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The dramatic slowing down of relaxation dynamics of liquids approaching the glass transition remains a highly debated problem, where the crux of the puzzle resides in the elusive increase of the activation barrier $\Delta E(T)$ with…

Soft Condensed Matter · Physics 2024-06-19 Geert Kapteijns , David Richard , Eran Bouchbinder , Thomas B. Schrøder , Jeppe C. Dyre , Edan Lerner

Hot-exciton relaxation in semiconductor nanocrystals (NCs) is often described using perturbative theories, but their accuracy is difficult to assess for realistic exciton--phonon Hamiltonians. Here, we benchmark the perturbative quantum…

By combining aspects of the coherent and self intermediate scattering functions, measured by dynamical light scattering on a suspension of hard sphere-like particles, we show that the arrest of particle number density fluctuations spreads…

Soft Condensed Matter · Physics 2015-05-13 W. van Megen , V. A. Martinez , G. Bryant

We present simulation results addressing the dynamics of a colloidal system with attractive interactions close to gelation. Our interaction also has a soft, long range repulsive barrier which suppresses liquid-gas type phase separation at…

Soft Condensed Matter · Physics 2007-05-23 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

A superfluid flow beyond a critical momentum in an optical lattice decays drastically by the interplay between nonlinearity due to the interparticle interactions in Bose-Einstein condensate and periodicity of the lattice; this instability…

Quantum Gases · Physics 2014-11-17 Rui Asaoka , Hiroki Tsuchiura , Makoto Yamashita , Yuta Toga

We present mode-coupling equations for the description of the slow dynamics observed in supercooled molecular liquids close to the glass transition. The mode-coupling theory (MCT) originally formulated to study the slow relaxation in simple…

Soft Condensed Matter · Physics 2009-10-31 L. Fabbian , A. Latz , R. Schilling , F. Sciortino , P. Tartaglia , C. Theis

Hybrid particle-field molecular dynamics is a molecular simulation strategy wherein particles couple to a density field instead of through ordinary pair potentials. Traditionally considered a mean-field theory, a momentum and…

Computational Physics · Physics 2023-02-03 Morten Ledum , Samiran Sen , Sigbjørn Løland Bore , Michele Cascella

Molecular dynamics simulations (mds) were carried out to investigate the reorientational motion of a rigid (fixed bond length), asymmetric diatomic molecule in the liquid and glassy states. In the latter the molecule reorients via…

Soft Condensed Matter · Physics 2015-06-04 D. Fragiadakis , C. M. Roland

We numerically study a nondisordered lattice spin system with a first order liquid-crystal transition, as a model for supercooled liquids and glasses. Below the melting temperature the system can be kept in the metastable liquid phase, and…

Statistical Mechanics · Physics 2009-11-07 Andrea Cavagna , Irene Giardina , Tomas S. Grigera

These lecture notes can be read in two ways. The first two Sections contain a review of the phenomenology of several physical systems with slow nonequilibrium dynamics. In the Conclusions we summarize the scenario derived from the solution…

Condensed Matter · Physics 2007-05-23 Leticia F. Cugliandolo

The generalized density matrix (GDM) method is used to calculate microscopically the parameters of the collective Hamiltonian. Higher order anharmonicities are obtained consistently with the lowest order results, the mean field…

Nuclear Theory · Physics 2011-09-23 L. Y. Jia

We review an scenario for the non-equilibrium dynamics of glassy systems that has been motivated by the exact solution of simple models. This approach allows one to set on firmer grounds well-known phenomenological theories. The old ideas…

Statistical Mechanics · Physics 2009-11-07 Leticia F. Cugliandolo

We develop a framework for understanding the difference between strong and fragile behavior in the dynamics of glass-forming liquids from the properties of the potential energy landscape. Our approach is based on a master equation…

Disordered Systems and Neural Networks · Physics 2015-05-30 Sumilan Banerjee , Chandan Dasgupta

We report a molecular dynamics (MD) study of the collective dynamics of a simple monatomic liquid -interacting through a two body potential that mimics that of lithium- across the liquid-glass transition. In the glassy phase we find…

Disordered Systems and Neural Networks · Physics 2009-11-07 T. Scopigno , G. Ruocco , F. Sette , G. Viliani

Recent theories predict that when a supercooled liquid approaches the glass transition, particle clusters with a special "amorphous order" nucleate within the liquid, which lead to static correlations dictating the dramatic slowdown of…

Soft Condensed Matter · Physics 2016-03-04 Bo Zhang , Xiang Cheng

The breakdown of the Stokes-Einstein (SE) law in fragile glassformers is examined by Molecular-Dynamics simulations of atomic liquids and polymers and consideration of the experimental data concerning the archetypical OTP glassformer. All…

Soft Condensed Matter · Physics 2018-05-09 F. Puosi , A. Pasturel , N. Jakse , D. Leporini

In this paper we extend the Gaussian self-consistent method to permit study of the equilibrium and kinetics of conformational transitions for heteropolymers with any given primary sequence. The kinetic equations earlier derived by us are…

Soft Condensed Matter · Physics 2009-10-31 E. G. Timoshenko , Yu. A. Kuznetsov , K. A. Dawson

We study the dynamics of a carrier, which performs a biased motion under the influence of an external field E, in an environment which is modeled by dynamic percolation and created by hard-core particles. The particles move randomly on a…

Statistical Mechanics · Physics 2009-10-31 O. Benichou , J. Klafter , M. Moreau , G. Oshanin

Low-energy excitations play a key role in all condensed-matter systems, yet there is limited understanding of their nature in glasses, where they correspond to local rearrangements of groups of particles. Here we introduce an algorithm to…

Soft Condensed Matter · Physics 2024-08-27 Wencheng Ji , Massimo Pica Ciamarra , Matthieu Wyart

We study the dynamics of the East model, comprising a chain of uncoupled spins in a downward-pointing field. Glassy effects arise at low temperatures $T$ from the kinetic constraint that spins can only flip if their left neighbour is up. We…

Statistical Mechanics · Physics 2007-05-23 P. Sollich , M. R. Evans
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