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Hydrogen uptake into body-centered cubic (bcc) iron as a root cause for subsequent hydrogen embrittlement, is initiated at the surface. In this paper, we quantify how readily H diffuses from the surface into the bulk. We consider a set of…

Materials Science · Physics 2025-05-27 Lukas Meier , Asif I. Bhatti , Leo Kestens , Stefaan Cottenier

First-principles density-functional theory has been used to investigate equilibrium geometries, total energies, and diffusion barriers for H as an interstitial impurity absorbed in $\alpha$-Fe. Internal strains/stresses upon hydrogen…

Materials Science · Physics 2011-06-03 J. Sanchez , J. Fullea , C. Andrade , P. L. de Andres

We have studied the high-pressure iron bcc to hcp phase transition by simultaneous X-ray Magnetic Circular Dichroism (XMCD) and X-ray Absorption Spectroscopy (XAS) with an X-ray dispersive spectrometer. The combination of the two techniques…

Other Condensed Matter · Physics 2009-11-10 O. Mathon , F. Baudelet , J. P. Itie , A. Polian , M. D'Astuto , J. C. Chervin , S. Pascarelli

The mechanism of the {\alpha}-{\epsilon} transition in iron is reconsidered. A path in the Burgers description of the bcc/hcp transition different from those previously considered is proposed. It relies on the assumption that shear and…

Materials Science · Physics 2013-01-09 Bertrand Dupé , Bernard Amadon , Yves-Patrick Pellegrini , Christophe Denoual

The effect of interstitial hydrogen on the elastic properties of $\alpha$-iron is investigated using \textit{ab initio} density functional theory. We find that while the overall strength properties are reduced by H, the effects are mainly…

Materials Science · Physics 2012-09-14 D. Psiachos , T. Hammerschmidt , R. Drautz

We use the Gutzwiller Density Functional Theory to calculate ground-state properties and bandstructures of iron in its body-centered-cubic (bcc) and hexagonal-close-packed (hcp) phases. For a Hubbard interaction $U=9\, {\rm eV}$ and…

Strongly Correlated Electrons · Physics 2016-06-02 Tobias Schickling , Jörg Bünemann , Florian Gebhard , Lilia Boeri

Under high pressures, phase transition, as well as deformation twins, are constantly reported in many BCC metals, whose interactions are of fundamental importance to understand strengthen mechanism of these metals under extreme conditions.…

Materials Science · Physics 2017-10-11 Kun Wang , Jun Chena , Xueyang Zhang , Wenjun Zhu

The effect of hydrostatic strain and of interstitial hydrogen on the elastic properties of $\alpha$-iron is investigated using \textit{ab initio} density-functional theory calculations. We find that the cubic elastic constants and the…

Materials Science · Physics 2014-04-07 D. Psiachos , T. Hammerschmidt , R. Drautz

First-principles atomistic molecular dynamics simulation in the micro-canonical and canonical ensembles has been used to study the diffusion of interstitial hydrogen in $\alpha$-iron. Hydrogen to Iron ratios between $\theta=1/16 and 1/2…

Materials Science · Physics 2011-06-03 J. Sanchez , F. Fullea , M. C. Andrade , P. L. de Andres

The crystal structure of iron in the Earth's inner core remains debated. Most recent experiments suggest a hexagonal-close-packed (hcp) phase. In simulations, it has been generally agreed that the hcp-Fe is stable at inner core pressures…

Geophysics · Physics 2018-04-17 Rostislav Hrubiak , Yue Meng , Guoyin Shen

We investigate the thermodynamics and kinetics of a hydrogen interstitial in magnetic {\alpha}-iron, taking account of the quantum fluctuations of the proton as well as the anharmonicities of lattice vibrations and hydrogen hopping. We show…

Materials Science · Physics 2018-06-06 Bingqing Cheng , Anthony T. Paxton , Michele Ceriotti

Metastable phases can lead to multistep nucleation processes, influencing the liquid-to-solid transition in various systems. In this study, we investigate the homogeneous nucleation of iron's crystalline phases under Earth's inner core…

Geophysics · Physics 2025-04-04 Chen Gao , Kai-Ming Ho , Renata M. Wentzcovitch , Yang Sun

Structural defects in materials such as vacancies, grain boundaries, and dislocations may trap hydrogen and a local accumulation of hydrogen at these defects can lead to the degradation of the materials properties. An important aspect in…

Materials Science · Physics 2019-06-18 Yaojun A. Du , Jutta Rogal , Ralf Drautz

By introducing appropriate lattice parameters for a bi-lattice smoothly connecting the hexagonal close-packed (hcp) with the cuboidal structures, namely the body-centered (bcc) and the face centered cubic (fcc) lattices, we were able to map…

Materials Science · Physics 2025-02-17 Andres Robles-Navarro , Shaun Cooper , Odile R. Smits , Peter Schwerdtfeger

The structure and stability of iron near melting at multi-megabar pressures are of significant interest in high pressure physics and earth and planetary sciences. While the body-centered cubic (BCC) phase is generally recognized as unstable…

Materials Science · Physics 2025-06-27 Shuai Zhang , Aliza Panjwani , Penghao Xiao , Maitrayee Ghosh , Tadashi Ogitsu , Yuan Ping , S. X. Hu

Hydrogen atoms absorbed by metals in the hydrogen-containing environments can lead to the premature fracture of the metal components used in load-bearing conditions. Since metals used in practice are mostly polycrystalline, grain boundaries…

Materials Science · Physics 2018-09-17 Liang Wan , Wen Tong Geng , Akio Ishii , Jun-Ping Du , Nobuyuki Ishikawa , Hajime Kimizuka , Shigenobu Ogata

Molecular dynamics simulations are performed to investigate the structural phase transition in body-centered cubic (bcc) single crystal iron under high strain rate loading. We study the nucleation and growth of the hexagonal-close-packed…

Materials Science · Physics 2015-05-14 Baotian Wang , Jianli Shao , Guangcai Zhang , Weidong Li , Ping Zhang

Layered magnetic materials are becoming a major platform for future spin-based applications. Particularly the air-stable van der Waals compound CrSBr is attracting considerable interest due to its prominent magneto-transport and…

Solid-solid phase transitions in metals are traditionally driven by changes in density or external pressure. Here we show that, under strong electronic excitation, structural stability is governed by the interplay between electronic effects…

Materials Science · Physics 2026-04-27 S. Azadi , S. M. Vinko , A. Principi , T. D. Kuehne , M. S. Bahramy

We compute the equilibrium crystal structure and phase stability of iron at the alpha(bcc)-gamma(fcc) phase transition as a function of temperature, by employing a combination of ab initio methods for calculating electronic band structures…

Strongly Correlated Electrons · Physics 2015-05-19 I. Leonov , A. I. Poteryaev , V. I. Anisimov , D. Vollhardt
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