnetic susceptibility $\chi$ of the layered anisotropic triangular-lattice spin-1/2 Heisenberg antiferromagnets Cs$_2$CuCl$_{4-x}$Br$_x$ with $x$…

Strongly Correlated Electrons · Physics 2019-10-10 U. Tutsch , O. Tsyplyatyev , M. Kuhnt , L. Postulka , B. Wolf , P. T. Cong , F. Ritter , C. Krellner , W. Aßmus , B. Schmidt , P. Thalmeier , P. Kopietz , M. Lang
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