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Deformable colloids and macromolecules adsorb at interfaces, as they decrease the interfacial energy between the two media. The deformability, or softness, of these particles plays a pivotal role in the properties of the interface. In this…

Although common in nature, the self-assembly of small molecules at sold-liquid interfaces is difficult to control in artificial systems. The high mobility of dissolved small molecules limits their residence at the interface, typically…

In Molecular Dynamics (MD) simulations, interactions between water molecules and graphitic surfaces are often modeled as a simple Lennard-Jones potential between oxygen and carbon atoms. A possible method for tuning this parameter consists…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 Giulio Scocchi , Danilo Sergi , Claudio D'Angelo , Alberto Ortona

We establish the equivalence of a recently introduced discrete model of the hydrophobic interaction, as well as its extension to continuous state variables, with the Ising model in a magnetic field with temperature-dependent strength. In…

Statistical Mechanics · Physics 2016-08-15 G. M. Schütz , I. Ispolatov , G. T. Barkema , B. Widom

Coarse grained molecular dynamics simulations are presented in which the sensitivity of the ice nucleation rate to the hydrophilicity of a graphene nanoflake is investigated. We find that an optimal interaction strength for promoting ice…

Materials Science · Physics 2015-06-01 Stephen J. Cox , Shawn M. Kathmann , Ben Slater , Angelos Michaelides

Fluid flow through layered materials with different wetting behavior is observed in a wide range of applications in biological, environmental and technical systems. Therefore, it is necessary to understand the occuring transport mechanisms…

Fluid Dynamics · Physics 2022-02-01 Cynthia Michalkowski , Kilian Weishaupt , Veronika Schleper , Rainer Helmig

We present a multiparticle collision dynamics (MPC) implementation of layered immiscible fluids $A$ and $B$ of different shear viscosities separated by planar interfaces. The simulated flow profile for imposed steady shear motion and the…

Soft Condensed Matter · Physics 2021-09-07 Zihan Tan , Vania Calandrini , Jan K. G. Dhont , Gerhard Nägele , Roland G. Winkler

This is a fluid dynamics video illustrating the impact of ferrofluidic droplets on surfaces of variable wettability. Surfaces studied include mica, teflon, and superhydrophobic. A magnet is placed beneath each surface, which modifies the…

Fluid Dynamics · Physics 2010-10-19 D. A. Bolleddula , H. E. Dillon , A. Alliseda , P. Bhosale , J. C. Berg

The motion of an object within a viscous fluid and in the vicinity of a soft surface induces a hydrodynamic stress field that deforms the latter, thus modifying the boundary conditions of the flow. This results in elastohydrodynamic (EHD)…

Soft Condensed Matter · Physics 2023-06-22 Vincent Bertin , Yacine Amarouchene , Elie Raphael , Thomas Salez

Extremely compliant elastic materials, such as thin membranes or soft gels, can be deformed when wetted by a liquid drop. It is commonly assumed that the solid capillarity in "soft wetting" can be treated in the same manner as liquid…

Soft Condensed Matter · Physics 2019-09-11 Bruno Andreotti , Jacco H. Snoeijer

We analyze a minimal model for a rigid spherical microswimmer and explore the consequences of its extended surface on the interplay between its self-propulsion and flow properties. The model is the first order representation of…

Soft Condensed Matter · Physics 2017-12-06 Tapan Chandra Adhyapak , Sara Jabbari-Farouji

This work tests the statistical mechanical theory of hydrophobic interactions, isolates consequences of excluded volume interactions, and obtains B2 for those purposes. Cavity methods that are particularly appropriate for study of…

Biological Physics · Physics 2013-03-27 M. I. Chaudhari , S. Holleran , H. S. Ashbaugh , L. R. Pratt

Droplets on hydrophobic surfaces are ubiquitous in microfluidic applications and there exists a number of commonly used multicomponent and multiphase lattice Boltzmann schemes to study such systems. In this paper we focus on a popular…

Fluid Dynamics · Physics 2011-02-02 Sebastian Schmieschek , Jens Harting

Patterned surfaces with large effective slip lengths, such as super-hydrophobic surfaces containing trapped gas bubbles, have the potential to reduce hydrodynamic drag. Based on lubrication theory, we analyze an approach of a hydrophilic…

Fluid Dynamics · Physics 2015-03-14 Aleksey V. Belyaev , Olga I. Vinogradova

Soft particles display highly versatile properties with respect to hard colloids, even more so at fluid-fluid interfaces. In particular, microgels, consisting of a cross-linked polymer network, are able to deform and flatten upon adsorption…

We directly measured the interactions between a hydrophobic solid and a hydrophobic liquid separated by water using force spectroscopy, where colloidal probes were coated with graphene oxide (GO) to interact with immobilized heptane…

Soft Condensed Matter · Physics 2023-12-27 Avishi Abeywickrama , Douglas H. Adamson , Hannes C. Schniepp

The role of electrostatics on the interfacial properties of polyelectrolyte microgels has been discussed controversially in the literature. It is not yet clear if, or how, Coulomb interactions affect their behavior under interfacial…

Diamondoids are promising materials for applications in catalysis and nanotechnology. Since many of their applications are in aqueous environments, to understand their function it is essential to know the structure and dynamics of the water…

Mesoscale and Nanoscale Physics · Physics 2022-11-29 Karol Palczynski , Thorren Kirschbaum , Annika Bande , Joachim Dzubiella

We study the interactions between two negatively charged macroscopic surfaces confining positive counterions. A density-functional approach is introduced which, besides the usual mean-field interactions, takes into account the correlations…

Soft Condensed Matter · Physics 2015-06-25 A. Diehl , M. N. Tamashiro , Marcia C. Barbosa , Yan Levin

Graphene-water interaction has been under scrutiny ever since graphene discovery and realization of its exceptional properties. Several computational and experimental reports exist that have tried to look into the interactions involved,…

Materials Science · Physics 2020-02-19 Priyanka Solanky , Vidushi Sharma , Kamalika Ghatak , Jatin Kashyap , Dibakar Datta