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Distortions of the oxygen octahedra influence the fundamental electronic structure of perovskite oxides, such as their bandwidth and exchange interactions. Utilizing a fully ab-initio methodology based on density functional theory plus…

Strongly Correlated Electrons · Physics 2021-07-02 Alexander Hampel , Jeremy Lee-Hand , Antoine Georges , Cyrus E. Dreyer

The oxide heterostructure [(YFeO$_3$)$_5$(LaFeO$_3$)$_5$]$_{40}$, which is magnetically ordered and piezoelectric at room temperature, has been constructed from two weak ferromagnetic AFeO$_3$ perovskites with different A cations using…

Interface engineering in perovskite oxide superlattices has developed into a flourishing field, enabling not only further tuning of the exceptional properties, but also giving access to emergent physical phenomena. Here, we reveal a new…

Materials Science · Physics 2015-03-13 X. Z. Lu , X. G. Gong , H. J. Xiang

Magnetoelectric multiferroic materials, particularly with the perovskite structure, are receiving a lot of attention because of their inherent coupling between electrical polarization and magnetic ordering. However, very few types of direct…

Applied Physics · Physics 2017-09-07 Hong Jian Zhao , M. N. Grisolia , Yurong Yang , Jorge Iniguez , M. Bibes , Xiang Ming Chen , L. Bellaiche

Metal-organic frameworks (MOFs) possess a hybrid nature, combining the inorganic properties from the metal ions and the organic properties from the molecular linkers. Stroppa, \textit{et al.}, showed that the perovskite-type MOF…

Materials Science · Physics 2022-02-15 Kunihiro Yananose , Jaejun Yu

While nature provides a plethora of perovskite materials, only a few exhibits large ferroelectricity and possibly multiferroicity. The majority of perovskite materials have the non-polar CaTiO$_3$(CTO)structure, limiting the scope of their…

Materials Science · Physics 2022-05-25 Hongwei Wang , Fujie Tang , Massimiliano Stengel , Hongjun Xiang , Qi An , Tony Low , Xifan Wu

Engineering oxygen octahedra rotation patterns in $ABO_3$ perovskites is a powerful route to design functional materials. Here we propose a strategy that exploits point defects that create local electric dipoles and couple to the oxygen…

Materials Science · Physics 2022-07-12 Jiahui Jia , Xu He , Arsalan Akhtar , Gervasi Herranz , Miguel Pruneda

High-temperature electronic materials are in constant demand as the required operational range for various industries increases. Here we design $(A,A^\prime)B_2$O$_6$ perovskite oxides with [111] ``rock salt" $A$-site cation order and…

Materials Science · Physics 2014-06-11 Joshua Young , James M. Rondinelli

A key property that drives research in ferroelectric perovskite oxides is their strong piezoelectric response in which an electric field is induced by an applied strain, and vice-versa for the converse piezoelectric effect. We have achieved…

Materials Science · Physics 2015-06-11 J. Sinsheimer , S. J. Callori , B. Bein , Y. Benkara , J. Daley , J. Coraor , D. Su , P. W. Stephens , M. Dawber

Spin-polarized two-dimensional electron gas (2DEG) at oxide interfaces is an emerging physical phenomenon, which is technologically important for potential device applications. However, most previous relevant studies only focused on the…

Strongly Correlated Electrons · Physics 2021-11-01 Yakui Weng , Wei Niu , Xin Huang , Ming An , Shuai Dong

Strong coupling among spontaneous structural symmetric breaking, magnetism and metallicity in an intrinsic polar magnetic metal can give rise to novel physical phenomena and holds great promise for applications in spintronics. Here, we…

Materials Science · Physics 2025-11-04 Hong-Fei Huang , Houssam Sabri , Jiadong Zang , Jie-Xiang Yu

Methylammonium lead iodide, as related organometal halide perovskites, emerged recently as a particularly attractive material for photovoltaic applications. The origin of its appealing properties is sometimes assigned to its potential…

Materials Science · Physics 2022-04-04 Wen-Yi Tong , Jin-Zhu Zhao , Philippe Ghosez

The octahedron tilt transitions of ABX_3 perovskite-structure materials lead to an anti-polar (or antiferroelectric) arrangement of dipoles, with the low temperature structure having six sublattices polarized along various crystallographic…

Strongly Correlated Electrons · Physics 2013-05-29 Philip B. Allen , Yiing-Rei Chen , Santanu Chaudhuri , Clare P. Grey

The possibility that metals may support ferroelectricity is an open issue. Anderson and Blount showed that certain martensitic transitions involve inversion symmetry breaking and the formal existence of a polar axis, so 'metallic…

Materials Science · Physics 2016-04-08 Alessio Filippetti , Vincenzo Fiorentini , Francesco Ricci , Pietro Delugas , Jorge Íñiguez

The Pr$_{0.50}$Sr$_{0.5}$0CoO$_3$ perovskite exhibits unique magnetostructural properties among the rest of ferromagnetic/metallic Ln$_{0.50}$Sr$_{0.50}$CoO$_3$ compounds. The sudden orthorhombic-tetragonal (Imma $\to$ I4/mcm) structural…

It is demonstrated based on continuum mechanics modeling and simulation that it is possible to obtain polycrystalline ceramic ferroelectric materials which beggars single crystals in electromechanical properties. The local inhomogeneities…

Materials Science · Physics 2010-11-15 K. P. Jayachandran , J. M. Guedes , H. C. Rodrigues

It is of great interest to design and make materials in which ferroelectric polarisation is coupled to other order parameters such as lattice, magnetic and electronic instabilities. Such materials will be invaluable in next-generation data…

Strongly Correlated Electrons · Physics 2018-05-09 Wei-Tin Chen , Chin-Wei Wang , Hung-Cheng Wu , Fang-Cheng Chou , Hung-Duen Yang , Arkadiy Simonov , Mark S. Senn

With reduced dimensionality, it is often easier to modify the properties of ultra-thin films than their bulk counterparts. Strain engineering, usually achieved by choosing appropriate substrates, has been proven effective in controlling the…

Mesoscale and Nanoscale Physics · Physics 2017-10-31 S. Thomas , B. Kuiper , J. Hu , J. Smit , Z. Liao , Z. Zhong , G. Rijnders , A. Vailionis , R. Wu , G. Koster , J. Xia

Halide perovskite semiconductors respond to electric fields in a way that varies across time and length scales. We discuss the microscopic processes that give rise to the macroscopic polarization of these materials, ranging from the optical…

Materials Science · Physics 2018-12-04 Jacob N. Wilson , Jarvist M. Frost , Suzanne K. Wallace , Aron Walsh

Piezoelectrics play a critical role in various applications. The permanent dipole associated with the molecular cations in organometal-halide perovskites (OMHPs) may lead to spontaneous polarization and thus piezoelectricity. Here, we…

Materials Science · Physics 2015-12-17 Shi Liu , Fan Zheng , Ilya Grinberg , Andrew M. Rappe