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We report the direct measurement of antiferromagnetic spin polarization at the oxygen sites in the multiferroic TbMn2O5, through resonant soft x-ray magnetic scattering. This supports recent theoretical models suggesting that the oxygen…

The electric polarization and its magnetic origins in multiferroic RMn2O5, where R is rare-earth ion, are still issues under debate. In this work, the temperature-dependent electric polarization of DyMn2O5, the most attractive member of…

Materials Science · Physics 2014-02-06 Z. Y. Zhao , M. F. Liu , X. Li , L. Lin , Z. B. Yan , S. Dong , J. -M. Liu

The commensurate and incommensurate magnetic structures of the magnetoelectric system YMn$_{2}$O$_{5}$, as determined from neutron diffraction, were found to be spin-density waves lacking a global center of symmetry. We propose a model,…

Materials Science · Physics 2009-11-11 L. C. Chapon , P. G. Radaelli , G. R. Blake , S. Park , S-W. Cheong

Neutron powder diffraction and single crystal x-ray resonant magnetic scattering measurements suggest that Dy plays an active role in enhancing the ferroelectric polarization in multiferroic DyMnO3 above TNDy = 6.5 K. We observe the…

Strongly Correlated Electrons · Physics 2007-05-23 O. Prokhnenko , R. Feyerherm , E. Dudzik , S. Landsgesell , N. Aliouane , L. C. Chapon , D. N. Argyriou

The ground state structural, electronic and magnetic properties of multiferroic TbMn$_2$O$_5$ are investigated via first-principles calculations. We show that the ferroelectricity in TbMn$_2$O$_5$ is driven by the non-centrosymmetric…

Materials Science · Physics 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

Cross-correlation between magnetic and dielectric properties has been attracting renewed interest because of the fundamental as well as technological importance of controlling the electric (magnetic) polarization by an external magnetic…

Strongly Correlated Electrons · Physics 2007-05-23 D. Higashiyama , N. Kida , S. Miyasaka , T. Arima , Y. Tokura

The low-temperature ferroelectric polarization of multiferroic $YMn_2O_5$ is completely reversed at a critical pressure of 10 kbar and the phase transition from the incommensurate to the commensurate magnetic phase is induced by pressures…

Strongly Correlated Electrons · Physics 2009-11-13 Rajit P. Chaudhury , Clarina R. dela Cruz , Bernd Lorenz , Yanyi Sun , Ching-Wu Chu , S. Park , Sang-W. Cheong

The magnetic, thermodynamic, and pyroelectric properties of LiFeP$_2$O$_7$ single crystals are investigated with emphasis on the magnetoelectric interaction of the electrical polarization with the magnetic order parameter. The magnetic…

Strongly Correlated Electrons · Physics 2012-09-13 K. -C. Liang , W. Zhang , B. Lorenz , Y. Y. Sun , P. S. Halasyamani , C. W. Chu

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

The electronic valence state of Mn in Pb(Zr0.2Ti0.8)O3/La0.8Sr0.2MnO3 multiferroic heterostructures is probed by near edge x-ray absorption spectroscopy as a function of the ferroelectric polarization. We observe a temperature independent…

Materials Science · Physics 2010-04-13 C. A. F. Vaz , J. Hoffman , Y. Segal , J. W. Reiner , R. D. Grober , Z. Zhang , C. H. Ahn , F. J. Walker

The structural, electronic and lattice dielectric properties of multiferroic TbMn$_2$O$_5$ are investigated using density functional theory within the generalized gradient approximation (GGA). We use collinear spin approximations and ignore…

Materials Science · Physics 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

Polarized neutron diffraction experiments have been performed on multiferroic materials $R$Mn$_{2}$O$_{5}$ ($R=$Ho, Er) under electric fields in the ferroelectric commensurate (CM) and the low-temperature incommensurate (LT-ICM) phases,…

Strongly Correlated Electrons · Physics 2015-05-13 S. Wakimoto , H. Kimura , M. Fukunaga , K. Nishihata , M. Takeda , K. Kakurai , Y. Noda , Y. Tokura

Neutron diffraction measurements under high magnetic fields have been performed for the multiferroic compound HoMn$_{2}$O$_{5}$. At zero field, high-temperature incommensurate magnetic (HT-ICM) -- commensurate magnetic (CM) --…

Strongly Correlated Electrons · Physics 2007-05-23 H. Kimura , Y. Kamada , Y. Noda , K. Kaneko , N. Metoki , K. Kohn

We have investigated the variation of induced ferroelectric polarization under magnetic field with various directions and magnitudes in a staggered antiferromagnet Ba$_2$CoGe$_2$O$_7$. While the ferroelectric polarization cannot be…

Strongly Correlated Electrons · Physics 2015-05-19 H. Murakawa , Y. Onose , S. Miyahara , N. Furukawa , Y. Tokura

A neutron scattering investigation of the magnetoelectric coupling in PbFe_{1/2}Nb_{1/2}O_{3} (PFN) has been undertaken. Ferroelectric order occurs below 400 K, as evidenced by the softening with temperature and subsequent recovery of the…

Materials Science · Physics 2018-07-20 C. Stock , S. R. Dunsiger , R. A. Mole , X. Li , H. Luo

We report observation of magneto-electric and magneto-dielectric couplings in ceramic Co3TeO6. Temperature dependent DC magnetization and dielectric constant measurements together indicate coupling between magnetic order and electronic…

Materials Science · Physics 2013-09-26 Harishchandra Singh , Haranath Ghosh , A. K. Sinha , M. N. Singh , G. Sharma , S. Patnaik , S. K. Deb

The electric polarization hysteresis loops and remanent polarization were revealed in multiferroics RMn$_2$O$_5$ with $R = Gd$ and $Bi$ at wide temperature interval from 5 K up to 330 K. Until recently, the long-range ferroelectric order…

Materials Science · Physics 2016-10-21 B. Kh. Khannanov , V. A. Sanina , E. I. Golovenchits , M. P. Scheglov

Ab initio calculations of the electric polarization of correlation-driven insulating materials, namely Mott insulators, have not been possible so far. Using a combination of density functional theory and dynamical-mean-field theory we study…

Materials Science · Physics 2014-12-11 R. Nourafkan , G. Kotliar , A. -M. S. Tremblay

Cu3Nb2O8 is an unusual multiferroic compound that undergoes a series of magnetic ordering at low temperatures. Concurrent development of electric polarization has been reported at TN1 ~25 K corresponding to a non-collinear helicoidal…

Strongly Correlated Electrons · Physics 2015-06-22 G. Sharma , J. Saha , S. D. Kaushik , V. Siruguri , S. Patnaik

Three independent contributions to the magnetically induced spontaneous polarization of multiferroic TbMn2O5 are uniquely separated by optical second harmonic generation and an analysis in terms of Landau theory. Two of them are related to…

Strongly Correlated Electrons · Physics 2012-03-07 N. Leo , D. Meier , R. V. Pisarev , N. Lee , S. -W. Cheong , M. Fiebig
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