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We report the observation and systematic investigation of the space charge effect and mirror charge effect in photoemission spectroscopy. When pulsed light is incident on a sample, the photoemitted electrons experience energy redistribution…

Strongly Correlated Electrons · Physics 2007-05-23 X. J. Zhou , B. Wannberg , W. L. Yang , V. Brouet , Z. Sun , J. F. Douglas , D. Dessau , Z. Hussain , Z. -X. Shen

The ionization of an atom by a high-frequency intense laser pulse, where the energy of a single-photon is sufficient to ionize the system, is investigated from first principles. It is shown that as a consequence of an AC Stark effect in the…

Atomic Physics · Physics 2012-06-26 Philipp V Demekhin , Lorenz S Cederbaum

A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon…

We calculate the photoionization with excitation-to photoionization ratios for atomic helium and heliumlike ions at intermediate values of the photon energies. The final state interactions between the electrons are included in the lowest…

Quantum Physics · Physics 2009-11-13 E. G. Drukarev , E. Z. Liverts , M. Ya. Amusia , R. Krivec , V. B. Mandelzweig

We investigate electron momentum distributions from single ionization of Ar by two orthogonally polarized laser pulses of different color. The two-color scheme is used to experimentally control the interference between electron wave packets…

If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…

We present efficient and reliable molecular dynamics simulations of the photodissociation of dichloromethane followed by Coulomb explosion. These simulations are performed by calculating trajectories on accurate potential energy surfaces of…

Chemical Physics · Physics 2025-07-22 Yijue Ding

We report on kinematically complete measurements and ab initio non-perturbative calculations of double ionization of He and H2 by a single 800 eV circularly polarized photon. We confirm the quasifree mechanism of photoionization for H2 and…

Electron-beam propagation experiments have been used to determine the energy and angle dependence of electron-electron (ee) scattering a two-dimensional electron gas (2DEG) in a very direct manner by a new spectroscopy method. The…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 A. V. Yanovsky , H. Predel , H. Buhmann , R. N. Gurzhi , A. N. Kalinenko , A. I. Kopeliovich , L. W. Molenkamp

Two-photon exchange contributions to elastic electron-scattering are reviewed. The apparent discrepancy in the extraction of elastic nucleon form factors between unpolarized Rosenbluth and polarization transfer experiments is discussed, as…

High Energy Physics - Phenomenology · Physics 2008-11-26 Carl E. Carlson , Marc Vanderhaeghen

Photostimulated electron detachment from aqueous inorganic anions is the simplest example of solvent-mediated electron transfer. Here we contrast the behavior of halide anions with that of small polyatomic anions, such as pseudohalide…

We present the first numerical simulation of the time delay in the photoionization of the simplest diatomic molecule H$_2^+$ as observed by attosecond streaking. We show that the strong variation of the Eisenbud-Wigner-Smith time delay as a…

Photovoltaic effect of double quantum dots under nonuniform light field intensity has been studied theoretically. Comparing with the traditional p-n type photovoltaic effect, the inhomogeneous light field provides asymmetric potential…

Mesoscale and Nanoscale Physics · Physics 2022-05-23 Wenxi Lai

We present the first theoretical treatment of the formation of highly excited neutral H atoms (H$^{*}$) for strongly driven H$_{2}$. This process, with one electron ionizing and one captured in a Rydberg state, was recently reported in an…

Atomic Physics · Physics 2015-05-28 A. Emmanouilidou , D. Tchitchekova , C. Lazarou , U. Eichmann

We apply time-dependent R-matrix theory to study inner-shell ionization of C atoms in ultra-short high-frequency light fields with a photon energy between 170 and 245 eV. At an intensity of 10$^{17}$ W/cm$^2$, ionization is dominated by…

Atomic Physics · Physics 2015-08-12 H. F. Rey , H. W. van der Hart

Photoelectron ionization spectra of a system interacting with a neighbor two-level atom are investigated using the Laplace-transform method. These spectra are typically composed of several peaks. Photoelectron ionization spectra conditioned…

Quantum Physics · Physics 2015-05-27 Jan Perina , Antonin Luks , Wieslaw Leonski , Vlasta Perinova

Propylene oxide, a favorite target of experimental and theoretical studies of circular dichroism, was recently discovered in interstellar space, further amplifying the attention to its role in the current debate on protobiological…

We present a theoretical study of ionization of the hydrogen atom due to an XUV pulse in the presence of an IR laser with both fields linearly polarized in the same direction. In particular, we study the energy distribution of…

Atomic Physics · Physics 2017-08-23 A. A. Gramajo , R. Della Picca , D. G. Arbó

We calculate the differential cross-section of the direct double photo-ionization of He physisorbed on a polarizable surface. By including the influence of the surface potential in the correlated two-electron final state wavefunction, we…

Materials Science · Physics 2009-10-31 G. Goldoni

For a molecule, the two-center interference and the molecular scattering phase of the electron are important for almost all the processes that may occur in a laser field. In this study, we investigate their effects in the transfer of linear…

Atomic Physics · Physics 2018-12-19 Hao Liang , Mu-Xue Wang , Xiang-Ru Xiao , Qihuang Gong , Liang-You Peng