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X-ray cavity quantum optics with inner-shell transitions has been hindered by the overlap between resonant and continuum states. Here, we report the first experimental demonstration of cavity-controlled co-to-core resonant inelastic x-ray…

We study the magnetic excitation spectra in L-edge resonant inelastic x-ray scattering (RIXS) from undoped cuprates. We analyze the second-order dipole allowed process that the strong perturbation works through the intermediate state in…

Strongly Correlated Electrons · Physics 2013-05-30 Jun-ichi Igarashi , Tatsuya Nagao

We explore the general phenomenology of resonant inelastic scattering (RIXS) using CuB2O4, a network of CuO4 plaquettes electronically isolated by B+3 ions. Spectra show a small number of well-separated features, and we exploit the simple…

Strongly Correlated Electrons · Physics 2013-05-29 J. N. Hancock , G. Chabot-Couture , Y. Li , G. Petrakovskii , K. Ishii , I. Jarrige , J. Mizuki , T. P. Devereaux , M. Greven

Resonant inelastic x-ray scattering (RIXS) is a widely used spectroscopic technique, providing access to the electronic structure and dynamics of atoms, molecules, and solids. However, RIXS requires a narrow bandwidth x-ray probe to achieve…

Taking spinon excitations in the quantum antiferromagnet CaCu2O3 as an example, we demonstrate that femtosecond dynamics of magnetic excitations can be probed by direct resonant inelastic x-ray scattering (RIXS). To this end, we isolate the…

Resonant inelastic X-ray scattering (RIXS) at the $L$-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the $K$-edge of…

We show that Resonant Inelastic X-ray scattering (RIXS) is sensitive to three-magnon excitations in cuprates. Even if it requires three electrons to simultaneously flip their spin, the RIXS tri-magnon scattering amplitude is not small. At…

Strongly Correlated Electrons · Physics 2010-02-22 Luuk J. P. Ament , Jeroen van den Brink

We theoretically investigate the resonant inelastic X-ray scattering (RIXS) spectra in a quasi-1D chain of weakly coupled frustrated spin-1/2 trimers, as realized in Na$_{2}$Cu$_{3}$Ge$_{4}$O$_{12}$, with Cu $d^{9}$ 1/2 spins. We compute…

Strongly Correlated Electrons · Physics 2024-10-22 Prabhakar , Subhajyoti Pal , Umesh Kumar , Manoranjan Kumar , Anamitra Mukherjee

We present a resonant inelastic x-ray scattering (RIXS) study of spin and charge excitations in overdoped La1.77Sr0.23CuO4 along two high-symmetry directions. The line shape of these excitations is analyzed and they are shown to be highly…

Superconductivity · Physics 2016-02-05 C. Monney , T. Schmitt , C. E. Matt , J. Mesot , V. N. Strocov , O. J. Lipscombe , S. M. Hayden , J. Chang

We investigate magnetic excitations in the spin-ladder compound Sr$_{14}$Cu$_{24}$O$_{41}$ using high-resolution Cu $L_3$-edge Resonant Inelastic X-ray Scattering (RIXS). Our findings demonstrate that RIXS couples to collective spin…

This review aims to introduce the x-ray emission spectroscopy (XES) and resonant inelastic x-ray scattering (RIXS) techniques to the materials scientist working with magnetic semiconductors (e.g. semiconductors doped with 3d transition…

Materials Science · Physics 2014-01-20 Mauro Rovezzi , Pieter Glatzel

We determine the spin-exchange dynamical structure factor of the Heisenberg spin chain, as is measured by indirect Resonant Inelastic X-ray Scattering (RIXS). We find that two-spin RIXS excitations nearly entirely fractionalize into *two…

Strongly Correlated Electrons · Physics 2012-12-03 Antoine Klauser , Jorn Mossel , Jean-Sebastien Caux , Jeroen van den Brink

Su-Schrieffer-Heeger (SSH)-like electron-phonon (e-ph) interactions can drive the formation of light (bi)polarons and several novel states of matter. It is, therefore, prudent to develop experimental protocols for identifying such couplings…

Strongly Correlated Electrons · Physics 2024-12-23 Debshikha Banerjee , Jinu Thomas , Alberto Nocera , Steven Johnston

Quasi-one-dimensional systems exhibit many-body effects elusive in higher dimensions. A prime example is spin-orbital separation, which has been measured by resonant inelastic X-ray scattering (RIXS) in Sr$_2$CuO$_3$. Here, we theoretically…

Strongly Correlated Electrons · Physics 2022-10-03 Aaron Müller , Francesco Grandi , Martin Eckstein

We develop a method to study the effect of the superconducting transition on resonant inelastic X-ray scattering (RIXS) signal in superconductors with an order parameter with an arbitrary symmetry within a quasiparticle approach. As an…

Superconductivity · Physics 2016-09-28 Yifei Shi , David Benjamin , Eugene Demler , Israel Klich

Resonant X-ray scattering (RXS) is a spectroscopy where both the power of site selective diffraction and the power of local absorption spectroscopy regarding atomic species are combined. By virtue of the dependence on the core level state…

Materials Science · Physics 2007-11-12 Yves Joly , Elena S. Nazarenko , José-Emilio Lorenzo , Sergio Di Matteo , Calogero R. Natoli

Resonant (elastic) soft x-ray scattering (RSXS) offers a unique element, site, and valence specific probe to study spatial modulations of charge, spin, and orbital degrees of freedom in solids on the nanoscopic length scale. It cannot only…

Materials Science · Physics 2013-04-12 J. Fink , E. Schierle , E. Weschke , J. Geck

The resonant X-ray scattering (magnetic elastic, RXMS, and inelastic, RIXS) of Ir$^{4+}$ at the L$_{2,3}$ edges relevant to spin-orbit Mott insulators A$_{n+1}$Ir$_{n}$O$_{3n+1}$ (A=Sr, Ba, etc.) are calculated using a single-ion model…

Strongly Correlated Electrons · Physics 2014-01-28 M. Moretti Sala , S. Boseggia , D. F. McMorrow , G. Monaco

Here we propose to exploit the low energy bandwidth, small wavelength and penetration power of ultrashort pulses from XFELs for resonant Small Angle Scattering (SAXS) on plasma structures in laser excited plasmas. Small angle scattering…

Plasma Physics · Physics 2016-03-09 Thomas Kluge , M. Bussmann , H. -K. Chung , C. Gutt , L. G. Huang , M. Zacharias , U. Schramm , T. E. Cowan

While new light sources allow for unprecedented resolution in experiments with X-rays, a theoretical understanding of the scattering cross-section is lacking. In the particular case of strongly correlated electron systems, numerical…

Strongly Correlated Electrons · Physics 2023-05-29 Krissia Zawadzki , Alberto Nocera , Adrian E. Feiguin