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We explore the phase behavior and structure of orthogonal smectic liquid crystals consisting of bent-core molecules (BCMs) by means of Monte Carlo molecular simulations. A simple athermal molecular model is introduced that describes the…

Soft Condensed Matter · Physics 2016-07-26 Stavros D. Peroukidis , Alexandros G. Vanakaras , Demetri J. Photinos

We carry out Monte Carlo simulations to investigate the effect of molecular shape on liquid-crystal order. In our approach, each model mesogen consists of several soft spheres bonded rigidly together. The arrangement of the spheres may be…

Soft Condensed Matter · Physics 2009-11-07 J. Xu , R. L. B. Selinger , J. V. Selinger , R. Shashidhar

Recently, a new class of smectic liquid crystal phases (SmCP phases) characterized by the spontaneous formation of macroscopic chiral domains from achiral bent-core molecules has been discovered. We have carried out Monte Carlo simulations…

Statistical Mechanics · Physics 2009-11-07 Yves Lansac , Prabal K. Maiti , Noel A. Clark , Matthew A. Glaser

Recent liquid-crystalline (LC) research is focused on structurally new molecular systems distinct from simple nematic or smectic phases. Sophisticated molecular shape may reveal structural complexity, combining helicity and polarity.…

Many bent-core nematic liquid crystals exhibit unusual physical properties due to the presence of smectic clusters, known as "cybotactic" clusters in the nematic phase. Effect of these clusters on complex shear modulus ($G^*(\omega)$) of…

Using Monte Carlo simulation methods, we explore the role of molecular shape in the phase behavior of liquid crystals and the electroclinic effect. We study a "bent-rod" mesogen shaped like the letter Z, composed of seven soft spheres…

Soft Condensed Matter · Physics 2009-10-31 J. Xu , R. L. B. Selinger , J. V. Selinger , B. R. Ratna , R. Shashidhar

We present the phase diagram of a system of mesogenic top-shaped molecules based on the Parsons- Lee density functional theory and Monte Carlo simulation. The molecules are modeled as a hard spherocylinder with a hard sphere embedded in its…

Soft Condensed Matter · Physics 2011-06-13 D. de las Heras , S. Varga , F. J. Vesely

Two-dimensional ensembles of bent-core shaped molecules attain at highly orienting surfaces liquid crystalline structures characteristic mostly for lamellar chiral or nonchiral antiferroelectric order. Here, using the Onsager-type of…

Soft Condensed Matter · Physics 2016-06-13 Paweł Karbowniczek , Michał Cieśla , Lech Longa , Agnieszka Chrzanowska

Liquid crystals formed by acute-angle bent-core (ABC) molecules with a 1,7 naphthalene central core show an intriguing phase behavior with the nematic phase accompanied by poorly understood additional phases. In this work, we characterize…

The effects of dipolar interactions and molecular flexibility on the structure and phase behavior of bent-core molecular fluids are studied using Monte Carlo computer simulations. Some calculations of flexoelectric coefficients are also…

Soft Condensed Matter · Physics 2007-05-23 Alastair Dewar , Philip J. Camp

We have numerically studied a liquid composed of achiral, bent-shaped molecules built of tangent spheres. The system is known to spontaneously break mirror symmetry, as it forms a macroscopically chiral, twist-bend nematic phase [Phys. Rev.…

Soft Condensed Matter · Physics 2022-09-27 Piotr Kubala , Wojciech Tomczyk , Michał Cieśla

Liquid crystals (LCs) composed of mesogens play important roles in various scientific and engineering problems. How a system with many mesogens can enter a LC state is an interesting and important problem. Using stiff and free-joint…

We report a molecular dynamics simulation demonstrating that the Smectic B crystalline phase (Cr-B), commonly observed in mesogenic systems of anisotropic molecules, can be formed by a system of identical particles interacting via a…

Soft Condensed Matter · Physics 2013-12-16 A. Metere , T. Oppelstrup , S. Sarman , A. Laaksonen , M. Dzugutov

We study the effect of fluctuations in opening angle of bent-core molecules on stability of the nematic phases. The molecules are built out of two Gay-Berne centers of $\kappa = 4$, $\kappa ' = 5$, $\mu = 1$ and $\nu = 2$, each…

Soft Condensed Matter · Physics 2009-04-07 W. Jozefowicz , L. Longa

The bent-core liquid crystals (LCs) are highly regarded as the next-generation materials for electro-optic devices. The nematic (N) phase of these LCs possesses highly ordered smectic-like cybotactic clusters which are promising in terms of…

Soft Condensed Matter · Physics 2019-02-06 Sourav Patranabish , Yiwei Wang , Aloka Sinha , Apala Majumdar

Fibers of bent-core liquid crystals present an internal structure of a rolled smectic layer and can be used as optical waveguides. We used a field-theoretical Monte Carlo simulation to analyze the internal configuration of such fibers as a…

Soft Condensed Matter · Physics 2016-08-04 N. Atzin , O. Guzmán , J. J. de Pablo

We formulate a simple Landau type model describing macroscopic behaviour recently discovered new smectic phases composed of achiral bent-shaped molecules. Films of such smectics exhibit three types of ordering related to dipole…

Soft Condensed Matter · Physics 2007-05-23 E. I. Kats , J. Lajzerowicz

By molecular modeling we demonstrate that the nematic long-range order discovered in bent-core liquid crystal systems should reveal further spatially homogeneous phases. Two of them are identified as a tetrahedratic nematic ($N_T$) phase…

Soft Condensed Matter · Physics 2009-04-30 Lech Longa , Grzegorz Pająk , Thomas Wydro

We propose a continuum tensorial model for chiral smectic C (SmC$^*$) liquid crystals using a tensor-valued order parameter $\mathbf{Q}$ to describe orientational order and a real-valued order parameter $\delta\rho$ to capture layer…

Soft Condensed Matter · Physics 2025-09-09 Jingmin Xia , Jinbing Wu , Yucen Han

Nematic liquid crystals confined to geometrically as well as chemically patterned substrate on one end and a flat substrate with strong anchoring on the other is studied using non-Boltzmann Monte Carlo methods. We observe significant…

Soft Condensed Matter · Physics 2010-10-18 D. Jayasri , Regina Jose , K. P. N. Murthy , V. S. S. Sastry
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